全文获取类型
收费全文 | 10917篇 |
免费 | 945篇 |
国内免费 | 110篇 |
学科分类
工业技术 | 11972篇 |
出版年
2024年 | 35篇 |
2023年 | 210篇 |
2022年 | 345篇 |
2021年 | 708篇 |
2020年 | 640篇 |
2019年 | 773篇 |
2018年 | 886篇 |
2017年 | 816篇 |
2016年 | 831篇 |
2015年 | 494篇 |
2014年 | 787篇 |
2013年 | 1179篇 |
2012年 | 766篇 |
2011年 | 821篇 |
2010年 | 553篇 |
2009年 | 470篇 |
2008年 | 287篇 |
2007年 | 226篇 |
2006年 | 178篇 |
2005年 | 130篇 |
2004年 | 120篇 |
2003年 | 68篇 |
2002年 | 70篇 |
2001年 | 38篇 |
2000年 | 37篇 |
1999年 | 42篇 |
1998年 | 63篇 |
1997年 | 45篇 |
1996年 | 36篇 |
1995年 | 38篇 |
1994年 | 21篇 |
1993年 | 25篇 |
1992年 | 16篇 |
1991年 | 22篇 |
1990年 | 22篇 |
1989年 | 26篇 |
1988年 | 17篇 |
1987年 | 13篇 |
1986年 | 14篇 |
1985年 | 19篇 |
1984年 | 16篇 |
1983年 | 14篇 |
1982年 | 9篇 |
1981年 | 7篇 |
1980年 | 7篇 |
1979年 | 5篇 |
1978年 | 5篇 |
1977年 | 4篇 |
1976年 | 5篇 |
1973年 | 6篇 |
排序方式: 共有10000条查询结果,搜索用时 93 毫秒
31.
Zohal Safaei Mahmoudabadi Alimorad Rashidi Mohammad Panahi 《International Journal of Hydrogen Energy》2021,46(7):5270-5285
Highly active ReS2 nanocatalysts were prepared by CVD method and characterized by XRD, BET -BJH, Raman spectroscopy, XPS, TPR, NH3-TPD, SEM, and HRTEM techniques. Catalytic activities were used in upgrading heavy crude oil using methane as hydrogen source. The results showed a significant increase in API and decrease in sulfur and nitrogen content of crude oil. RSM technique was used to investigate the interactive effects of temperature (200–400 °C), pressure (20–40 bar) and dosage of nanocatalyst (0.5–2 wt. %) on the performance of HDS reaction. The results represent that the maximum predicted HDS activity (74.375%) was estimated under the optimal conditions (400 °C, 20 bars, and 2 wt % of nanocatalyst). Also, the effect of reaction temperature, pressure and dosage of ReS2 nanorods catalyst on HDN of heavy crude oil was investigated and highest efficiency in the HDN process (93%) occurred at 400 °C and 40 bar using 2 wt % ReS2. 相似文献
32.
Zahra Kiarsi Mohammad Hojjati Behrooz Alizadeh Behbahani Mohammad Noshad 《Journal of Food Safety》2020,40(3):e12782
Nutmeg (Myristica fragrans) seed was subjected to the hydro-distillation method to extract its essential oil (NEO). Its main constituents were α-pinene (20.16%), sabinene (14.45%), and β-pinene (13.26%) with great antimicrobial and antioxidant actions. A novel edible coating was then fabricated based on the sage seed mucilage (SSM) and NEO, to ameliorate the quality and shelf-life of beef slices. The NEO-loaded SSM coating was able to significantly decrease the population of total viable count, Escherichia coli, Staphylococcus aureus, psychrotrophic bacteria, and fungi. Moreover, lipid oxidation of beef slices was remarkably suppressed upon the application of bioactive NEO-loaded SSM edible coating, as compared with the control by Day 6. The coated beef sample, especially NEO-rich SSM coated ones perceived a higher consumer acceptance and firmness than the SSM coated and noncoated samples. The SSM edible coating containing NEO could therefore have the potential to control the growth of pathogenic microorganisms and lipid oxidation, and to improve the color stability and sensory properties of meat and meat products. 相似文献
33.
A stochastic model for local disturbances, particularly for a temporal harmonic with random modulations in amplitude and/or phase, is proposed in this paper. Results for the second moment responses of a linear single-degree-of-freedom system to this type of stochastic loading demonstrate a significant change in response characteristics due to a small uncertainty. A local phenomenon may last much longer and resonance may be smeared to a broad range. Integrated with wavelet transform, the proposed approach may be used to model a random process with non-stationary frequency content. Especially, it can be effectively used for Monte Carlo simulation to generate large size of samples that have similar characteristics in time and frequency domains as a pre-selected mother sample has. The technique has a great potential for the case where uncertainty study is warranted but the available samples are limited. 相似文献
34.
OBJECTIVE: To study the effects of an aldose reductase inhibitor (ARI-509, Wyeth-Ayerst, Princeton, NJ) and aminoguanidine (AMG), agents that have been reported to prevent or delay diabetic retinopathy, on retinal vascular abnormalities and the immunocytochemical expression in the retina of vascular endothelial growth factor (VEGF) in rats maintained for up to 2 years on a 50% galactose diet. METHODS: Albino rats were placed on a control diet, a diet containing 50% galactose, or the 50% galactose diet containing either ARI-509 or AMG. Treatment with ARI-509 or AMG was initiated at the beginning of the experiment or after 12 months of galactose feeding. After 22 to 24 months, the rats were killed and the retinal vasculature from half of one eye was isolated by trypsin-elastase digestion for semiquantitative evaluation of retinal vascular lesions. The other half of the retina was prepared for immunocytochemistry and stained for the presence of VEGF, factor VIII, vimentin, and glial fibrillary acidic protein. Red blood cells, sciatic nerves, and a portion of the retina from the second eye were assayed for glucose, galactose, fructose, sorbitol, galactitol, and myo-inositol. Red blood cells were also assayed for galactosylated hemoglobin. RESULTS: Galactose-fed animals developed a vascular retinopathy characterized by severe cellular loss in the retinal capillaries and intensification of periodic acid-Schiff staining of the vascular basement membranes. Some animals also displayed dilation and hypercellularity of vessels in the posterior retina. These changes were substantially reduced in animals receiving ARI-509 from the beginning of the galactose diet, but were unaffected in all of the other treatment groups. None of the rats receiving ARI-509 or AMG treatment, whether initiated from the onset or after 12 months of galactosemia, demonstrated VEGF immunoreactivity. With the exception of the animals receiving ARI-509 from the beginning of the experiment, all of the galactose-fed animals developed dense cataracts within 6 weeks of the beginning of the galactose diet. Galactitol levels in animals receiving ARI-509 were 86% to 93% lower in red blood cells, retina, and sciatic nerve than those in the other galactose-fed groups. CONCLUSIONS: Although ARI-509 and AMG have different abilities to delay or prevent the diabetic-like retinopathy in galactosemic rats, even when substantial retinal microvascular acellularity occurs, both drugs prevent the immunocytochemical expression of VEGF. These results suggest that factors other than hypoxia may be responsible for VEGF expression in the retina, and that aldose reductase inhibitors and AMG have potential roles in preventing such expression and, thus, perhaps preventing retinal neovascularization. 相似文献
35.
Murad Nour Mohammad Belfiore Jean Claude Guisantes George Rodriguez 《Wireless Personal Communications》2002,20(2):145-161
In DS-WCDMA mobile systems such the UMTS, asynchronous cell site operation,assigning different long spreading code to each cell, yields the advantageof flexible system deployment. We can design an indoor system basedon an outdoor one. However, in general, much longer search time isrequired in asynchronous operation than in synchronous. This paperproposes three techniques to take decisions about synchronizationbased on observation of correlated signals. Classical decision criterialike maximum and threshold criterion are presented. A new decisioncriteria that we call Threshold&Max combined decision criteriais analyzed. The results of this new introduced technique is comparedwith the classical ones. 相似文献
36.
Novel polyurethane insulating coatings were prepared from the reaction of glycerin‐terminated polyurethane prepolymers (GPUPs) and a blocked isocyanate curing agent (BIC). The GPUPs were prepared from the reaction of one equivalent of polycaprolactone polyol (CAPA 210) with an excess amount of 4,4′‐methylene bis(phenyl isocyanate) (MDI) and subsequent reaction of the NCO‐terminated polyurethane with glycerin. The BIC was prepared from the reaction of trimethylol propane (TMP), toluene diisocyanate (TDI) and N‐methylaniline (NMA). The polyols and curing agent were characterized by conventional methods while the curing condition was optimized via gel content measurements. The curing kinetics of the polyurethane coating were investigated and the kinetic parameters derived. The crosslink densities of the samples were determined via the equilibrium swelling method, using the Flory–Rehner equation. The relationships between the crosslink density and the electrical, physical, mechanical and dynamic mechanical properties of the coatings were also studied. Copyright © 2005 Society of Chemical Industry 相似文献
37.
Mohammad Mozammel Hoq Tsuneo Yamane Shoichi Shimizu Tadashi Funada Shiro Ishida 《Journal of the American Oil Chemists' Society》1985,62(6):1016-1021
Continuous hydrolysis of olive oil byCandida cylindracea’s lipase was studied in a microporous hydrophobic membrane bioreactor. Olive oil and buffer solution, fed continuously through two compartments partitioned by membrane, caused reaction at the interface of lipase-adsorbed membrane and buffer solution. Fatty acid was obtained in a single phase without being mixed with components of other phases. At all mean residence times, countercurrent flow mode was superior to cocurrent one. The lipase was adsorbed onto the membrane, and its adsorption was suggested to be partially specific from the experiments with enzymes having various levels of purity. The percent hydrolysis depended hyperbolically on the interfacial enzyme concentration. The hydrolysis seemed to be limited by diffusion of fat or fatty acid through the micropores of the membrane at higher interfacial enzyme concentrations. The lipase was stabilized significantly by glycerol added to the buffer solution. Satisfactory performance of the membrane bioreactor was obtained in a longterm continuous operation which lasted for 24 days by feeding buffer-glycerol (18.0%) solution over the adsorbed lipase. The operational half-life of the adsorbed enzyme was 15 days at 40 C. 相似文献
38.
39.
40.
Mohammad Ziabari Vahid Mottaghitalab Scott T. McGovern A. K. Haghi 《Nanoscale research letters》2007,2(12):597-600
In this paper, a new image analysis based method for electrospun nanofiber diameter measurement has been presented. The method
was tested by a simulated image with known characteristics and a real web. Mean (M) and standard deviation (STD) of fiber
diameter obtained using this method for the simulated image were 15.02 and 4.80 pixels respectively, compared to the true
values of 15.35 and 4.47 pixels. For the real web, applying the method resulted in M and STD of 324 and 50.4 nm which are
extremely close to the values of 319 and 42 nm obtained using manual method. The results show that this approach is successful
in making fast, accurate automated measurements of electrospun fiber diameters. 相似文献