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Jaye E. Cable Jonathan B. Martin Peter W. Swarzenski Mary K. Lindenberg Joel Steward 《Ground water》2004,42(7):1011-1020
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Seasonal records of climatic change in annually laminated tufas: short review and future prospects 总被引:3,自引:0,他引:3
Many Recent and fossil freshwater tufa stromatolites contain millimetre‐scale, alternating laminae of dense micrite and more porous or sparry crystalline calcites. These alternating laminae have been interpreted to represent seasonally controlled differences in the biotic activity of microbes, and/or seasonally controlled changes in the rate of calcification. Either way, couplets of these microbially mediated alternating calcified laminae are generally agreed to represent annual seasonality. Combined stable isotope (δ18O and δ13C) and trace element (Mg, Sr, Ba) geochemistry from Recent tufa stromatolites show that seasonal climatic information is available from these calcites. Variability in δ18O (and in one case Mg concentration) has been shown to be controlled primarily by stream temperature change, usually driven by solar insolation. In arid climates, seasonal evaporation can also cause δ18O enrichment by at least 1‰. Variability in δ13C results potentially from: (1) seasonal change in plant uptake of 12C‐enriched CO2; (2) seasonal change in degassing of 12C‐enriched CO2 in the aquifer system; and (3) precipitation of calcite along the aquifer or river flow path, a process that increases δ13C of dissolved inorganic carbon (DIC) in the remaining water. Mechanisms 2 and 3 are linked because calcite precipitates in aquifers where degassing occurs, e.g. air pockets. The latter mechanism for δ13C enrichment has also been shown to cause sympathetic variation between trace element/Ca ratios and δ13C because trace elements with partition coefficients much greater than 1 (e.g. Sr, Ba) remain preferentially in solution. Since degassing in air pockets will be enhanced during decreased recharge when water saturation of the aquifer is lowest, sympathetic variation in trace element/Ca ratios and δ13C is a possible index of recharge and therefore precipitation intensity. High‐resolution geochemical data from well‐dated tufa stromatolites have great potential for Quaternary palaeoclimate reconstructions, possibly allowing recovery of annual seasonal climatic information including water temperature variation and change in rainfall intensity. However, careful consideration of diagenetic effects, particularly aggrading neomorphism, needs to be the next step. Copyright © 2005 John Wiley & Sons, Ltd. 相似文献
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Tiffany A. Wilson Aria Amirbahman Stephen A. Norton Mary A. Voytek 《Journal of Paleolimnology》2010,44(1):279-294
Historical phosphorus (P) dynamics were studied using sediment cores from three oligotrophic, acidic lakes in Maine, USA.
Long-term oligotrophy of these lakes is consistent with high sediment aluminum (as Al(OH)3) concentrations, as Al inhibits internal P loading, even under reducing conditions. The role of microbially-mediated reactions
in controlling redox conditions was evaluated by estimating microbial biomass and relative abundance of specific functional
groups. Sediments were fractionated using a sequential chemical extraction technique and all lakes met criteria for P retention
based on threshold sediment concentrations of Al, Fe, and P fractions as determined by (Kopáček et al. (2005) Limnol Oceanogr 52: 1147–1155). Sediment NaOH-extractable molybdate-reactive P (rP) and non-reactive P (nrP) represent P
associated with non-reducible phases, and organic matter-related P, respectively. Total P (TP) does not decrease with sediment
depth, as is typical of eutrophic lake sediments; however, nrP/TP decreases and rP/TP increases for all three lakes, indicating
nrP mineralization without any significant upward diffusion and release into the hypolimnion; i.e. diagenesis of P is conservative
within the sediment. Two diagenetic models were developed based on nrP and rP concentrations as a function of sediment age.
The first model assumes a first-order decay of nrP, the rate coefficient being a function of time, and represents irreversible
nrP mineralization, where the produced PO4 is permanently sequestered by the sediment. The second model assumes a first-order reversible transformation between nrP
and rP, representing biotic mineralization of organic P followed by incorporation of inorganic P into microbial biomass. Both
models reflect preservation of TP with no loss to overlying water. The rate coefficients give us insight into qualities of
the sediment that have affected mineralization and sequestration of phosphorus throughout the 210Pb-dateable history of each lake. Similar models could be constructed for other lakes to help reconstruct their trophic histories.
Paleolimnological reconstruction of the sediment P record in oligotrophic lakes shows mineralization of nrP to rP, but unlike
the case in eutrophic lake sediments, sediment TP is preserved in these sediments. 相似文献
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There are few studies on the hydrogeology of sedimentary rock aquitards although they are important controls in regional ground water flow systems. We formulate and test a three-dimensional (3D) conceptual model of ground water flow and hydrochemistry in a fractured sedimentary rock aquitard to show that flow dynamics within the aquitard are more complex than previously believed. Similar conceptual models, based on regional observations and recently emerging principles of mechanical stratigraphy in heterogeneous sedimentary rocks, have previously been applied only to aquifers, but we show that they are potentially applicable to aquitards. The major elements of this conceptual model, which is based on detailed information from two sites in the Maquoketa Formation in southeastern Wisconsin, include orders of magnitude contrast between hydraulic diffusivity (K/S(s)) of fractured zones and relatively intact aquitard rock matrix, laterally extensive bedding-plane fracture zones extending over distances of over 10 km, very low vertical hydraulic conductivity of thick shale-rich intervals of the aquitard, and a vertical hydraulic head profile controlled by a lateral boundary at the aquitard subcrop, where numerous surface water bodies dominate the shallow aquifer system. Results from a 3D numerical flow model based on this conceptual model are consistent with field observations, which did not fit the typical conceptual model of strictly vertical flow through an aquitard. The 3D flow through an aquitard has implications for predicting ground water flow and for planning and protecting water supplies. 相似文献
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<Emphasis Type="Italic">M</Emphasis><Subscript>W</Subscript>9 Tohoku earthquake in 2011 in Japan: precursors uncovered by natural time analysis 下载免费PDF全文
Panayiotis A. Varotsos Nicholas V. Sarlis Efthimios S. Skordas Mary S. Lazaridou-Varotsos 《地震科学(英文版)》2017,30(4):183-191
This paper reviews the precursory phenomena of the 2011 M W9 Tohoku earthquake in Japan that emerge solely when we analyze the seismicity data in a new time domain termed natural time. If we do not consider this analysis, important precursory changes cannot be identified and hence are missed. Natural time analysis has the privilege that enables the introduction of an order parameter of seismicity. In this frame, we find that the fluctuations of this parameter exhibit an unprecedented characteristic change, i.e., an evident minimum, approximately two months before Tohoku earthquake, which strikingly is almost simultaneous with unique anomalous geomagnetic field variations recorded mainly on the z component. This is consistent with our finding that such a characteristic change in seismicity appears when a seismic electric signal (SES) activity of the VAN method (from the initials of Varotsos, Alexopoulos, Nomicos) initiates, and provides a direct confirmation of the physical interconnection between SES and seismicity. 相似文献
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R.M. Brown H.R. Andrews G.C. Ball N. Burn Y. Imahori J.C.D. Milton E.L. Fireman 《Earth and Planetary Science Letters》1984,67(1):1-8
14C has been measured in three North American and seven Antarctic meteorites with the Chalk River MP tandem accelerator. In most cases cosmogenic14C, which is tightly bound, was separated from absorbed atmospheric radiocarbon by stepwise heating extractions. Terrestrial ages obtained by comparing cosmogenic14C in the meteorite to that in Bruderheim are (7.2 ± 0.6) × 103 years for Yamato 7304, (11.6 ± 0.4) × 103 years for Estacado, and range from (32.7 ± 0.5) × 103 to (41.0 ± 0.8) × 103 years for six meteorites recovered at Allan Hills and its vicinity. The present upper limit to age determination by the accelerator method varies from 50 × 103 to 70 × 103 years depending upon mass and carbon content of the sample. The natural limit caused by cosmic ray production of14C in silicate rocks at 2000 m elevation is estimated to be (55 ± 5) × 103 years. “Weathering ages” were estimated for the Antarctic meteorites from the specific activity of loosely-bound CO2 considered to be absorbed from the terrestrial atmosphere on weathering. The accelerator measurements are in accordance with previous low-level counting measurements but have higher precision and sensitivity. 相似文献
10.
Luis Andrés Guillén Mary Beth Adams Emily Elliot Jason Hubbart Charlene Kelly Brenden McNeil William Peterjohn Nicolas Zegre 《水文研究》2021,35(4):e14106
Long-term experimental watershed studies have significantly influenced our global understanding of hydrological processes. The discovery and characterization of how stream water quantity and quality respond to a changing environment (e.g. land-use change, acidic deposition) has only been possible due to the establishment of catchments devoted to long-term study. One such catchment is the Fernow Experimental Forest (FEF) located in the headwaters of the Appalachian Mountains in West Virginia, a region that provides essential freshwater ecosystem services to eastern and mid-western United States communities. Established in 1934, the FEF is among the earliest experimental watershed studies in the Eastern United States that continues to address emergent challenges to forest ecosystems, including climate change and other threats to forest health. This data note describes available data and presents some findings from more than 50 years of hydrologic research at the FEF. During the first few decades, research at the FEF focused on the relationship between forest management and hydrological processes—especially those related to the overall water balance. Later, research included the examination of interactions between hydrology and soil erosion, biogeochemistry, N-saturation, and acid deposition. Hydro-climatologic and water quality datasets from long-term measurements and data from short-duration studies are publicly available to provide new insights and foster collaborations that will continue to advance our understanding of hydrology in forested headwater catchments. As a result of its rich history of research and abundance of long-term data, the FEF is positioned to continue to advance understanding of forest ecosystems in a time of unprecedented change. 相似文献