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71.
Weikang Dong Ruishi Qi Tiansheng Liu Yi Li Ning Li Ze Hua Zirui Gao Shuyuan Zhang Kaihui Liu Jiandong Guo Peng Gao 《Advanced materials (Deerfield Beach, Fla.)》2020,32(46):2002014
Hyperbolic phonon polaritons (HPhPs) in orthorhombic-phase molybdenum trioxide (α-MoO3) show in-plane hyperbolicity, great wavelength compression, and ultralong lifetime, therefore holding great potential in nanophotonic applications. However, its polaritonic response in the far-infrared (FIR) range remains unexplored due to challenges in experimental characterization. Here, monochromated electron energy loss spectroscopy (EELS) in a scanning transmission electron microscope (STEM) is used to probe HPhPs in α-MoO3 in both mid-infrared (MIR) and FIR frequencies and correlate their behaviors with microstructures and orientations. It is found that low structural symmetry leads to various phonon modes and multiple Reststrahlen bands (RBs) over a broad spectral range (over 70 meV) and in different directions (55–63 meV and 119–125 meV along the b-axis, 68–106 meV along the c-axis, and 101–121 meV along the a-axis). These HPhPs can be selectively excited by controlling the direction of swift electrons. These findings provide new opportunities in nanophotonic and optoelectronic applications, such as directed light propagation, hyperlenses, and heat transfer. 相似文献
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In order to perform multi-dimensional data aggregation operations efficiently in edge computing-based Internet of things (IoT) systems, a new efficient privacy-preserving multi-dimensional data aggregation (EPMDA) scheme is proposed in this paper. EPMDA scheme is characterized by employing the homomorphic Paillier encryption and SM9 signature algorithm. To improve the computation efficiency of the Paillier encryption operation, EPMDA scheme generates a pre-computed modular exponentiation table of each dimensional data,and the Paillier encryption operation can be implemented by using only several modular multiplications. For the multi-dimensional data, the scheme concatenates zeros between two adjacent dimensional data to avoid data overflow in the sum operation of ciphertexts. To enhance security, EPMDA scheme sets random number at the high address of the exponent. Moreover, the scheme utilizes SM9 signature scheme to guarantee device authentication and data integrity. The performance evaluation and comparison show that EPMDA scheme is more efficient than the existing multi-dimensional data aggregation schemes. 相似文献
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对锂辉石-氧化钙烧结过程进行热力学分析,绘制了各反应Gibbs自由能与温度的关系图。结果表明,Al2O3会优先和Na2O、Li2O、K2O反应,然后与CaO反应生成CaO·Al2O3,而且烧结温度需高于1060℃以保证LiAlSi2O6能够完成晶形转变。并探讨了锂辉石-氧化钙烧结法提锂的反应机理。考察了不同烧结条件对锂浸出率的影响并对熟料进行X射线衍射(XRD)分析表征。实验结果表明,在配料比为1∶1.25、烧结温度1150℃、烧结时间60min时,锂的浸出率达到92.14%,熟料中的主要物相为Ca2SiO4与LiAlO2。利用XRD和扫描电镜-能谱联用仪(SEM-EDS)对熟料与浸出渣的物相、显微形貌及元素分布情况进行了分析表征。为了确定烧结反应的控制性步骤,在最优烧结条件的基础上对烧结过程进行动力学分析,结果表明,锂辉石-氧化钙烧结体系属于球形颗粒三维界面化学反应控制,烧结过程的动力学拟合方程为 。 相似文献
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考虑旋流衰减的影响,对气液螺旋环状流的压降特性进行研究并推导出了螺旋环状流压降预测模型。定义压降旋-直比系数为气液两相螺旋环状流和气液两相直流的压降之比,以此来表征旋流衰减对压降的影响。基于量纲分析的方法对压降旋-直比系数进行分析,推导出其表达式,压降旋-直比系数依赖于Lockhart-Martinelli 参数和气相Froude数变化。最终,得出了气液两相螺旋环状流的压降预测模型。在50 mm内径的水平管内对螺旋环状流的压降特性进行了实验研究,其中气相表观流速变化范围为10~16 m/s,体积含液率(LVF)变化范围为0.6%~4.8%。通过与实验数据进行对比,压降预测模型的相对误差在±15%以内,为工程应用提供了参考。 相似文献
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Anti-washout and tissue adhesion properties are essential for the clinical application of injectable bone materials. In this study, we prepared calcium phosphate cement (CPC) with anti-washout and tissue adhesion properties and attempted to build covalent bonds between CPC and the amino groups in bone tissue under a self-regulating pH system in the CPC (acidic to basic). The results of push-out tests demonstrated that a significant enhancement (from 6.42 ± 0.76 N to 61.5 ± 4.09 N) in tissue adhesion was obtained with the addition of 6% (w/w) oxidized sodium alginate (OSA) in CPC. The FTIR, XRD, anti-washout test, XPS, pH test, and SEM results suggested that the synergistic effect of OSA-citric acid (CA) led to the formation of a three-dimensional gel network structure in the CPC, and the Schiff base reaction between aldehyde and amino groups induced adhesion between CPC and the bone tissue. Further, the addition of less OSA had no significant negative effect on the hydration properties of CPC. Our work aims to promote the development of injectable bone material in clinical applications. 相似文献
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