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Strategies for Improving the Catalytic Performance of 2D Covalent Organic Frameworks for Hydrogen Evolution and Oxygen Evolution Reactions
Authors:Dr Yang Deng  Yue Wang  Dr Yibo Chen  Dr Zhen Zhang
Affiliation:1. Tianjin Key Laboratory of Molecular Optoelectronic Department of Chemistry, School of Science, Tianjin University, Tianjin, 300072 P. R. China

These authors contributed equally.;2. School of Chemistry and Chemical Engineering/ Guangzhou Key Laboratory for Clean Energy and Materials, Guangzhou University, Guangzhou, 510006 P. R. China;3. Tianjin Key Laboratory of Molecular Optoelectronic Department of Chemistry, School of Science, Tianjin University, Tianjin, 300072 P. R. China

Abstract:Hydrogen evolution reaction (HER) and oxygen evolution reaction (OER) have been deemed as clean and sustainable strategies to solve the energy crisis and environmental problems. Various catalysts have been developed to promote the process of HER and OER. Among them, two-dimensional covalent organic frameworks (2D COFs) have received great attention due to their diverse and designable structure. In this minireview, we mainly summarize the diverse linkages of 2D COFs and strategies for enhancing the catalytic performance of 2D COFs for HER and OER, such as introducing active building blocks, metal ions and tailored linkages. Furthermore, a brief outlook for the development directions of COFs in the field of HER and OER is provided, expecting to stimulate new opportunities in future research.
Keywords:Covalent organic frameworks  Diverse linkages  catalysis  Hydrogen evolution reactionkeyword  Oxygen evolution reaction
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