HNO3和有机介质中U（Ⅳ）的稳定性研究

研究了ＨＮＯ＿３和ＴＢＰ－煤油介质中Ｕ（Ⅳ）的稳定性。测定了两种介质中Ｕ（Ⅳ）、ＨＮＯ＿３、ＴＢＰ浓度和气相中氧浓度对Ｕ（Ⅳ）氧化速率的影响。Ｕ（Ⅳ）的氧化速率都随温度提高而明显增加．其表观活化能分别为９１ｋＪ／ｍｏｌ（ＨＮＯ＿３介质）和４２ｋＪ／ｍｏｌ（ＴＢＰ－煤油介质）。对两种介质中Ｕ（Ⅳ）的氧化速率规律进行了比较。     

钍归-化在盆地γ能谱资料处理中的应用

在应用γ能谱资料寻找砂岩型铀矿的过程中，要尽可能地消除非矿化因素引起的干扰，提取与铀矿化有关的信息。介绍了钍归-化的原理及特点，采用与矿化有关的元素迁移信息的钍归-化方法，分析了二连盆地东部的γ能谱资料，揭示了该区放射性元素的分布特征、地球化学作用和后期铀元素的迁移与富集。结合其他地质资料，分析了钾剩差的变异区（正、负高值区）及铀剩差正高值区形成的原因，同时指出了经过钍归-化处理所得到的铀剩差正高值区应为氧化与还原作用过渡带的直接指示，也是该区进一步寻找砂岩型铀矿的重要标志。     

一种简便的饮用水除铀方法及其机理

本文介绍一种利用原水中含有的无机盐,加入廉价的化学试剂除去饮用水中微量铀的简便方法。并对其除铀机理进行了探讨,证明除铀主要是以软化水过程中产生的氢氧化镁表面吸附共沉淀机理进行的。     

Effect of Water Vapor on the Release of Fission Gases from Uranium Oxycarbide in High-Temperature, Gas-Cooled Reactor Coated Fuel Particles

The hydrolysis of uranium oxycarbide (UCO) was studied by injecting water vapor into a fuel element containing a known number of high-temperature, gas-cooled reactor (HTGR) coated particles with exposed fuel kernels. The experiments were conducted in the High Flux Isotope Reactor (HFIR) at temperatures between 700° and 1000°C, a system pressure of 200 kPa, and partial pressures of water vapor between 21 and 199 Pa. The general sequential response of the exposed fuel kernels to water vapor addition consisted of (1) a rapid release of stored fission gas with a concomitant increase in the steady-state release and (2) a period of constant steady-state release. Upon cessation of the addition of water vapor, a decline in the release to prehydrolysis values generally occurred. The release of stored fission gas was dependent on the square of the partial pressure of water vapor. The ratio of the constant steady-state release to the prehydrolysis value was independent of the partial pressure of water vapor. The time constant for the decline in the release was the same in all of the hydrolysis tests.     

低浓度含铀废水处理技术的研究进展

各种人为因素使得环境中的铀及其化合物越来越多,对水体造成了放射性污染。在分析环境中低浓度铀来源的基础上,介绍了对低浓度铀污染水体进行处理的最新技术,并着重探讨了应用植物修复技术处理铀污染的研究现状与发展趋势。     

偕胺肟基功能高分子膜吸附铀量的测定

以偶氮氯膦Ⅲ(CPAⅢ)作为显色剂,研究可见光分光光度计测定含偕胺肟基功能高分子膜螯合电极对铀酰离子的吸附量的实验方法。确定了分光光度法测定的铀酰离子吸附量的实验条件:吸收光波长670 nm,CPAⅢ标准溶液(0.001 mol.L-1)的用量3mL,测定体系的最佳pH值1.0,室温下显色时间2 min。在此实验条件下,绘制了铀的工作曲线,并得到摩尔吸光系数为ε=29 750 mol-1.L.cm-1。对比电子能谱法所测定的脱附铀前后的螯合电极表面的铀含量(脱附前后亮区铀含量分别为38.12%和6.29%,暗区铀含量都为零),得到分光光度计法测定的铀含量并不是螯合电板表面的真实铀含量,但却是脱附下来的铀的真实量,这肯定了分光光度法测定铀的吸附量优势所在。     

双热中子束流治疗孔道低浓化BNCT堆初步设计

以我国已经建成的高浓铀为燃料的BNCT堆为研究对象,将其堆芯低浓化并且添加水平热中子双束流治疗孔道,开展双热中子束流BNCT堆堆芯低浓化初步设计,计算分析该BNCT堆的keff、控制棒价值、顶铍效率、堆芯能谱、堆芯径向通量、轴向通量、辐照管通量等参数,得到双热中子束流治疗孔道低浓化BNCT堆初步设计方案.     

Water as a Promoter of the Complete Oxidation of Volatile Organic Compounds over Uranium Oxide Catalysts

The effect of water addition on the complete oxidation of benzene and propane VOCs by uranium oxide catalysts has been investigated. Benzene oxidation was studied using a silica supported U₃O₈ catalyst. Complete oxidation is promoted by the addition of 2.6% water compared with the reactivity when no water is added to the reactant feed. Increasing the water concentration to 12.1% resulted in a suppression of oxidation activity. Investigation of propane oxidation using U₃O₈ shows a dramatic promotion of activity. Propane conversion was ca. 50% at 600 °C without added water, whilst it increased to 100% at 400 °C with the addition of 2.6% water. A comparison of oxidation activity has been made with Mn₂O₃, an oxide recognised for complete oxidation. In contrast to the U₃O₈ catalysts the addition of 2.6% water suppresses the activity of Mn₂O₃. In situ powder X-ray diffraction studies showed that the bulk U₃O₈ structure was stable under all the reaction conditions. The origin of the increased activity is not clear but may be due to modification of the catalyst surface and the contribution from new reaction pathways such as steam reforming.     

RADIOIMMUNOTOXICOLOGICAL EFFECT OF ENRICHED URANIUM ON CENTRAL AND PERIPHERAL IMMUNE CELLS AND THE PROTECTIVE ACTION OF IL－1 AND IL－2

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