非弹性中子散射谱仪

非弹性中子散射是利用中子与材料晶格或自旋散射发生能量和动量交换来测量材料动力学性质的实验技术.非弹性中子散射谱仪可以直接测量声子谱、自旋波、晶体场等性质,且能量和动量分辨率高,在物理、材料、化学、生物等领域有广泛应用,是前沿科学研究中重要的实验仪器.本文概述了非弹性中子散射的发展过程、基本理论、散射谱仪及应用范例.     

探测系统能量分辨在中子能谱数值模拟中的应用

针对中子能谱实验的数值模拟研究中涉及到的探测系统能量分辨问题,基于系统探测伽玛和中子的对应关系以及对伽玛射线的能量分辨率,介绍了一种简便实用的数值模拟方案,利用探测系统对中子、伽玛的光响应对应关系以及其对伽玛的能量分辨率,得到系统对中子的能量分辨率,再进一步把它应用到中子能谱的数值模拟中,并对数值计算结果与相关实验数据进行比较分析。结果表明,该方法可以很好地应用于中子能谱的数值模拟研究。     

基于前冲康普顿电子高能伽马能谱测量系统设计

除中子外,聚变核心同时释放大量高能伽马,其能谱可反映聚变过程的关键物理参数,并为过程诊断提供重要信息.由于聚变伽马的时间与能量特性,需要设计高探测效率及能量分辨率的伽马谱仪.根据高能伽马谱仪的概念设计(gamma-to-electron magnetic spectrometer),针对该系统中伽马-电子转换靶、电子偏转汇聚、电子探测等关键环节进行优化设计以提高系统探测效率及能量分辨率.其中采用Monte-Carlo程序Geant4模拟研究了伽马-电子转换靶中康普顿散射与多次库仑散射对由转换靶出射电子的能谱与角分布的影响.开发并行遗传算法对复杂几何偏转磁场参数进行优化,得到低强度(小于100 Gauss)复杂边界偏转磁场.根据系统优化设计结果,采用Geant4模拟了该系统对不同能量伽马的响应.此外,还可模拟该系统对特征聚变伽马能谱的测量,结果显示,该系统可在聚变中子产额分别为2.5×10~(15)及1.2×10~(16)条件下,对10—20 MeV高能伽马能谱测量实现能量分辨分别满足0.5 MeV(小于5%)及0.25 MeV(小于2.5%),说明该系统可用于聚变过程伽马能谱的诊断.     

质子和1MeV中子在硅中能量沉积的模拟计算

在现有中子截面数据和粒子与物质相互作用的理论基础上,编写了计算中子非电离能量损失(NIEL)和电离能量损失(IEL)程序,利用该程序和引进的TRIM95程序计算了1MeV中子和质子在硅中IEL和NIEL的大小和分布等,并对计算结果进行了分析和比较.     

配有BGO晶体阵列的L3强子量能器性能的模拟测试

本文介绍子配有BGO(锗酸铋)晶体阵列的L3铀强子量能器性能的模拟测试.对L3强子量能器以及测试实验作了简要介绍,并给出了该量能器对4—20GeV能量范围的π介子的能量分辨率、e/π响应比、角分辨、能量分辨率随入射π介子方向的变化以及强子穿透率等实验结果.     

高反射效率高定向性的热解石墨晶体X射线谱仪

基于高定向热解石墨晶体(highly oriented pyrolitic graphite,HOPG)研制了一种新型反射式X射线谱仪.该谱仪具有高反射效率、较高能谱分辨率及相对较宽的能谱测量范围.根据计算,在相同的入射条件下,该谱仪的效率比一般X射线弯晶谱仪高3个量级;谱仪能谱分辨率理论值最高达350;理论探测范围是6.891keV至9.193 keV.我们将该谱仪应用在高功率密度激光与固体靶相互作用的实验中,发现在普通弯晶谱仪无法采到信号的实验条件下,HOPG谱仪依然采集到清晰的Cu K谱线.分析发现在8.048 keV(Cu的Kα光子能量)附近的能谱分辨能力最高达到40 eV,分辨率大于200.     

氢化锆中氢的热中子散射总截面

利用中子晶体谱仪在入射中子能量为0.05—0.54电子伏范围内测量了氢化锆中氢的全截面。并在简谐和非相干近似下,假设声子谱可用两个“类高斯分布”来表示,用声子展开的办法得到了氢化锆中氢的热中子散射双微分截面,再用蒙特-卡洛方法求积分后得到散射总截面。理论计算结果和实验结果在误差范围内基本符合。     

数值模拟高能中子照相

 模拟了14 MeV中子在穿透样品后与闪烁体光纤的作用。对每根光纤中的能量沉积进行了计算，并转换成可见光(496 nm)光子数。在模拟实验中，分析了影响图像质量的因素。计算了散射中子本底与闪烁体和样品(聚乙烯)间距的关系。当间距为cm量级时，散射中子本底对图像的影响很小。计算表明系统对样品的甄别厚度与入射中子总数有关，在一定范围内近似与中子总数的对数成线性关系。通过模拟结果给出了理想平行中子束入射情况下系统的平面分辨率。     

中子与9Be和6,7Li反应的次级中子发射谱实验研究

测量了8.17MeV与10.27MeV中子与⁹Be和^6,7Li作用的次级中子双微分截面. 对于10.27MeV, 为了消除从D(d,np)破裂反应来的源破裂中子对双微分截面测量结果的影响, 采用了常规多探测器快中子飞行时间谱仪和非常规多探测器快中子飞行时间谱仪相结合的办法. 用Monte-Carlo方法对实验测量得到的飞行时间谱进行了详细的模拟, 通过测量谱与模拟谱的比较, 得到了实验测量的次级中子双微分截面. 实验测量结果以n-p(常规谱仪)和n-C(非常规谱仪)弹性散射微分截面作为归一. 测量结果与评价数据以及其他测量数据进行了比较. 用一个基于Hauser-Feshbach和激子模型的轻核核反应理论模型对^6,7Li的次级中子双微分截面进行了计算, 理论计算结果与实验结果符合得较好.     

4He闪烁裂变中子探测器的中子灵敏度

对4He闪烁裂变中子探测器的中子灵敏度进行了理论和实验研究。采用蒙特卡罗方法模拟了不同能量中子和不同厚度裂变靶产生的裂变碎片在4He中的能量沉积,计算结果表明:中子在4He气中的能量沉积曲线和裂变碎片的能量沉积曲线能够互补,从而使探测器对中子的能量响应变得更平坦;探测器的中子灵敏度为10-15 Ccm2量级。并对探测器的中子灵敏度进行了实验标定,实验结果与理论计算结果较为一致。     

Localized excitation in the hybridization gap in YbAl3

The intermediate valence compound YbAl3 exhibits a broad magnetic excitation in the inelastic neutron scattering spectrum with characteristic energy E1 approximately 50 meV, equal to the Kondo energy (T(K) approximately 600-700 K). In the low temperature (T < T(coh) approximately 40 K) Fermi liquid state, however, a new peak in the scattering occurs at E2 approximately 33 meV, which lies in the hybridization gap that exists in this compound. We report inelastic neutron scattering results for a single-crystal sample. The scattering at energies near E1 qualitatively has the momentum (Q) dependence expected for interband scattering across the indirect gap. The scattering near E2 has a very different Q dependence: it is a weak function of Q over a large fraction of the Brillouin zone and is smallest near (1/2,1/2, 1/2). A possibility is that the peak at E2 arises from a spatially localized excitation in the hybridization gap.     

YBa2Cu3O6+δ的高频模及其随氧含量δ的变化

在中国原子能科学研究院新建的宽角(～30°)Be过滤探测器中子非弹性散射谱仪上,在入射中子能量从10直至150meV的范围内,测量了几种不同氧含量的YBa₂Cu₃O_6+δ样品的中子非弹性散射能谱。结果表明:(1)在δ=0和0.2时,在60至150meV能量范围内,发现有强的高频模存在,当其温度高到Nel点(～410K)以上直至466K时,没有观察出高频模强度的减弱。而δ=0.78和0.97时,在75至150meV能量范围内,散射强度在测量误 关键词：     

Phonon density of states of single-wall carbon nanotubes

The vibrational density of states of single-wall carbon nanotubes (SWNT) was obtained from inelastic neutron scattering data from 0 to 225 meV. The spectrum is similar to that of graphite above 40 meV, while intratube features are clearly observed at 22 and 36 meV. An unusual energy dependence below 10 meV is assigned to contributions from intertube modes in the 2D triangular lattice of SWNT bundles, and from intertube coupling to intratube excitations. Good agreement between experiment and a calculated density of states for the SWNT lattice is found over the entire energy range.     

Spin correlations among the charge carriers in an ordered stripe phase

We have observed a diffuse component to the low-energy magnetic excitation spectrum of stripe-ordered La(5/3)Sr(1/3)NiO4 probed by neutron inelastic scattering. The diffuse scattering forms a square pattern with sides parallel and perpendicular to the stripe directions. The signal is dispersive, with a maximum energy of approximately 10 meV. Probed at 2 meV, the scattering decreases in strength with increasing temperature, and is barely visible at 100 K. We argue that the signal originates from dynamic, quasi-one-dimensional, antiferromagnetic correlations among the stripe electrons.     

Direct evidence for the localized single-triplet excitations and the dispersive multitriplet excitations in SrCu2(BO3)2

We performed inelastic neutron scattering on the 2D Shastry-Sutherland system SrCu2(11BO3)2 with an exact dimer ground state. Three energy levels at around 3, 5, and 9 meV were observed at 1.7 K. The lowest excitation at 3.0 meV is almost dispersionless with a bandwidth of 0.2 meV at most, showing a significant constraint on a single-triplet hopping owing to the orthogonality of the neighboring dimers. In contrast, the correlated two-triplet excitations at 5 meV exhibit a more dispersive behavior.     

Inelastic neutron scattering in Zr<Subscript>2</Subscript>NiH<Subscript>1.9</Subscript> and Zr<Subscript>2</Subscript>NiH<Subscript>4.6</Subscript>

In this paper we report the results obtained from inelastic neutron scattering measurements on Zr₂NiH_1.9 and Zr₂NiH_4.6 using triple-axis spectrometer at Dhruva reactor, Trombay. The spectrum up to 35 meV represents largely the lattice modes of Zr and Ni atoms. The vibrational frequencies of hydrogen atoms are expected predominantly at higher energies. The phonon spectra from 35–180 meV were recorded using a Be filter as analyser. In order to analyse the observed neutron spectra, we assume a set of Ein-stein modes due to the hydrogen atoms which are delta functions in energy. These delta functions are broadened by the resolution of the instrument. The vibrational frequencies obtained from the fitting of the observed phonon spectra have been assigned to various tetrahedral sites in both the compounds.     

First measurement of a phonon dispersion curve by inelastic X-ray scattering

Inelastic scattering of 13.8 keV X-rays with very high energy resolution of E=55 meV was used to measure the phonon dispersion curves for theLA andLO modes in the [00] direction in Be. The results agree with inelastic neutron scattering data known from the literature. The X-ray scattering intensities of the phonon excitations for different momentum transfers are in very good agreement with the prediction from the scattering law.     

Neutron scattering study of NiHx at 77K

The results of simultaneous measurements of inelastic incoherent neutron scattering (IINS) and neutron diffraction on NiH_x system with x = 0.40, 0.28 and 0.12 at temperatures of 77 K are briefly presented. In the phonon density of states, supposing a one-phonon mechanism for the scattering process, the optic modes appear as a broad band from 70 to 140 meV with a strong peak at 90 meV and weak peaks at 105 and 130 meV. Neutron diffraction confirms information about the phase composition of the samples investigated.     

Inelastic neutron scattering study of the dynamics of the AlNiCo decagonal phase

The dynamics of the decagonal AlNiCo phase has been investigated on a single-grain quasicrystalline sample using inelastic neutron scattering. The decagonal structure can be viewed as a periodic stacking of quasiperiodic planes. The anisotropy between the modes propagating in the periodic and quasiperiodic directions is found to be much weaker than theoretically predicted. A strong resonance splitting is observed at an energy transfer of 15 meV for transverse modes polarized in the quasiperiodic plane. Received: 18 November 1998 / Accepted: 27 November 1998