全文获取类型
收费全文 | 433篇 |
免费 | 10篇 |
国内免费 | 8篇 |
学科分类
环境安全 | 451篇 |
出版年
2023年 | 5篇 |
2022年 | 14篇 |
2021年 | 15篇 |
2020年 | 7篇 |
2019年 | 9篇 |
2018年 | 15篇 |
2017年 | 8篇 |
2016年 | 13篇 |
2015年 | 11篇 |
2014年 | 24篇 |
2013年 | 46篇 |
2012年 | 20篇 |
2011年 | 27篇 |
2010年 | 10篇 |
2009年 | 20篇 |
2008年 | 29篇 |
2007年 | 15篇 |
2006年 | 19篇 |
2005年 | 18篇 |
2004年 | 17篇 |
2003年 | 20篇 |
2002年 | 10篇 |
2001年 | 4篇 |
2000年 | 8篇 |
1999年 | 3篇 |
1998年 | 3篇 |
1997年 | 2篇 |
1996年 | 3篇 |
1995年 | 4篇 |
1994年 | 4篇 |
1991年 | 3篇 |
1989年 | 5篇 |
1987年 | 2篇 |
1986年 | 3篇 |
1985年 | 3篇 |
1984年 | 4篇 |
1983年 | 2篇 |
1982年 | 5篇 |
1981年 | 4篇 |
1980年 | 3篇 |
1979年 | 1篇 |
1978年 | 1篇 |
1974年 | 1篇 |
1971年 | 1篇 |
1968年 | 1篇 |
1967年 | 1篇 |
1966年 | 1篇 |
1964年 | 1篇 |
1962年 | 1篇 |
1954年 | 1篇 |
排序方式: 共有451条查询结果,搜索用时 15 毫秒
1.
2.
Air quality field data, collected as part of the fine particulate matter Supersites Program and other field measurements programs, have been used to assess the degree of intraurban variability for various physical and chemical properties of ambient fine particulate matter. Spatial patterns vary from nearly homogeneous to quite heterogeneous, depending on the city, parameter of interest, and the approach or method used to define spatial variability. Secondary formation, which is often regional in nature, drives fine particulate matter mass and the relevant chemical components toward high intraurban spatial homogeneity. Those particulate matter components that are dominated by primary emissions within the urban area, such as black carbon and several trace elements, tend to exhibit greater spatial heterogeneity. A variety of study designs and data analysis approaches have been used to characterize intraurban variability. High temporal correlation does not imply spatial homogeneity. For example, there can be high temporal correlation but with spatial heterogeneity manifested as smooth spatial gradients, often emanating from areas of high emissions such as the urban core or industrial zones. 相似文献
3.
Yanni Ma Jay D. Hmielowski 《Environmental Communication: A Journal of Nature and Culture》2019,13(1):71-86
Scholars continue to search for solutions to shift climate change skeptics’ views on climate science and policy. However, research has shown that certain audiences are resistant to change regarding environmental issues. To explore this issue further, we examine the presence of reactance among different audiences in response to simple, yet prominently used, climate change messages. Our results show that emphasizing the scientific consensus of climate change produces reactance, but only among people who question the existence of climate change. Moreover, adding political identification to the model as an additional moderating variable shows the increases in reactance occur among Republicans who question the existence of climate change. Finally, our results show that reactance to climate change messaging may lead to backfiring effects on important outcomes tied to climate change such as risk perceptions, climate change beliefs, and support for mitigation policies. 相似文献
4.
Zhi-Ping Wang Yang Song Jay Gulledge Qiang Yu Hong-Sheng Liu Xing-Guo Han 《Atmospheric environment (Oxford, England : 1994)》2009,43(13):2148-2153
A budget for the methane (CH4) cycle in the Xilin River basin of Inner Mongolia is presented. The annual CH4 budget in this region depends primarily on the sum of atmospheric CH4 uptake by upland soils, emission from small wetlands, and emission from grazing ruminants (sheep, goats, and cattle). Flux rates for these processes were averaged over multiple years with differing summer rainfall. Although uplands constitute the vast majority of land area, they consume much less CH4 per unit area than is emitted by wetlands and ruminants. Atmospheric CH4 uptake by upland soils was ?3.3 and ?4.8 kg CH4 ha?1 y?1 in grazed and ungrazed areas, respectively. Average CH4 emission was 791.0 kg CH4 ha?1 y?1 from wetlands and 8.6 kg CH4 ha?1 y?1 from ruminants. The basin area-weighted average of all three processes was 6.8 kg CH4 ha?1 y?1, indicating that ruminant production has converted this basin to a net source of atmospheric CH4. The total CH4 emission from the Xilin River basin was 7.29 Gg CH4 y?1. The current grazing intensity is about eightfold higher than that which would result in a net zero CH4 flux. Since grazing intensity has increased throughout western China, it is likely that ruminant production has converted China's grazed temperate grasslands to a net source of atmospheric CH4 overall. 相似文献
5.
Ann M. Dillner Chin H. Phuah Jay R. Turner 《Atmospheric environment (Oxford, England : 1994)》2009,43(37):5937-5943
Ambient carbonaceous material collected on quartz filters is prone to measurement artifacts due to material gained or lost during post-sampling field latency, shipping, and storage. In seventeen sampling events over a one year period, ambient PM2.5 aerosols were collected on quartz filters (without denuders) and subjected to various filter treatments to assess the potential for and extent of artifacts. The filter treatments simulated post-sampling environments that filters may be exposed to and included: storage at 40 °C for up to 96 h, storage at ?16 °C for 48 h, and storage at room temperature (~21 °C) for 48 h. Carbon mass on the filters was measured using a thermal-optical method. The total carbon (TC), total organic carbon (TOC) and total elemental carbon (TEC) as well as carbon thermal fraction masses were obtained. Statistical analyses were performed to identify significant differences in carbon fraction concentrations between filters analyzed immediately after sampling and after being subjected to treatment.TOC and TC concentrations decreased by on average 15 ± 5% and 10 ± 4%, respectively, for filters maintained at 40 °C for 96 h but did not change for filters stored at room temperature or frozen for 48 h. TEC did not change for any of the filter treatments. The mass concentration for the organic carbon thermal fraction that evolves at the lowest temperature step (OC1) decreased with increasing storage time at 40 °C with average losses of 70 ± 7% after 96 h. Therefore, OC1 is not a stable measurement due to post-sampling conditions that may be encountered. This work demonstrates that TOC and TC can have substantial measurement artifacts on filters subjected to field latency and other non-temperature controlled post-sampling handling, compared to the carbon loadings on the filter at the end of the sampling period. 相似文献
6.
Nabil Semmar Maurice Jay Muhammad Farman Maurice Roux 《Environmental Modeling and Assessment》2008,13(1):17-33
The quantitative assessment of plant diversity and its monitoring with time represent a key environmental issue for management
and conservation of natural resources. Assessment of plant diversity could be based on chemical analyses of secondary metabolites
(e.g. flavonoids, terpenoids), because of the substantial quantitative and qualitative between-individual variability in such
compounds. At a geographical scale, the plant populations become widely dispersed, and their monitoring from numerous routine
individual analyses could become restricting. To overcome such constraint, this study develops a multivariate calibration
model giving the relative frequency of a particular taxon from a simple high-performance liquid chromatography (HPLC) analysis
of a plant mixture. The model was built from a complete set of mixtures combining different taxons, according to an experimental
design (Scheffé’s matrix). For each mixture, a reference HPLC pattern was simulated by averaging the individual HPLC profiles
of the constitutive taxons. The calibration models, based on Bayesian discriminant analysis (BDA), gave statistical relationships
between the contributions of each taxon in mixtures and reference HPLC patterns of these mixtures. Finally, these models were
validated on new mixtures by using outside plants. This new biodiversity survey approach is illustrated on four chemical taxons
(four chemotypes) of Astragalus caprinus (Fabaceae). The more differentiated the taxon, the better predicted its contributions (in mixtures) were by BDA calibration
model. This new approach could be very useful for a global routine survey of plant diversity. 相似文献
7.
Jay M. Iwasaki Barbara I. P. Barratt Janice M. Lord Alison R. Mercer Katharine J. M. Dickinson 《Ambio》2015,44(7):694-704
The Varroa mite (Varroa destructor) is implicated as a major disease factor in honey bee (Apis mellifera) populations worldwide. Honey bees are extensively relied upon for pollination services, and in countries such as New Zealand and Australia where honey bees have been introduced specifically for commercial pollinator services, the economic effects of any decline in honey bee numbers are predicted to be profound. V. destructor established in New Zealand in 2000 but as yet, Australia remains Varroa-free. Here we analyze the history of V. destructor invasion and spread in New Zealand and discuss the likely long-term impacts. When the mite was discovered in New Zealand, it was considered too well established for eradication to be feasible. Despite control efforts, V. destructor has since spread throughout the country. Today, assessing the impacts of the arrival of V. destructor in this country is compromised by a paucity of data on pollinator communities as they existed prior to invasion. Australia’s Varroa-free status provides a rare and likely brief window of opportunity for the global bee research community to gain understanding of honey bee-native pollinator community dynamics prior to Varroa invasion. 相似文献
8.
9.
Jay S. Jacobson 《Journal of the Air & Waste Management Association (1995)》2013,63(10):1071-1073
Editor’s note: This paper by Dr. Jacobson was presented at the 74th annual meeting of the Air Pollution Control Association as part of a panel discussion entitled “Acid Rain–1981: An International Issue.” The session was held on June 22, 1981, and was arranged by APCA’s TT-6 Energy-Environmental Interactions Committee. 相似文献
10.
Effect of pH control at the anode for the electrokinetic removal of phenanthrene from kaolin soil 总被引:14,自引:0,他引:14
Polycyclic aromatic hydrocarbon (PAH)-contaminated soils exist at numerous sites, and these sites may threaten public health and the environment because many PAH compounds are toxic, mutagenic, and/or carcinogenic. PAHs are also hydrophobic and persistent, so conventional remediation methods are often costly or inefficient, especially when the contaminants are present in low permeability and/or organic soils. An innovative technique, electrokinetically enhanced in situ flushing, has the potential to increase soil-solution-contaminant interaction and PAH removal efficiency for low permeability soils; however, the electrolysis reaction at the anode may adversely affect the remediation of low acid buffering capacity soils, such as kaolin. Therefore, the objective of this study was to improve the remediation of low acid buffering soils by controlling the pH at the anode to counteract the electrolysis reaction. Six bench-scale electrokinetic experiments were conducted, where each test employed one of three different flushing solutions, deionized water, a surfactant, or a cosolvent. For each of these solutions, tests were performed with and without a 0.01 M NaOH solution at the anode to control the pH. The test using deionized water with pH control generated a higher electroosmotic flow than the equivalent test performed without pH control, but the electroosmotic flow difference between the surfactant and cosolvent tests with and without pH control was minor compared to that observed with the deionized water tests. Controlling the pH was beneficial for increasing contaminant solubilization and migration from the soil region adjacent to the anode, but the high contaminant concentrations that resulted in the middle or cathode soil regions indicates that subsequent changes in the soil and/or solution chemistry caused contaminant deposition and low overall contaminant removal efficiency. 相似文献