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高分辨(e,2e)谱仪采用二维位置灵敏探测器同时对能量和角度进行多道测量.二维位置灵敏探测器由级联使用的微通道板和电阻阳极板组成,由于电阻阳极板的边缘效应和制造工艺的缺陷,测量得到的位置图像与实际图像总会有一定的形变,存在一定的非线性.本文针对高分辨(e,2e)谱仪二维位置灵敏探测器输出图像的“桶形”畸变及位置非线性,采用一种简易的冷刻法(用脉冲信号来模拟真实电子束团),检验了二维位置灵敏探测器的Gear型电阻阳极板的线性好坏,并用分割成小三角形的方法找出测量得到的畸变图像与原始真实图像的映射关系,再用此关系对其它测量得到的畸变图像进行修正,并对修正的结果进行了评估.通过修正,由“桶形”畸变所造成的图像扭曲得到明显改善.修正后的x方向非线性由修正前的2.1%变为0.59%.这种检验和修正方法对其它领域类似探测器输出图像的修正也有一定的指导意义. 相似文献
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用包含极化效应和后碰撞作用的扭曲波玻恩近似计算了共面不对称几何条件下Ar(3s^2)的低能(e,2e)三重微分截面,并与实验进行了比较。指出极化效应在共面不对称几何条件下Ar(3s^2)的低能(e,2e)过程中起着重要的作用。 相似文献
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This paper calculates the five most stable conformers of serine with Hartree--Fock theory, density functional theory (B3LYP), Moller--Plesset perturbation theory (MP4(SDQ)) and electron propagation theory with the 6-311++G(2d,2p) basis set. The calculated vertical ionization energies for the valence molecular orbitals of each conformer are in agreement with the experimental data, indicating that a range of molecular conformations would coexist in an equilibrium sample. Information of the five outer valence molecular orbitals for each conformer is explored in coordinate and momentum spaces using dual space analysis to investigate the conformational processes, which are generated from the global minimum conformer Ser1 by rotation of C2--C3 (Ser4), C1--C2 (Ser5) and C1--O2 (Ser2 and Ser3). Orbitals 28a, 27a and 26a are identified as the fingerprint orbitals for all the conformational processes. 相似文献
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由于低动量区域理论和实验的严重差异,重新分析了系列氟利昂分子CF3Cl、CF2Cl2和CFCl3 (CFxCl4-x, x=1~3)的4a1轨道的电子动量分布. 利用分子离子的平衡几何构型计算得到的动量分布很大地改善了,与实验数据之间的吻合,这一结果表明在p<0.5 a.u.区域实验观测到的偏高的动量分布值可能是电离瞬间分子构型的扭曲带来的. 进一步的分 相似文献
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The relativistic and distorted wave effects are investigated for the electron momentum distributions of Xe 4d electrons.The theoretical results show good agreements with the experimental data measured previously with electron momentum spectroscopy. The distorted wave effect and the relativistic effect are found to play important roles in the low and high momentum regions, respectively. 相似文献
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本文用自旋平均静态交换势三体扭曲波波恩近似(DWBA)计算了Li+(1s2)和He(1s2)、K+(3p6) 和Ar(3p6)在1?000?eV入射能下的共面不对称(e, 2e)三重微分截面(TDCS).通过比较离子和原子靶三重微分截面的角分布,表明两体碰撞图像在离子靶的情形不成立. 相似文献
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The dissociative ionization of CO2 induced by 5 keV electrons in two-body and three-body dissociative channels of CO2+2 and CO3+2 is identified by the ion-ion coincidence- method using a momentum imaging spectrometer. The partial ionization cross sections (PICSs) of different ionic fragments are measured and the results generally agree with the calculations made by a semi-empirical approach. Furthermore, the PICSs of the dissociative channels are also obtained by carefully considering the detection efficiency of the micro-channel plates and the total transmission efficiency of the time of flight system. 相似文献