西北太平洋热带气旋降水特征分析

利用1997—2006年GPCP(Global Precipitation Climatology Project)逐日卫星降水资料、上海台风研究所西北太平洋热带气旋资料,研究了近10年西北太平洋热带气旋降水的时空分布特征。发现整个西北太平洋区域多年平均TC(tropical cyclone)降水为175 mm,TC降水占总降水的比率为12%。年均TC降水场有两个极大值区域,分别位于菲律宾北部和菲律宾以东洋面。纬带平均的经向分布显示,总降水呈双峰分布,主、次峰值分别出现在6°N和35°N;而TC降水呈单峰分布,峰值出现在16°N。10年中TC降水以2004年最强;El Ni?o年TC降水在135°E以东偏多,而在南海中部和菲律宾至台湾等地区偏少;La Ni?a年TC降水在南海地区偏多,在菲律宾以东地区则显著偏少。     

西北太平洋风速垂直切变异常对热带气旋活动年际变化的影响

应用中国《台风年鉴》资料、欧洲中心40年月平均再分析资料和NOAA的逐月海温资料,研究了西北太平洋(5°—30°N,110°E—180°)风速垂直切变异常对热带气旋(TC)活动年际变化的影响。研究发现,西北太平洋所有TC、风暴以上级别的TC(TSTY,即达到热带风暴级别及以上的所有TC)和所有台风(WTY,包括台风、强台风和超强台风)年频数与西北太平洋风速垂直切变都显著负相关。西北太平洋风速垂直切变大小对生成源地在南海(5°—30°N,110°—120°E)TC和西北太平洋西部海域(5°—30°N,120°—150°E)TC的影响较小,而对西北太平洋东部海域(5°—30°N,150°E—180°)生成的TC影响最大:即西北太平洋风速垂直切变负异常年,有利于西北太平洋东部海域TC生成发展,使得负异常年较正异常年TC频数偏多和源地平均位置偏东;并且风速垂直切变的变化对TC频数和生成源地影响的显著性,随着TC强度的增加而增加。对TSTY生成环境场的进一步分析表明,西北太平洋风速垂直切变偏小年,季风槽偏强位置偏东,它的东端位于宽阔的太平洋洋面,与弱风速垂直切变区相配合,暖的海温加上低层强烈的正涡度和强烈辐合,且相应的高层有强的气流辐散区,这些环境场都有利于TSTY在主要源地尤其是西北太平洋东部海域生成,这是风速垂直切变偏小年TSTY偏多和生成源地偏东的重要原因。     

GFDL_RegCM对21世纪西北太平洋热带气旋活动的情景预估

首先评估了GFDL模式对西北太平洋热带气旋(TC)环境热力及动力因子的模拟性能,再利用夏威夷大学国际太平洋研究中心高分辨率区域气候模式( IPRC-RegCM),进行降尺度研究西北太平洋TC活动特征,在此基础上预估21世纪全球变暖背景下(A1B)西北太平洋TC活动的主要特点.结果显示,在西北太平洋TC活动区,GFDL控制试验的海平面温度(SST)比ERSST偏低.与NCEP/NCAR再分析资料相比,GFDL模拟的1980-1999年大尺度环流平均场表现为:副高脊线平均位置近乎一致,西伸脊点偏东,强度偏弱,面积偏小；季风槽槽线的范围偏小,强度偏弱；水平风垂直切变值在南海及菲律宾群岛海域偏小,而在160°E～170°W的20°N以南偏强.与NCEP/NCAR强迫的模拟结果相比,GFDL强迫得到的TC源地频数在南海偏少,菲律宾群岛以东海域偏多,两者的季节及年际变化特征相似.路径频数在南海北部和我国华南沿岸显著偏多.AlB情景下,西北太平洋TC生成数目将增加一倍,生成源地偏北且同时向东部洋而扩展,路径频数增多主要发生在20°N以北的中东部洋面上,移经西北太平洋西部的TC频数减少,由此影响我国的TC将减少.TC频数的季节分布发生较大变化,最多的月份在10月.TC平均强度增强,最大强度在10月增加最多,这与10月SST的增加和环境风切变的减小均为最大值有密切的关系.     

西北太平洋和南海不同时段生成热带气旋频数及其水汽条件的分类

对1961—2010年南海和西北太平洋不同时段生成热带气旋(tropical cyclone,TC)频数的时空分布及水汽条件对其产生的影响进行了分类研究。结果表明,可以将TC活动划分为活跃期(6—11月)和平静期(上年12—当年5月)两个时段。在TC活跃期和平静期,南海和西北太平洋上TC频数的EOF第一特征向量都表现为一致的增加或减少。活跃期EOF的第二特征向量表现为南海与西北太平洋中西部的TC频数存在相反的变化趋势,平静期EOF的第二特征向量则表现为130°E以西海域的TC频数与130~150°E范围内生成热带气旋存在相反的变化趋势。活跃期和平静期西北太平洋TC的生成频数与水汽通量散度均存在显著的负相关;而在活跃期南海TC频数与水汽通量散度仅在南海中北部有弱的负相关,在平静期南海东部到菲律宾附近海域有显著的负相关。因此,水汽条件的影响使得在活跃期南海和西北太平洋TC高频年中,南海北部和西北太平洋中东部TC频数明显偏多,而平静期高频年中,南海东部以及西北太平洋中西部TC频数明显偏多。     

赤道中东太平洋表层水温异常与热带气旋活动的统计关系

利用1950-2005年西北太平洋热带气旋(TC)和赤道中东太平洋表层水温(SST)资料,统计分析了赤道中东太平洋表层水温异常与TC频数、强度、源地和路径等的关系.结果表明,赤道中东太平洋暖异常年:(1)TC发生频数偏少,较常年平均偏少2～3个,但强度偏强,强台风和超强台风发生数偏多,较常年平均偏多1个左右,且随着暖异常强度的增强,TC发生频数偏少,强度增强愈加明显;(2)TC生成位置偏东偏南,145°E以东海区TC生成频数较冷异常年和La Nina年增加明显;(3)TC路径偏东,转向路径出现频次增加,西向路径出现频次减少,从而导致日本东部海区TC通过频数增加,而我国南海和华东沿海TC通过频数减少;(4)在我国登陆的TC频数偏少,较常年平均偏少1～2个.赤道中东太平洋冷异常年,情况基本与上相反.上述影响主要是由于赤道中东太平洋SST异常导致大气环流发生异常造成的.     

2008年西北太平洋热带气旋活动异常特征及成因分析

2008年西北太平洋热带气旋活动的特点:(1)初台异常偏早;(2)生成热带气旋异常偏少,但登陆热带气旋异常偏多,登陆热带气旋与生成热带气旋比例高;(3)从热带气旋的生成源地来看,2008年的热带气旋生成位置明显偏西.2008年热带气旋生成年频数异常偏少的主要原因:2008年仍处在生成热带气旋偏少的气候背景下,对流层低层...     

2010年西北太平洋与南海热带气旋活动异常的成因分析

利用中国气象局热带气旋（TC）资料、NCEP/NCAR 再分析资料和美国 NOAA 向外长波辐射（OLR）等资料,分析了2010年西北太平洋（WNP）及南海（SCS）热带气旋活动异常的可能成因,讨论了同期大气环流配置和海温外强迫对TC生成和登陆的动力和热力条件的影响。结果表明,2010年生成TC频数明显偏少,生成源地显著偏西,而登陆TC频数与常年持平。导致7～10月TC频数明显偏少的大尺度环境场特征为：副热带高压较常年异常偏强、西伸脊点偏西,季风槽位置异常偏西,弱垂直风切变带位置也较常年偏西且范围偏小,南亚高压异常偏强,贝加尔湖附近对流层低高层均为反气旋距平环流,这些关键环流因子的特征和配置都不利于 TC 在WNP的东部生成。影响TC活动的外强迫场特征为：2010年热带太平洋经历了El Ni?o事件于春末夏初消亡、La Ni?a事件于7月形成的转换;7～10月,WNP海表温度维持正距平,140°E以东为负距平且对流活动受到抑制;暖池次表层海温异常偏暖,对应上空850 hPa为东风距平,有利于季风槽偏西和TC在WNP的西北侧海域生成。WNP海表温度和暖池次表层海温的特征是2010年TC生成频数偏少、生成源地异常偏西的重要外强迫信号。有利于7～10月热带气旋西行和登陆的500 hPa风场特征为：北太平洋为反气旋环流距平,其南侧为东风异常,该东风异常南缘可到25°N,并向西扩展至中国大陆地区;南海和西北太平洋地区15°N以南的低纬也为东风异常;在这样的风场分布型下,TC容易受偏东气流引导西行并登陆我国沿海地区。这是2010年生成TC偏少但登陆TC并不少的重要环流条件。     

两类厄尔尼诺事件对登陆中国热带气旋的影响

利用上海台风研究所整编的1951—2016年西北太平洋热带气旋最佳路径数据集,NCEP/NCAR再分析资料和NOAA的COBE SST再分析资料,〖JP〗按照热带气旋生成区域将热带气旋分为南海热带气旋与西北太平洋热带气旋两类,采用合成分析等统计学方法探讨了热带气旋活动盛期,登陆中国的热带气旋对东部型和中部型厄尔尼诺（El Niño）事件的响应。结果表明,热带气旋活动盛期,南海热带气旋在两类El Niño事件下生成频数差异不大;东部型El Niño存续期南海热带气旋登陆中国比率较中部型El Niño时偏低,登陆时强度较中部型偏弱。中部型El Niño存续期间,西北太平洋热带气旋生成频数比东部型El Niño时的频数偏高,而登陆中国热带气旋较东部型偏少,登陆时热带气旋强度较东部型偏弱;但两类El Niño事件期间西北太平洋热带气旋在中国的登陆率差异没有通过显著性检验。与中部型El Niño事件相比,在东部型El Niño事件期间,西北太平洋海面温度偏低,对流层中部水汽条件较差,对流层低层涡度异常偏低,同时在热带气旋较为集中生成的海域存在沃克（Walker）环流的异常下沉气流,西太平洋副热带高压偏强偏东偏南,共同导致登陆中国热带气旋频数偏少。     

印度洋海盆增暖及ENSO对西北太平洋热带气旋活动的影响

本文主要分析1950～2010年间印度洋海盆增暖和西北太平洋热带气旋(TC)活动的关系, 并与ENSO对西北太平洋TC活动的影响相比较, 结果表明:印度洋海盆异常增暖与西北太平洋地区总TC生成年频数尤其是弱TC相关较好, 印度洋海盆异常增暖, 西北太平洋地区为异常的反气旋, 对流抑制, 降水偏少, 不利于TC的生成, 反之亦然。而ENSO对西北太平洋热带气旋的影响, 主要体现在对强TC的年生成频数的影响, El Ni?o 发展年, 季风槽加深东伸, TC生成位置偏东, 由于TC在海洋上的生命史较长, TC的平均强度偏强, 因而强TC年生成频数偏多;La Ni?a发展年, 季风槽较浅, TC生成位置偏西, TC的平均强度偏弱, 强TC年生成频数偏少。但是ENSO指数与强TC年频数的相关有着年代际的变化, 在1950～1969年和1990～2009年间, ENSO指数和强TC年频数相关很好, 分别为0.532和0.687, 而在1970～1989这二十年间, 两者相关很弱, 只有0.081。     

西北太平洋热带气旋频数的气候变化及其与环境要素间的联系

使用Emanuel和Nolan完善的潜在生成指数(GPI)的计算方法,利用美国联合台风警报中心提供的热带气旋(TC)资料和欧洲中期数值天气预报中心提供的全球ERA-40再分析资料,比较了1970-2001年西北太平洋海域的TC生成频数和GPI的气候特征,分析了包含于GPI中的环境要素对西北太平洋TC频数年代际变化空间分布的影响.结果表明:GPI能近似地表述西北太平洋TC频数的季节变化和空间分布.各环境要素对TC、较弱类TC和较强类TC生成频数的影响有显著差异,相对湿度随着TC强度的增强而减弱,风速垂直切变则相反.西北太平洋TC频数年代际变化空间分布的正异常主要分布于130°E以东,(15°N,140°E)附近最大的正异常频数中心主要受绝对涡度和相对湿度正异常变化的影响;负的风速垂直切变和正的相对湿度异常变化引起了(10～15°N,160°E)附近的TC频数正异常.     

COMPARATIVE ANALYSIS OF VARIOUS DATA OF AIR–SEA TEMPERATURE DIFFERENCE AND ITS VARIATION ACROSS SOUTH CHINA SEA IN THE PAST 35 YEARS

Using the International Comprehensive Ocean-Atmosphere Data Set(ICOADS) and ERA-Interim data, spatial distributions of air-sea temperature difference(ASTD) in the South China Sea(SCS) for the past 35 years are compared,and variations of spatial and temporal distributions of ASTD in this region are addressed using empirical orthogonal function decomposition and wavelet analysis methods. The results indicate that both ICOADS and ERA-Interim data can reflect actual distribution characteristics of ASTD in the SCS, but values of ASTD from the ERA-Interim data are smaller than those of the ICOADS data in the same region. In addition, the ASTD characteristics from the ERA-Interim data are not obvious inshore. A seesaw-type, north-south distribution of ASTD is dominant in the SCS; i.e., a positive peak in the south is associated with a negative peak in the north in November, and a negative peak in the south is accompanied by a positive peak in the north during April and May. Interannual ASTD variations in summer or autumn are decreasing. There is a seesaw-type distribution of ASTD between Beibu Bay and most of the SCS in summer, and the center of large values is in the Nansha Islands area in autumn. The ASTD in the SCS has a strong quasi-3a oscillation period in all seasons, and a quasi-11 a period in winter and spring. The ASTD is positively correlated with the Nio3.4 index in summer and autumn but negatively correlated in spring and winter.     

CHARACTERISTICS AND TRENDS OF CLIMATIC EXTREMES IN CHINA DURING 1959–2014

The spatial and temporal variations of daily maximum temperature(Tmax), daily minimum temperature(Tmin), daily maximum precipitation(Pmax) and daily maximum wind speed(WSmax) were examined in China using Mann-Kendall test and linear regression method. The results indicated that for China as a whole, Tmax, Tmin and Pmax had significant increasing trends at rates of 0.15℃ per decade, 0.45℃ per decade and 0.58 mm per decade,respectively, while WSmax had decreased significantly at 1.18 m·s~(-1) per decade during 1959—2014. In all regions of China, Tmin increased and WSmax decreased significantly. Spatially, Tmax increased significantly at most of the stations in South China(SC), northwestern North China(NC), northeastern Northeast China(NEC), eastern Northwest China(NWC) and eastern Southwest China(SWC), and the increasing trends were significant in NC, SC, NWC and SWC on the regional average. Tmin increased significantly at most of the stations in China, with notable increase in NEC, northern and southeastern NC and northwestern and eastern NWC. Pmax showed no significant trend at most of the stations in China, and on the regional average it decreased significantly in NC but increased in SC, NWC and the mid-lower Yangtze River valley(YR). WSmax decreased significantly at the vast majority of stations in China, with remarkable decrease in northern NC, northern and central YR, central and southern SC and in parts of central NEC and western NWC. With global climate change and rapidly economic development, China has become more vulnerable to climatic extremes and meteorological disasters, so more strategies of mitigation and/or adaptation of climatic extremes,such as environmentally-friendly and low-cost energy production systems and the enhancement of engineering defense measures are necessary for government and social publics.     

IMPACT OF ATMOSPHERIC LOW-FREQUENCY OSCILLATION ON THE IMMIGRATION OF NILAPARVATA LUGENS(STL) IN HUNAN AND JIANGXI PROVINCES

Various features of the atmospheric environment affect the number of migratory insects, besides their initial population. However, little is known about the impact of atmospheric low-frequency oscillation(10 to 90 days) on insect migration. A case study was conducted to ascertain the influence of low-frequency atmospheric oscillation on the immigration of brown planthopper, Nilaparvata lugens(Stl), in Hunan and Jiangxi provinces. The results showed the following:(1) The number of immigrating N. lugens from April to June of 2007 through 2016 mainly exhibited a periodic oscillation of 10 to 20 days.(2) The 10-20 d low-frequency number of immigrating N. lugens was significantly correlated with a low-frequency wind field and a geopotential height field at 850 h Pa.(3) During the peak phase of immigration, southwest or south winds served as a driving force and carried N. lugens populations northward, and when in the back of the trough and the front of the ridge, the downward airflow created a favorable condition for N. lugens to land in the study area. In conclusion, the northward migration of N. lugens was influenced by a low-frequency atmospheric circulation based on the analysis of dynamics. This study was the first research connecting atmospheric low-frequency oscillation to insect migration.     

A COMPARATIVE ANALYSIS OF ATMOSPHERIC AND OCEANIC CONDITIONS BEFORE THE OCCURRENCE OF TWO TYPES OF EL NIO EVENTS

The atmospheric and oceanic conditions before the onset of EP El Ni?o and CP El Ni?o in nearly 30 years are compared and analyzed by using 850 hPa wind, 20℃ isotherm depth, sea surface temperature and the Wheeler and Hendon index. The results are as follows: In the western equatorial Pacific, the occurrence of the anomalously strong westerly winds of the EP El Ni?o is earlier than that of the CP El Ni?o. Its intensity is far stronger than that of the CP El Ni?o. Two months before the El Ni?o, the anomaly westerly winds of the EP El Ni?o have extended to the eastern Pacific region, while the westerly wind anomaly of the CP El Ni?o can only extend to the west of the dateline three months before the El Ni?o and later stay there. Unlike the EP El Ni?o, the CP El Ni?o is always associated with easterly wind anomaly in the eastern equatorial Pacific before its onset. The thermocline depth anomaly of the EP El Ni?o can significantly move eastward and deepen. In addition, we also find that the evolution of thermocline is ahead of the development of the sea surface temperature for the EP El Ni?o. The strong MJO activity of the EP El Ni?o in the western and central Pacific is earlier than that of the CP El Ni?o. Measured by the standard deviation of the zonal wind square, the intensity of MJO activity of the EP El Ni?o is significantly greater than that of the CP El Ni?o before the onset of El Ni?o.     

Could the Recent Taal Volcano Eruption Trigger an El Ni?o and Lead to Eurasian Warming?

正The Taal Volcano in Luzon is one of the most active and dangerous volcanoes of the Philippines. A recent eruption occurred on 12 January 2020(Fig. 1a), and this volcano is still active with the occurrence of volcanic earthquakes. The eruption has become a deep concern worldwide, not only for its damage on local society, but also for potential hazardous consequences on the Earth's climate and environment.     

VARIABILITY OF INTER-ANNUAL RELATIONSHIP BETWEEN INDIAN OCEAN DIPOLE AND HUAXI REGION’S AUTUMN PRECIPITATION

The moving-window correlation analysis was applied to investigate the relationship between autumn Indian Ocean Dipole (IOD) events and the synchronous autumn precipitation in Huaxi region, based on the daily precipitation, sea surface temperature (SST) and atmospheric circulation data from 1960 to 2012. The correlation curves of IOD and the early modulation of Huaxi region’s autumn precipitation indicated a mutational site appeared in the 1970s. During 1960 to 1979, when the IOD was in positive phase in autumn, the circulations changed from a “W” shape to an ”M” shape at 500 hPa in Asia middle-high latitude region. Cold flux got into the Sichuan province with Northwest flow, the positive anomaly of the water vapor flux transported from Western Pacific to Huaxi region strengthened, caused precipitation increase in east Huaxi region. During 1980 to 1999, when the IOD in autumn was positive phase, the atmospheric circulation presented a “W” shape at 500 hPa, the positive anomaly of the water vapor flux transported from Bay of Bengal to Huaxi region strengthened, caused precipitation ascend in west Huaxi region. In summary, the Indian Ocean changed from cold phase to warm phase since the 1970s, caused the instability of the inter-annual relationship between the IOD and the autumn rainfall in Huaxi region.     

ANALYSIS OF “BIMODAL PATTERN” STORM ACTIVITY CHARACTERISTICS OF THE BAY OF BENGAL

Storms that occur at the Bay of Bengal (BoB) are of a bimodal pattern, which is different from that of the other sea areas. By using the NCEP, SST and JTWC data, the causes of the bimodal pattern storm activity of the BoB are diagnosed and analyzed in this paper. The result shows that the seasonal variation of general atmosphere circulation in East Asia has a regulating and controlling impact on the BoB storm activity, and the “bimodal period” of the storm activity corresponds exactly to the seasonal conversion period of atmospheric circulation. The minor wind speed of shear spring and autumn contributed to the storm, which was a crucial factor for the generation and occurrence of the “bimodal pattern” storm activity in the BoB. The analysis on sea surface temperature (SST) shows that the SSTs of all the year around in the BoB area meet the conditions required for the generation of tropical cyclones (TCs). However, the SSTs in the central area of the bay are higher than that of the surrounding areas in spring and autumn, which facilitates the occurrence of a “two-peak” storm activity pattern. The genesis potential index (GPI) quantifies and reflects the environmental conditions for the generation of the BoB storms. For GPI, the intense low-level vortex disturbance in the troposphere and high-humidity atmosphere are the sufficient conditions for storms, while large maximum wind velocity of the ground vortex radius and small vertical wind shear are the necessary conditions of storms.     

LOW-FREQUENCY CIRCULATION AND EXTENDED-RANGE FORECAST IN CONNECTION WITH AUTUMN EXTREME HEAVY RAINFALL PROCESS IN HAINAN

Observed daily precipitation data from the National Meteorological Observatory in Hainan province and daily data from the National Centers for Environmental Prediction/National Center for Atmospheric Research (NCEP/NCAR) reanalysis-2 dataset from 1981 to 2014 are used to analyze the relationship between Hainan extreme heavy rainfall processes in autumn (referred to as EHRPs) and 10–30 d low-frequency circulation. Based on the key low-frequency signals and the NCEP Climate Forecast System Version 2 (CFSv2) model forecasting products, a dynamical-statistical method is established for the extended-range forecast of EHRPs. The results suggest that EHRPs have a close relationship with the 10–30 d low-frequency oscillation of 850 hPa zonal wind over Hainan Island and to its north, and that they basically occur during the trough phase of the low-frequency oscillation of zonal wind. The latitudinal propagation of the low-frequency wave train in the middle-high latitudes and the meridional propagation of the low-frequency wave train along the coast of East Asia contribute to the ‘north high (cold), south low (warm)’ pattern near Hainan Island, which results in the zonal wind over Hainan Island and to its north reaching its trough, consequently leading to EHRPs. Considering the link between low-frequency circulation and EHRPs, a low-frequency wave train index (LWTI) is defined and adopted to forecast EHRPs by using NCEP CFSv2 forecasting products. EHRPs are predicted to occur during peak phases of LWTI with value larger than 1 for three or more consecutive forecast days. Hindcast experiments for EHRPs in 2015–2016 indicate that EHRPs can be predicted 8–24 d in advance, with an average period of validity of 16.7 d.     

AN ATTRIBUTION ANALYSIS OF CHANGES IN POTENTIAL EVAPOTRANSPIRATION IN THE BEIJING–TIANJIN–HEBEI REGION UNDER CLIMATE CHANGE

Based on the measurements obtained at 64 national meteorological stations in the Beijing–Tianjin–Hebei (BTH) region between 1970 and 2013, the potential evapotranspiration (ET0) in this region was estimated using the Penman–Monteith equation and its sensitivity to maximum temperature (Tmax), minimum temperature (Tmin), wind speed (Vw), net radiation (Rn) and water vapor pressure (Pwv) was analyzed, respectively. The results are shown as follows. (1) The climatic elements in the BTH region underwent significant changes in the study period. Vw and Rn decreased significantly, whereas Tmin, Tmax and Pwv increased considerably. (2) In the BTH region, ET0 also exhibited a significant decreasing trend, and the sensitivity of ET0 to the climatic elements exhibited seasonal characteristics. Of all the climatic elements, ET0 was most sensitive to Pwv in the fall and winter and Rn in the spring and summer. On the annual scale, ET0 was most sensitive to Pwv, followed by Rn, Vw, Tmax and Tmin. In addition, the sensitivity coefficient of ET0 with respect to Pwv had a negative value for all the areas, indicating that increases in Pwv can prevent ET0 from increasing. (3) The sensitivity of ET0 to Tmin and Tmax was significantly lower than its sensitivity to other climatic elements. However, increases in temperature can lead to changes in Pwv and Rn. The temperature should be considered the key intrinsic climatic element that has caused the "evaporation paradox" phenomenon in the BTH region.     

Revisiting the Concentration Observations and Source Apportionment of Atmospheric Ammonia

正While China’s Air Pollution Prevention and Control Action Plan on particulate matter since 2013 has reduced sulfate significantly, aerosol ammonium nitrate remains high in East China. As the high nitrate abundances are strongly linked with ammonia, reducing ammonia emissions is becoming increasingly important to improve the air quality of China. Although satellite data provide evidence of substantial increases in atmospheric ammonia concentrations over major agricultural regions, long-term surface observation of ammonia concentrations are sparse. In addition, there is still no consensus on