NiPd合金在升温过程中择尤溅射的研究

用卢瑟福背散射技术,测定了NiPd(48.2wt%Pd)合金在不同温度时的溅射原子角分布,从而确定了Ni和Pd原子的部分产额随样品温度的变化关系。结果发现:Ni和Pd的部分溅射产额在居里温度附近均有较大变化,而且Pd的产额变化幅度比Ni的变化幅度大;Ni是择尤溅射元素,但是在磁相转变过程中,其择尤溅射程度却随样品温度的升高而减小。经讨论后指出,上述现象可能是由于在磁相转变过程中原子表面结合能减小和离子轰击引起的表面偏析共同引起的。 关键词：     

高电荷态离子与SiO2表面相互作用的研究

高电荷态离子(Pbq ,Arq )由兰州近代物理研究所的ECR实验平台所产生,轰击非晶态SiO2表面.用微通道板测量溅射粒子产额的角分布.用公式拟合实验溅射角分布得到了较好的结果,并给出了初步的理论解释.由此得出了高电荷态离子与SiO2表面作用的微分溅射截面.实验结果表明高电荷态离子能够增加动能溅射;同时高电荷态离子入射能够引起势能溅射.在大角度入射时,溅射产额主要是由碰撞引起的;在小角入射时势能溅射所占比重会增大.     

Al-50wt% Sn合金的离子溅射研究

用捕获膜技术和卢瑟福背散射(RBS)分析,测定Al-Sn多相合金在30keV Ar⁺离子轰击时Al和Sn的溅射原子角分布。溅射后的样品用扫描电子显微镜(SEM)进行观察,并用电子微探针分析仪(EPMA)对轰击样品(靶点)和未轰击样品作成分分析。结果表明,Al的溅射原子角分布近于cosine形状,而Sn却是over-cosine型角分布。本文给出一个按不同表面形貌特征划分的各元素富集区i进行叠加的产额表达式,Y(θ)=∑Y_i(θ),解释了实验结果。 关键词：     

溅射角分布形状与Spike效应的相关性

Sigmund 69年提出的线性碰撞级联理论,成功地解决了多晶体与无定形的单元素靶的溅射产额问题。根据反冲原子速度分布是各向同性的假定,他又推导出单元素靶溅射角分布是cosine形状,即溅射角分布可用A(cosβ)”函数描述,其中形状指数n=1。但是不少实验事实表明,对于中等以上质量的离子和靶原子来说,当离子能≥10~1Kev数量级级时,单元素靶溅射角分布是 over——cosine形状,即形状指数n>1。产生这种现象的机制至今仍不清楚。本文认为:在整个碰撞级联中,不全是线性碰撞,     

离子轰击入射角对溅射参数的影响

本文用基于两体碰撞近似的蒙特-卡罗模拟方法研究离子轰击入射角对溅射参数的影响,讨论了入射角与溅射产额、溅射粒子能谱、角分布和阈能的关系,并把计算结果与某些半经验公式和实验数据进行了比较。 关键词：     

Ni－50wt％Ti合金的择优溅射

用卢瑟福背散射技术测定了Ｎｉ５０ｗｔ％Ｔｉ合金在３０ｋｅＶＡｒ＋离子轰击时的组分原子（Ｎｉ和Ｔｉ）溅射角分布．结果表明，Ｎｉ原子和Ｔｉ原子的角分布存在差别：Ｎｉ原子在靶表面法线方向（发射角θ＝０°附近）择优发射，而Ｔｉ原子则在大发射角区域（θ＞４５°）发射较Ｎｉ强．根据元素在靶点表面按形貌特征局域富集情况的观测，对实验结果进行了讨论     

中能中子与208Pb反应的理论计算和分析

在中子与原子核Pb及其同位素反应的总截面,去弹性散射截面,弹性散射截面和弹性散射角分布的实验数据基础上,获得了入射中子能量从1—300MeV的一组普适中子与Pb及其同位素反应的光学模型势参数.应用光学模型,扭曲波玻恩近似理论,宽度涨落修正的Hauser-Feshbach理论,预平衡反应的激子模型和核内级联模型,计算和分析了中子与²⁴⁸Pb反应的所有截面、角分布和能谱.理论计算与实验数据进行了分析比较     

超短超强激光与固体靶相互作用中超热电子的角分布

 用3TW超短超强激光器进行了激光与固体靶相互作用实验。采用电子角分布仪和LiF热释光探测器探测了超热电子的角分布。测量结果显示：能量较高的电子发射的定向性好于能量较低的电子；能量较低的电子呈溅射状发射；能量较高的电子发射出现两个尖锐的发射峰，其中，激光反射方向的超热电子发射峰则由反射激光、有质动力径向分量、侧向拉曼散射等加速机制共同作用的结果，靠近靶法线方向的超热电子发射峰是由其振吸收机制产生，且理论预言与实验结果相吻合。     

中子与52Cr反应截面的理论分析

根据中子与天然核Cr及其同位素反应的总截面,去弹性散射截面和弹性散射角分布的实验数据,获得了入射中子能量从1MeV—250MeV的一组普适中子与Cr及其同位素反应的光学模型势参数.应用光学模型,扭曲波玻恩近似理论,宽度涨落修正的Hauser-Feshbach理论,和预平衡反应的激子模型,计算和分析了中子与⁵²Cr反应的所有截面、角分布、能谱和双微分截面.理论计算与实验数据进行了分析比较.     

溅射原子角分布与靶点表面形貌的关联研究

27keV的Ar⁺离子垂直轰击处于不同温度的Cd靶,用捕获膜技术和Rutherford背散射谱仪(RBS)测定溅射原子角分布,并对所有样品的靶点形貌进行扫描电子显微镜(SEM)观察。结果发现,所有的角分布都呈over-cosine形状,但是在极角为0°处实验值与cosine值的偏离△,是不同的,在靶温度为150℃时的偏离△_T小于在室温时的偏离△_R,亦即△_T<△_R,提出一个简单的模型对这种溅射角分布 关键词：     

Angular distribution of Cherenkov radiation from relativistic heavy ions taking into account deceleration in the radiator

Numerical methods are used to study the dependence of the structure and the width of the angular distribution of Vavilov-Cherenkov radiation with a fixed wavelength in the vicinity of the Cherenkov cone on the radiator parameters (thickness and refractive index), as well as on the parameters of the relativistic heavy ion beam (charge and initial energy). The deceleration of relativistic heavy ions in the radiator, which decreases the velocity of ions, modifies the condition of structural interference of the waves emitted from various segments of the trajectory; as a result, a complex distribution of Vavilov-Cherenkov radiation appears. The main quantity is the stopping power of a thin layer of the radiator (average loss of the ion energy), which is calculated by the Bethe-Bloch formula and using the SRIM code package. A simple formula is obtained to estimate the angular distribution width of Cherenkov radiation (with a fixed wavelength) from relativistic heavy ions taking into account the deceleration in the radiator. The measurement of this width can provide direct information on the charge of the ion that passes through the radiator, which extends the potentialities of Cherenkov detectors. The isotopic effect (dependence of the angular distribution of Vavilov-Cherenkov radiation on the ion mass) is also considered.     

Temperature dependence of angular characteristics of boron nitride sputtering

The angular dependence of the sputtering yield and the spatial distribution of particles ejecting from a boron nitride polycrystal with a wurtzite structure in the temperature range from 0 to 2800°C under bombardment with 300 eV xenon ions are calculated by the molecular dynamics method. A reduction of steepness of the curves of angular dependence of boron nitride sputtering with increasing temperature is revealed. Features of the obtained distributions are analyzed on the basis of mechanisms of interaction of slow heavy ions with surface target atoms.     

On the equilibrium isotopic composition of the thorium–uranium–plutonium fuel cycle

The equilibrium isotopic compositions and the times to equilibrium in the process of thorium–uranium–plutonium oxide fuel recycling in VVER-type reactors using heavy water mixed with light water are estimated. It is demonstrated thEhfat such reactors have a capacity to operate with self-reproduction of active isotopes in the equilibrium mode.     

Closed Thorium-Uranium-Plutonium Cycle Concept in Nuclear Power Engineering

The use of 232Th instead of 238U as a fertile isotope, 233U instead of 239Pu as the main fissile isotope, heavy water instead of light water as a coolant, and its dilution with light water in the VVER reactor campaign make possible self-enrichment of fuel with fissile isotopes, including the time upon achieving the balanced isotopic abundance ratio of actinides, and also provide conditions for closing the Th-U-Pu fuel cycle. This allows increasing the fuel lifetime by around two orders of magnitude, making it much easier to handle radioactive waste, reducing the nuclear hazard of PWE reactors, and providing a technological barrier to prevent the distribution of fissile materials and nuclear technologies.     

Production of neutron-deficient nuclei around N = 126 by proton-induced spallation

Many isotopes of Np, Pu, Am, and Cm around the N = 126 shell still have not been produced in the laboratory. This study aims to investigate the cross sections and yields of the neutron-deficient nuclei of Np, Pu, Am, and Cm produced in the proton-induced spallations of transuranium elements. The isospin-dependent quantum molecular dynamics (IQMD) model is applied to study the dynamical process of reaction, and the subsequent decay process is simulated by the GEMINI++ model. The IQMD-GEMINI++ model is applied to calculate the cross section, kinetic energy, and angular distribution of the isotopic productions around N = 126. The Lindhand, Scharff, and Schiott theory is applied to calculate the energy loss of different heavy nuclei in the target material. A comparison between the data and the calculations shows that the IQMD-GEMINI++ model can reproduce the production cross sections of the neutron-deficient nuclei in spallation within approximately 1.5 orders of magnitude. The maximum cross section of the undiscovered isotopes of Np, Pu, Am, and Cm is about 10^?5 mb, while the kinetic energies of the productions are all less than 16 MeV. The angular distribution shows that the emission direction of production is mostly at a backward angle. The range of production in the target is within the range of 10^?7 to 10^?5 cm. This range is the effective target thickness for the online identification of undiscovered isotopes. Based on the effective thickness of the target and assuming an intensity of 120 μA for the proton beam, the yields of the undiscovered neutron-deficient nuclei are calculated. Productions of the undiscovered isotopes of Np, Pu, Am, and Cm by the proton-induced spallations of transuranium elements are feasible. However, experimental techniques for online identification of neutron-deficient nuclei produced in proton-induced spallation should be developed.     

Computer simulation of two-component target sputtering

The TRIM SP computer simulation program, which is based on the binary collision approximation, is applied to sputtering of two component targets. The topics discussed in this paper are: contribution of different processes leading to sputtering, total and partial sputtering yields, surface compositions at stationary conditions, sputtering of isotopic mixtures, angular and energy distributions and the escape depth of sputtered particles. Targets investigated are TaC, WC, TiC, TiD₂, and B (as an isotope mixture), bombarded by the noble gas ions and D (in the case of TiD₂). Comparison with experimental data and calculated results show good agreement demonstrating that collisional effects are sufficient to describe the experimental data in the examples investigated.     

Recoil study of multinucleon transfer reactions: Capture of six charges by Nd targets in Ar induced reactions

Multinucleon transfer reactions induced with Ar ions and involving the capture of six charges by the target have been studied. The targets were all the separated isotopes of Nd, and the observed nuclei were ^149gTb, ¹⁵⁰Dy, ¹⁵¹Dy. The experimental technique involved the measurement of the cross sections, angular distributions, and recoil range at each recoil angle, of the heavy residual nuclei. After transformation of the data into the c.m. system, the angular distributions appear to be peaked backwards, close to 180°. This observation suggests that the present reactions are of the same type as the multinucleon transfer reactions studied by other authors for which the angular distribution of the light fragment was peaked forward in the c.m. system. The energy distributions in the c.m. system were used to check the feasibility of various mechanisms which could lead to the production of the observed isotopes. Each mechanism was supposed to be a two-step process: the first step was the exchange, from the projectile to the target, of a number n of nucléons, leading to an excited intermediate nucleus, and the second step the deexcitation of the intermediate nucleus by nuclear evaporation. This analysis indicates that the most probable mechanisms correspond to n close to 12 (6 protons and 6 neutrons), and to an excitation energy of about 60 MeV for the intermediate nucleus. The distribution of cross sections versus the number of nucléons gained by the target is also in accord with this reaction model.     

Temperature of Heavy Fragments in Heavy-Ion Collisions

The heavy fragments in heavy-ion collisions are finally formed after the hot prefragments undergo sequential decay,of whom the temperature should be much lower than that of prefragments.Using the double ratio(DR) method,the isotopic thermometer(Tiso) for heavy fragment is constructed using the yield of heavy isotopes.T iso of heavy fragment is obtained by analyzing the measured data in the 1A GeV124,136Xe and 140A MeV 48Ca/64Ni reactions.Result shows that T iso varies from 0.5 MeV to 10 MeV.But most T iso is around 1±0.5 MeV,which is much lower than temperature of light particles.Result also indicates that the difference between T iso of heavy fragments in different reactions is very small,and T iso is independent on the size of the reaction system,the incident energy and the neutron-richness of the projectile.     

离子轰击引起的表面形貌对Ag的溅射产额的影响

用捕获膜技术和卢瑟福背散射(RBS)谱仪测定Ag靶在27keV Ar⁺离子轰击下的溅射原子角分布,从而确定不同剂量下Ag的溅射产额,并对其靶点表面形貌进行扫描电子显微镜(SEM)观察。结果发现,所有的角分布都呈over-cosine形状,但其溅射产额却随着表面形貌不同而不同。根据溅射产额Y与轰击离子入射角φ变化关系,讨论不同轰击剂量下溅射产额的差别,肯定了表面形貌是影响溅射产额的一个重要因素,并由此提出“表观产额”的新概念。 关键词：     

Disentangling effects of nuclear structure in heavy element formation

Forming the same heavy compound nucleus with different isotopes of the projectile and target elements allows nuclear structure effects in the entrance channel (resulting in static deformation) and in the dinuclear system to be disentangled. Using three isotopes of Ti and W, forming 232Cm, with measurement spanning the capture barrier energies, alignment of the heavy prolate deformed nucleus is shown to be the main reason for the broadening of the mass distribution of the quasifission fragments as the beam energy is reduced. The complex, consistently evolving mass-angle correlations that are observed carry more information than the integrated mass or angular distributions, and should severely test models of quasifission.