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1.
Surface waters of Alsea Bay, an unpolluted estuary on the Oregon coast, were analysed for nitrous oxide, nitrate and nitrite on a weekly or biweekly basis during the summer of 1979. The estuary was found to be a variable source of N2O to the atmosphere. Large and rapid increases in the concentrations of N2O, NO3?, and NO2? occurred at the beginning of the sampling period and are attributed to the influx of nutrient-rich upwelling water into the estuary with the tide. The subsequent decline in concentrations of nitrate, nitrite and nitrous oxide over the remainder of the summer is attributed to a decrease in upwelling intensity, a decline in nitrification rates and to assimilatory nitrate reduction. Measurements of nitrous oxide at six stations along the Alsea River were also made in September and October before and after the onset of the rainy season. Samples taken after flood conditions were established were systematically 50% higher than pre-flood samples. The data suggest that soil runoff results in elevated concentrations of N2O in rivers. 相似文献
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Yves Goddéris Louis M. François Jacques Schott David Labat 《Geochimica et cosmochimica acta》2006,70(5):1128-1147
A numerical model of chemical weathering in soil horizons and underlying bedrock (WITCH) has been coupled to a numerical model of water and carbon cycles in forest ecosystems (ASPECTS) to simulate the concentration of major species within the soil horizons and the stream of the Strengbach granitic watershed, located in the Vosges Mountains (France). For the first time, simulations of solute concentrations in soil layers and in the catchment river have been performed on a seasonal basis. The model is able to reproduce the concentrations of most major species within the soil horizons, as well as catching the first-order seasonal fluctuations of aqueous calcium, magnesium and silica concentrations. However, the WITCH model underestimates concentrations of Mg2+ and silica at the spring of the catchment stream, and significantly underestimates Ca2+ concentration. The deficit in calculated calcium can be compensated for by dissolution of trace apatite disseminated in the bedrock. However, the resulting increased Ca2+ release yields important smectite precipitation in the deepest model layer (in contact with the bedrock) and subsequent removal of large amount of silica and magnesium from solution. In contrast, the model accurately accounts for the concentrations of major species (Ca, Mg and silica) measured in the catchment stream when precipitation of clay minerals is not allowed. The model underestimation of Mg2+ and H4SiO4 concentrations when precipitation of well crystallized smectites is allowed strongly suggests that precipitation of well crystallized clay minerals is overestimated and that more soluble poorly crystallized and amorphous materials may be forming. In agreement with observations on other watersheds draining granitic rocks, this study indicates that highly soluble trace calcic phases control the aqueous calcium budget in the Strengbach watershed. 相似文献
5.
Re-Os Isotopic Measurements at the Femtomole Level in Natural Samples 总被引:17,自引:0,他引:17
Jean Louis Birck Matthieu Roy Barman Françoise Capmas 《Geostandards and Geoanalytical Research》1997,21(1):19-27
Here we describe a new chemical separation method for Os and an improved mass spectrometric procedure for Re and Os. This technique is based on the selective extraction of OsO4 from aqueous solution in liquid bromine. Among other advantages, this procedure avoids the cumbersome distillation procedure for Os and uses only commercial "off the shelf" PFA teflon labware. Blank levels for 0.5 g sample sizes are: 0.06 pg and 0.5 pg for Os and Re respectively. Samples containing as little as 1 pg g−1 Os can be analysed reliably with this method. Adaptation to other dissolution methods is also discussed. 相似文献
6.
Gérald Darnis Dominique Robert Corinne Pomerleau Heike Link Philippe Archambault R. John Nelson Maxime Geoffroy Jean-éric Tremblay Connie Lovejoy Steve H. Ferguson Brian P. V. Hunt Louis Fortier 《Climatic change》2012,115(1):179-205
As part of the Canadian contribution to the International Polar Year (IPY), several major international research programs have focused on offshore arctic marine ecosystems. The general goal of these projects was to improve our understanding of how the response of arctic marine ecosystems to climate warming will alter food web structure and ecosystem services provided to Northerners. At least four key findings from these projects relating to arctic heterotrophic food web, pelagic-benthic coupling and biodiversity have emerged: (1) Contrary to a long-standing paradigm of dormant ecosystems during the long arctic winter, major food web components showed relatively high level of winter activity, well before the spring release of ice algae and subsequent phytoplankton bloom. Such phenological plasticity among key secondary producers like zooplankton may thus narrow the risks of extreme mismatch between primary production and secondary production in an increasingly variable arctic environment. (2) Tight pelagic-benthic coupling and consequent recycling of nutrients at the seafloor characterize specific regions of the Canadian Arctic, such as the North Water polynya and Lancaster Sound. The latter constitute hot spots of benthic ecosystem functioning compared to regions where zooplankton-mediated processes weaken the pelagic-benthic coupling. (3) In contrast with another widely shared assumption of lower biodiversity, arctic marine biodiversity is comparable to that reported off Atlantic and Pacific coasts of Canada, albeit threatened by the potential colonization of subarctic species. (4) The rapid decrease of summer sea-ice cover allows increasing numbers of killer whales to use the Canadian High Arctic as a hunting ground. The stronger presence of this species, bound to become a new apex predator of arctic seas, will likely affect populations of endemic arctic marine mammals such as the narwhal, bowhead, and beluga whales. 相似文献
7.
Vertical distributions of particulate silica, and of production and dissolution rates of biogenic silica, were determined on two N-S transects across the Pacific sector of the Antarctic Circumpolar Current during the austral spring of 1978. Particulate silica profiles showed elevated levels in surface water and near the bottom, with low (35–110 nmol Si · 1?1) and vertically uniform values through the intervening water column. Both the particulate silica content of the upper 200 m and the production rate of biogenic silica in the photic zone increased from north to south, reaching their highest values near the edge of the receding pack ice. A significant, but variable, fraction (18–58%) of the biogenic silica produced in the surface layer was redissolving in the upper 90–98 m. Net production of biogenic silica in the surface layer (production minus dissolution) was proceeding at a mean rate of ca. 2 mmol Si · m?2 · day?1. This is ca. 4 times greater than the most recent estimate of the mean accumulation rate of siliceous sediments beneath the ACC. We estimate, based on mass balance, that the mean dissolution rate of biogenic silica in subsurface water column in the Southern Ocean is 1.2–2.9 mmol Si · m?2 · day?1. 相似文献
8.
An automatic sample changer based upon a commercially available 20-port rotary valve has been developed for use in automated seawater nutrient analyses. All parts exposed to seawater are of stainless steel, Teflon®, or Kel-F®. The sampler has proven to be rugged and efficient in both shore and shipboard laboratories. 相似文献
9.
Louis M. Barbier Robert Smith Scott Murphy Eric R. Christian Rodger Farley John F. Krizmanic John W. Mitchell Robert E. Streitmatter Eugene C. Loh Stephen Stochaj 《Astroparticle Physics》2005,22(5-6):439-449
We have designed and built an instrument to measure and monitor the “nightglow” of the Earth’s atmosphere in the near ultraviolet (NUV). In this paper we describe the design of this instrument, called NIGHTGLOW. NIGHTGLOW is designed to be flown from a high altitude research balloon, and circumnavigate the globe. NIGHTGLOW is a NASA, University of Utah, and New Mexico State University project. A test flight took place from Palestine, Texas on July 5, 2000, lasting about 8 h. The instrument performed well and landed safely in Stiles, Texas with little damage. The resulting measurements of the NUV nightglow are compared with previous measurements from sounding rockets and balloons. 相似文献
10.
Douglas S. Hall Gregory W. Henry Dietmar Böhme Peter A. Brooks Sandy Chang Ales Dolzan George L. Fortier Robert E. Fried Russell M. Genet Bruce S. Grim James Hannon Darrel B. Hoff Kevin Krisciunas Howard J. Landis Howard P. Louth Larry P. Lovell Paul Nielsen Bobby E. Powell Harry D. Powell Don Pray Thomas R. Renner Charles W. Rogers Stephen Shervais Douglas M. Slauson Samuel Slote Harold J. Stelzer Arthur J. Stokes Jack C. Troeger Louis C. Turner Norman F. Wasson Kenneth W. Zeigler 《Journal of Astrophysics and Astronomy》1991,12(4):281-287
We present photoelectric photometry of λ And never before published, obtained between February 1982 and December 1990 at 29
different observatories. Then we combine it with all other photometry available to us (previously published, contained in
the I.A.U. Commission 27 Archives, and obtained with the Vanderbilt 16-inch automatic telescope but not yet published), to
yield a 14.8-year data base. Analysis reveals a long-term cycle in mean brightness, with a full range of 0m.15 and a period of 11.4 ± 0.4 years. Because most of our new photometry was concentrated in the 1983-84 observing season,
we analyze that one well-defined light curve with a two-spot model. Spot A keeps a 0m.04 amplitude throughout four rotation cycles whereas the amplitude of spot B diminishes from 0m.09 down almost to 0m.03. The spot rotation periods were 55d.9 ± 0d.6 and 520d.8 ± 1d.0, respectively. 相似文献