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CQDs@MIL-125复合光催化剂的制备及其光生载流子传输特性
引用本文:张富青,汪花丽,何漩,赵雷,李薇馨.CQDs@MIL-125复合光催化剂的制备及其光生载流子传输特性[J].功能材料,2019,50(1):1203-1209.
作者姓名:张富青  汪花丽  何漩  赵雷  李薇馨
作者单位:武汉科技大学 省部共建耐火材料与冶金国家重点实验室,武汉 430081;武汉工程大学 化学与环境工程学院,武汉 430205;武汉科技大学 省部共建耐火材料与冶金国家重点实验室,武汉,430081
基金项目:湖北省教育厅科学技术研究项目;新型反应器与绿色化学工艺湖北省重点实验、绿色化工过程教育部重点实验室资助项目
摘    要:将碳量子点(CQDs)引入钛基金属有机框架材料MIL-125中,旨在将MOFs的高比表面积、多催化位点的优势与CQDs优异的光学特性有机结合,发生协同效应,以期有效提高催化剂的光吸收效率和催化效率。对复合光催化剂的形貌与结构及光电性能进行了测试表征,系统研究了其在可见光催化降解有机染料的催化性能,探索了CQDs的引入方式对复合催化剂结构与性能的影响。

关 键 词:碳量子点  钛基MOFs  光催化  协同效应

The preparation of CQDs@MIL-125 and its optical carrier transmission characteristics
ZHANG Fuqing,WANG Huali,HE Xuan,ZHAO Lei,LI Weixin.The preparation of CQDs@MIL-125 and its optical carrier transmission characteristics[J].Journal of Functional Materials,2019,50(1):1203-1209.
Authors:ZHANG Fuqing  WANG Huali  HE Xuan  ZHAO Lei  LI Weixin
Affiliation:(The State Key Laboratory of Refractories and Metallurgy, Wuhan University of Science & Technology, Wuhan 430081, China;College of Chemical Engineering and Technology, Wuhan Institute of Technology, Wuhan 430205, China)
Abstract:In this paper, in order to effectively improve the efficiency of the light absorption of catalysts and catalytic efficiency, carbon quantum dots (CQDs) were introduced into titanium-based metal organic framework material MIL-125, aiming to organically combine the advantages of high specific surface area and more catalytic sites of MOFs with the excellent optical properties of CQDs, and achieve synergistic effect. The morphology, structure and photoelectric properties of the composite photocatalyst were characterized. Its catalytic properties in the visible light catalytic degradation of organic dyes were systematically studied and the way of the introduction of CQDs effects on structure and performance of composite catalyst was explored.
Keywords:carbon quantum dots (CQDs)  Ti-based MOFs  photocataly  synergistic effect
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