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491.
Geoffrey F. Davies 《Physics and Chemistry of Minerals》1981,7(6):246-252
Several deficiencies are demonstrated in previous formulations of three-body interatomic forces, and revised and extended formulations are presented for the case of the NaCl lattice. A commonly used formulation of non-central forces and a formulation of the effect of ellipsoidal atom deformation are incorrect. Atom deformation should in general introduce two degrees of freedom in the NaCl lattice, but the only previous correct formulation of deformation effects, the commonly used “breathing shell model,” includes only one degree of freedom. The “shell model” of polarizable atoms has been correctly formulated, but applications seem to have been arbitrarily restricted to the case where short-range forces act only on shells, and not on cores. Because of these errors and incompletenesses, it is concluded that no three-body forces have been convincingly established or characterized, although the necessity of their inclusion in models is clear. 相似文献
492.
This paper uses the MERGE integrated assessment model to identify the least-cost mitigation strategy for achieving a range of climate policies. Mitigation is measured in terms of GDP foregone. This is not a benefit-cost analysis. No attempt is made to calculate the reduction in damages brought about by a particular policy. Assumptions are varied regarding the availability of energy-producing and energy-using technologies. We find pathways with substantial reductions in temperature change, with the cost of reductions varying significantly, depending on policy and technology assumptions. The set of scenarios elucidates the potential energy system transformation demands that could be placed on society. We find that policy that allows for “overshoot” of a radiative forcing target during the century results in lower costs, but also a higher temperature at the end of the century. We explore the implications of the costs and availability of key mitigation technologies, including carbon capture and storage (CCS), bioenergy, and their combination, known as BECS, as well as nuclear and energy efficiency. The role of “negative emissions” via BECS in particular is examined. Finally, we demonstrate the implications of nationally adopted emissions timetables based on articulated goals as a counterpoint to a global stabilization approach. 相似文献
493.
This paper synthesizes results of the multi-model Energy Modeling Forum 27 (EMF27) with a focus on climate policy scenarios. The study included two harmonized long-term climate targets of 450 ppm CO2-e (enforced in 2100) and 550 pm CO2-e (not-to-exceed) as well as two more fragmented policies based on national and regional emissions targets. Stabilizing atmospheric GHG concentrations at 450 and 550 ppm CO2-e requires a dramatic reduction of carbon emissions compared to baseline levels. Mitigation pathways for the 450 CO2-e target are largely overlapping with the 550 CO2-e pathways in the first half of the century, and the lower level is achieved through rapid reductions in atmospheric concentrations in the second half of the century aided by negative anthropogenic carbon flows. A fragmented scenario designed to extrapolate current levels of ambition into the future falls short of the emissions reductions required under the harmonized targets. In a more aggressive scenario intended to capture a break from observed levels of stringency, emissions are still somewhat higher in the second half due to unabated emissions from non-participating countries, emphasizing that a phase-out of global emissions in the long term can only be reached with full global participation. A key finding is that a large range of energy-related CO2 emissions can be compatible with a given long-term target, depending on assumptions about carbon cycle response, non-CO2 and land use CO2 emissions abatement, partly explaining the spread in mitigation costs. 相似文献
494.
Geoffrey M. Morrison Sonia Yeh Anthony R. Eggert Christopher Yang James H. Nelson Jeffery B. Greenblatt Raphael Isaac Mark Z. Jacobson Josiah Johnston Daniel M. Kammen Ana Mileva Jack Moore David Roland-Holst Max Wei John P. Weyant James H. Williams Ray Williams Christina B. Zapata 《Climatic change》2015,131(4):545-557
495.
Measurements of the Henry's Law Coefficients of 2-Methyl-3-buten-2-ol, Methacrolein, and Methylvinyl Ketone 总被引:1,自引:0,他引:1
Laura T. Iraci Bradly M. Baker Geoffrey S. Tyndall John J. Orlando 《Journal of Atmospheric Chemistry》1999,33(3):321-330
Using an equilibrium headspace technique, Henry's law coefficients were measured for methacrolein (H = 6.5 ± 0.7 M atm-1) and methylvinyl ketone (41 ± 7.0 M atm-1) in water at 25 °C. In addition, 2-methyl-3-buten-2-ol was studied at 30 °C in water and in an aqueous ionic solution representative of plant tissue. Similar values were found in deionized water (65 ± 3.5 M atm-1) and in a 0.05 mol kg-1 Ca2+, K+, NO3-, SO42- solution (62 ± 0.8 M atm-1). These Henry's Law coefficients are too small to allow for significant partitioning of methacrolein, methylvinyl ketone or methylbutenol into cloud water under equilibrium conditions. 相似文献
496.