全文获取类型
收费全文 | 3129篇 |
免费 | 51篇 |
国内免费 | 8篇 |
学科分类
工业技术 | 3188篇 |
出版年
2023年 | 11篇 |
2022年 | 9篇 |
2021年 | 45篇 |
2020年 | 15篇 |
2019年 | 31篇 |
2018年 | 27篇 |
2017年 | 25篇 |
2016年 | 32篇 |
2015年 | 21篇 |
2014年 | 47篇 |
2013年 | 126篇 |
2012年 | 89篇 |
2011年 | 135篇 |
2010年 | 102篇 |
2009年 | 123篇 |
2008年 | 133篇 |
2007年 | 100篇 |
2006年 | 79篇 |
2005年 | 79篇 |
2004年 | 83篇 |
2003年 | 90篇 |
2002年 | 90篇 |
2001年 | 67篇 |
2000年 | 54篇 |
1999年 | 62篇 |
1998年 | 331篇 |
1997年 | 180篇 |
1996年 | 167篇 |
1995年 | 96篇 |
1994年 | 89篇 |
1993年 | 91篇 |
1992年 | 45篇 |
1991年 | 37篇 |
1990年 | 34篇 |
1989年 | 45篇 |
1988年 | 46篇 |
1987年 | 40篇 |
1986年 | 27篇 |
1985年 | 30篇 |
1984年 | 26篇 |
1983年 | 29篇 |
1982年 | 28篇 |
1981年 | 25篇 |
1980年 | 35篇 |
1979年 | 16篇 |
1978年 | 16篇 |
1977年 | 20篇 |
1976年 | 33篇 |
1975年 | 8篇 |
1973年 | 4篇 |
排序方式: 共有3188条查询结果,搜索用时 93 毫秒
91.
Takashi Inoue 《Carbon》2007,45(11):2164-2170
Iron-based nanoparticles, centrifugally classified by size, with variation of subnanometer order, have been used for the growth of diameter-controlled carbon nanotubes (CNTs) for the first time via catalytic chemical vapor deposition. The centrifugal classification of nanoparticles is facilitated by fractional precipitations through the sequential addition of ethanol to a hexane solution containing the nanoparticles. Three different nanoparticle sizes were obtained, which have average diameters and standard deviations of 3.9 ± 0.8 nm, 3.3 ± 0.6 nm, and 2.8 ± 0.4 nm. By the classification process of nanoparticles, the standard deviation of the average diameter of the fractionated nanoparticles decreased by around one half of that of the as-synthesized nanoparticles. In addition, we demonstrate a technique for estimating the average diameter of each classified nanoparticle using conventional low-angle X-ray diffraction, without the need for time-consuming TEM observation and analysis. From the three classified nanoparticle sizes, with average diameters of 2.8, 3.3, and 3.9 nm, CNTs with average diameters of 3.1, 3.6, and 4.5 nm were obtained by changing growth temperatures, respectively. Therefore, centrifugally classified nanoparticles are one of the most promising ‘seeds’ for use in the diameter-selective growth of CNTs. 相似文献
92.
H. Kominami J. Kato Y. Takada Y. Doushi B. Ohtani S. Nishimoto M. Inoue T. Inui Y. Kera 《Catalysis Letters》1997,46(3-4):235-240
Thermal decomposition of titanium(IV) tetra-tert-butoxide (TTB) in inert organic solvents at 573 K yielded microcrystalline
anatase (titanium(IV) oxide, TiO2) powders with a crystallite size of ca. 9 nm and a surface area of <100 m2 g-1. Primary and secondary alkoxides of titanium(IV), however, were not decomposed under similar conditions, indicating that
the thermal stability of C-O bonds in the alkoxides was a decisive factor for their decomposition. The TiO2 prepared from TTB by this manner was thermally stable upon calcination in air and retained high surface area of ca. 100 m2 g-1 even after calcination at 823 K. The as-prepared TiO2 powders, without calcination, exhibited much higher rate of carbon dioxide formation than any other active photocatalysts
such as Degussa P-25 and Ishihara ST-01 in the photocatalytic mineralization of acetic acid in aerated aqueous solutions.
The higher activity of the present TiO2 photocatalysts is attributed to both high crystallinity and large surface of the present product. The calcination of the
as-prepared TiO2 in air reduced the photocatalytic activity, but it was still higher than the other commercially available TiO2's.
This revised version was published online in July 2006 with corrections to the Cover Date. 相似文献
93.
Reactive blending of polyamide 6 (PA) with polyethylene (PE) having reactive sites, maleic anhydride (MAH content=0.1 wt%),and glycidyl methacrylate (GMA content=3-12 wt%), was carried out at 70/30 and 65/35 (PA/PE) blend ratios. Blend morphology evolved by reactive blending was analyzed by light scattering and transmission electron microscopy. The blends were then irradiated by electron beam. The degree of crosslinking was estimated by measuring the dynamic storage modulus at a temperature above melting point of PA. It was found that surface-to-surface interparticle distance τ was significantly reduced by the micelle formation via pull-out of in situ-formed graft copolymers. The blend with shorter τ was crosslinked by electron-beam irradiation at the lower dose level. A blend having the minimum τ (∼0.2 μm) was nicely crosslinked at a low dose level same as for PE, and even for the PA matrix system. 相似文献
94.
Norihiro Moriyama Yuta Kawano Qing Wang Ryota Inoue Meng Guo Makoto Yokoji Hiroki Nagasawa Masakoto Kanezashi Toshinori Tsuru 《American Institute of Chemical Engineers》2021,67(7):e17223
Pervaporation (PV) is a membrane technology that holds great promise for industrial applications. To better understand the PV mechanism, PV dehydrations of various types of organic solvents (methanol, ethanol, iso-propanol, tert-butanol, and acetone) were performed on five types of organosilica and two types of silicon carbide-based membranes, all with different pore sizes. Water permeance was dependent on the types of organic aqueous solutions, which suggested that organic solvents penetrated the pores and hindered the permeation of water. In addition, water permeance of various types of membranes in PV was well correlated with hydrogen permeance in single-gas permeation. Furthermore, a clear correlation was obtained between the permeance ratio in PV and that in single-gas permeation, which was confirmed via the modified-gas translation model. These correlations make it possible to use single-gas permeation properties to predict PV performance. 相似文献
95.
A. Ohmori Z. Zhou K. Inoue K. Murakami T. Sasaki 《Journal of Thermal Spray Technology》1996,5(2):134-138
The penetration phenomena of liquid manganese (Mn) alloy into porous ZrO2 (8 vvt % Y2O3) coating plasma sprayed on SS400 steel substrate was studied by heating in a vacuum atmosphere. The improvement in mechanical
properties of the coating by heat treatment with liquid Mn alloys was examined. Liquid Mn alloys, such as Mn-Cu, Mn-Sn, and
Mn-In, rapidly penetrated the coating and formed a chemical bond between the coating and the substrate. The densification
of the ZrO2 coating occurred when ZrO2 particles were sintered with liquid Mn alloys that penetrated the porous coating. The dense coating was free of porosity,
and its hardness increased after heat treatment with Mn alloys, compared with assprayed ZrO2 coating. Moreover, the fracture toughness of the coating reached the same levels as those of sintered yttria-stabilized PSZ. 相似文献
96.
Toshiji Mukai T. G. Nieh Yoshihito Kawamura Akihisa Inoue Kenji Higashi 《Intermetallics》2002,10(11-12)
Mechanical deformation of Pd40Ni40P20 was characterized in compression over a wide strain rate range (3.3×10−5 to 2×103 s−1) at room temperature. The compression sample fractured with a shear plane inclined 42 degree with respect to the loading axis, in contrast to 56 degree for the case of tension. This suggests the yielding of the material deviates from the classical von Mises yield criterion, but follows the Mohr-Coulomb yield criterion. Fracture stress as well as strain was found to decrease with increasing applied strain rate. The compressive stress (1.74 GPa) was also found to be higher than the tensile fracture stress at a quasi-static strain rate. Close examination of the stress–strain curves revealed that localized shear might have occurred at a compressive stress of about 1.4 GPa, much lower than the “apparent” yield stress of 1.74 GPa. However, the stress of 1.4 GPa for shear band initiation is almost the same as the fracture stress measured at a dynamic strain rate of 5×102 s−1. These results suggested that the fracture of a bulk metallic glass is sensitive to the applied loading rate. 相似文献
97.
Recently, we revealed a standard pattern of a macroscopic molecular network for controlling morphogenetic processes such as the development of organs, including blast, mesoderm, heart, and hands during about sevenfold cell divisions and a standard bio-chemical clock like the circadian one (Naitoh in Artif Life Robot 13, 2008; Japan J Ind Appl Math 28(1), 2011; J Phys Conf Ser 344, 2012; Artif Life Robot 17, 2012) A network model derived logically based on experimental observations is described by a nonlinear differential equation for predicting time evolutions of six macroscopic molecular groups: three gene groups and three enzyme groups, which include promoting and suppressing factors. Here, the macroscopic model extended for also describing aging processes shows various types of cycles and reveals the physical condition for determining whether or not living beings such as humans can survive after getting ill. It is stressed that, after becoming ill, living systems with overly fast generation of information molecules such as various genes end in death, whereas relatively fast production of enzymes leads to recovery. This may also explain an essential feature underlying carcinogenic processes. 相似文献
98.
Hamid Noori Farhad Mehdipour Kazuaki Murakami Koji Inoue Morteza Saheb Zamani 《The Journal of supercomputing》2008,45(3):313-340
To improve the performance of embedded processors, an effective technique is collapsing critical computation subgraphs as
application-specific instruction set extensions and executing them on custom functional units. The problem with this approach
is the immense cost and the long times required to design a new processor for each application. As a solution to this issue,
we propose an adaptive extensible processor in which custom instructions (CIs) are generated and added after chip-fabrication.
To support this feature, custom functional units are replaced by a reconfigurable matrix of functional units (FUs). A systematic
quantitative approach is used for determining the appropriate structure of the reconfigurable functional unit (RFU). We also
introduce an integrated framework for generating mappable CIs on the RFU. Using this architecture, performance is improved
by up to 1.33, with an average improvement of 1.16, compared to a 4-issue in-order RISC processor. By partitioning the configuration
memory, detecting similar/subset CIs and merging small CIs, the size of the configuration memory is reduced by 40%. 相似文献
99.
Kenichi Mori Michiaki Sakamoto Jin Matsushima Daisuke Inoue Kenichirou Naka Ken Sumiyoshi 《Journal of the Society for Information Display》2009,17(6):513-518
Abstract— In order to improve the reflective contrast ratio of transflective IPS‐LCDs, a novel pixel design for a normally white reflective IPS has been proposed. In this design, the large‐inter‐electrode‐spacing layout using a novel driving method and a double‐layered electrode have effectively reduced the light leakage. By applying these two technologies, a transflective IPS‐LCD has been successfully demonstrated with a high contrast ratio (15:1) in the reflective mode and a wide‐viewing‐angle characteristic in the transmissive mode. 相似文献
100.
We developed equipment and methods for measuring quantitatively the local Young's modulus of solids. It consists of an electrodeless langasite oscillator and line antennas, and oscillator vibrations are generated and detected contactlessly. A constant biasing force results from oscillator mass and is independent of surface roughness. The effect of material anisotropy on the measured stiffness is theoretically discussed for studying the limitation of the quantitative measurement. The microscopy has been applied to polycrystalline copper, and the measured modulus is compared to calculations based on electron-backscatter-diffraction measurements. Also, we applied it to a duplex stainless steel and an embedded silicon-carbide fiber. The results reveal textured regions, defects with high sensitivity, and even stiffness distribution in a single grain. 相似文献