Capability of Raman lidar for monitoring the variation of atmospheric CO2 profile

Lidar （Light detection and ranging） has special capabilities for remote sensing of many different behaviours of the atmosphere. One of the techniques which show a great deal of promise for several applications is Raman scattering. The detecting capability, including maximum operation range and minimum detectable gas concentration is one of the most significant parameters for lidar remote sensing of pollutants. In this paper, based on the new method for evaluating the capabilities of a Raman lidar system, we present an evaluation of detecting capability of Raman lidar for monitoring atmospheric CO2 in Hefei. Numerical simulations about the influence of atmospheric conditions on lidar detecting capability were carried out, and a conclusion can be drawn that the maximum difference of the operation ranges caused by the weather conditions alone can reach about 0.4 to 0.5km with a measuring precision within 30ppmv. The range of minimum detectable concentration caused by the weather conditions alone can reach about 20 to 35 ppmv in vertical direction for 20000 shots at a distance of 1 km on the assumption that other parameters are kept constant. The other corresponding parameters under different conditions are also given. The capability of Raman lidar operated in vertical direction was found to be superior to that operated in horizontal direction. During practical measurement with the Raman lidar whose hardware components were fixed, aerosol scattering extinction effect would be a significant factor that influenced the capability of Raman lidar. This work may be a valuable reference for lidar system designing, measurement accuracy improving and data processing.     

A new differential absorption lidar for NO_2 measurements using Raman-shifted technique

Based on Raman-shifted wavelengths of D2 and CH4 pumped by third harmonic of Nd:YAG laser, a differential absorption lidar was presented in this paper and had been constructed for probing environmental NO2 concentration. NO2 experimental measurements were carried out at Anhui Institute of Optics and Fine Mechanics in Hefei. Some NO2 measurement results were given and discussed.     

SO2在吸收池内的稳定性研究

在室温条条件下,以Xe灯为光源,利用SO2的紫外吸收光谱,研究了SO2的浓度随时间连续变化规律。实验中考虑了温度和充垫气体N2对SO2的浓度变化的影响。实验结果表明：SO2的浓度基本上是随时间线性变化的;同时,SO2的浓度变化率与光照时间有关。     

偏振-米散射激光雷达对卷云的探测

 研制了一台偏振-米散射激光雷达,用于卷云和沙尘气溶胶后向散射光退偏振比的探测研究。介绍了偏振-米散射激光雷达的探测原理,叙述了偏振-米散射激光雷达的结构、技术参数、测量方法和数据处理方法。给出了偏振-米散射激光雷达对合肥市西郊上空卷云的结构、退偏振比垂直廓线以及光学厚度的典型探测结果,对这些结果进行了分析和讨论。初步探测结果表明,合肥西郊上空高度在6～10 km的卷云的退偏振比在0.2～0.5之间,该激光雷达可以对卷云进行有效的探测,能较好地反映卷云及其光学特性的时空分布。     

大气气溶胶粒子折射率虚部反演方法研究

提出了反演折射率虚部的方法.以光散射为原理的粒子计数器测量光学等效直径,其结果受折射率虚部的影响较大;以粒子飞行时间为原理的粒子计数器测量空气动力学直径,其结果不受折射率虚部的影响.利用两种仪器的测量结果受折射率影响的差异来反演大气气溶胶的折射率虚部.通过与其它独立的测量结果对比表明,该方法反演气溶胶折射率虚部是合理的.     

激光雷达信号随机误差的估算

在分析随机误差来源和激光雷达数据特点的基础上,介绍一种新的随机误差计算方法--噪音比例因子方法.该方法用一次测量数据列中远处背景信号算出噪音比例因子,再由噪音比例因子求出任一距离上有用信号的随机误差.用实测的激光雷达信号进行检验,结果表明,这种方法是可靠且可行的.     

Er3+在二氧化硅介孔分子筛中的高效率发光及其分析

研究了一种新型的负载Er³⁺的二氧化硅介孔分子筛纳米材料,分析了其在有无功能化试剂全氟甲基磺酰(bis(perfluoromethylsulfonyl)amine)修饰作用下的吸收和荧光光谱特性,获得了高强度的荧光发射. 应用Judd-Ofelt理论计算了强度参数(Ω₂＝1.88×10^-20cm²,Ω₄＝5.45×10^-20cm^{2关键词： 发光 二氧化硅介孔分子筛 稀土离子 Judd-Ofelt理论}     

偏振-米散射激光雷达的研制

研制的偏振-米散射激光雷达（PML）,可用于探测卷云和沙尘气溶胶的后向散射光退偏振比以及研究流层大气气溶胶的消光特性。采用窄带滤光片和光阑,将接收到的激光大气回波信号谱线（米散射和瑞利散射光谱）从天空太阳背景噪声中分离出来,以提高系统的白天探测能力。介绍了偏振-米散射激光雷达的结构、技术参数、测量方法和数据处理方法。对偏振-米散射激光雷达的性能参数进行了测定,并对测定结果进行了分析与讨论,给出了偏振-米散射激光雷达对合肥市地区(117.16°E, 31.90°N)上空大气气溶胶的消光特性和卷云的结构、退偏振比垂直廓线以及光学厚度的典型探测结果,对这些结果进行了分析和讨论。结果表明：研制的偏振-米散射激光雷达性能可靠,能对大气气溶胶和卷云的物理和光学特性进行有效的探测。     

用于微全分析系统的数字化微流控芯片的研究

研制出一种基于介质上电润湿(electrowetting-on-d ielectric,EWOD)机制的可编程数字化微流控芯片。它采用“三明治”结构:受控离散液滴被夹在两极板之间;下极板以硅为衬底,掺杂多晶硅作为芯片微电极阵列,其上涂覆有Teflon(AF1600薄膜的S iO2作为疏水性介质层;上极板是涂覆有Teflon(AF1600疏水薄膜的透明电极。通过分析数字化微流控系统的基本操作(离散液滴的传输、拆分及混合)的物理机理和模拟优化,在35 V低驱动电压下实现了约0.35μL和0.45μL去离子水离散液滴的传输和合并,并在70 V驱动电压下实现了0.8μL液滴的拆分等操作。     

有限线性空间的可解线-传递自同构群

设S是一个有限线性空间 ,G是S的自同构群的一个可解线 传递子群 ,则对于给定的线长k ,除了有限对 (S ,G)外 ,S有v =pⁿ 个点 ,且G≤AΓL( 1 ,pⁿ ) .