Quantum phase interference and spin-parity in Mn12 single-molecule magnets

Magnetization measurements of Mn12 molecular nanomagnets with spin ground states of S=10 and S=19/2 show resonance tunneling at avoided energy level crossings. The observed oscillations of the tunnel probability as a function of the magnetic field applied along the hard anisotropy axis are due to topological quantum phase interference of two tunnel paths of opposite windings. Spin-parity dependent tunneling is established by comparing the quantum phase interference of integer and half-integer spin systems.     

Nonequilibrium dynamics of anisotropic large spins in the kondo regime: time-dependent numerical renormalization group analysis

We investigate the time-dependent Kondo effect in a single-molecule magnet (SMM) strongly coupled to metallic electrodes. Describing the SMM by a Kondo model with large spin S>1/2, we analyze the underscreening of the local moment and the effect of anisotropy terms on the relaxation dynamics of the magnetization. Underscreening by single-channel Kondo processes leads to a logarithmically slow relaxation, while finite uniaxial anisotropy causes a saturation of the SMM's magnetization. Additional transverse anisotropy terms induce quantum spin tunneling and a pseudospin-1/2 Kondo effect sensitive to the spin parity.     

All-electric-controlled spin current switching in single-molecule magnet-tunnel junctions

A single-molecule magnet (SMM) coupled to two normal metallic electrodes can both switch spin-up and spin-down electronic currents within two different windows of SMM gate voltage. Such spin current switching in the SMM tunnel junction arises from spin-selected single electron resonant tunneling via the lowest unoccupied molecular orbit of the SMM. Since it is not magnetically controlled but all-electrically controlled,the proposed spin current switching effect may have potential applications in future spintronics.     

Manipulating the spin states in a double molecular magnets tunneling junction

We theoretically explore the spin transport through nano-structures consisting of two serially coupled single-molecular magnets (SMM) sandwiched between two nonmagnetic electrodes. We find that the magnetization of SMM can be controlled by the spin transfer torque with respect to the bias voltage direction, and the electron current can be switched on/off in different magnetic structures. Such a manipulation is performed by full electrical manner, and needs neither external magnetic field nor ferromagnetic electrodes in the tunneling junction. The proposal device scheme can be realized with the use of the present technology [6] and has potential applications in molecular spintronics or quantum information processing.     

Topological phase interference effects in resonant quantum tunneling of the Néel vector between nonequivalent magnetic wells in mesoscopic single-domain antiferromagnets

Resonant quantum tunneling of the Néel vector between nonequivalent magnetic wells is investigated theoretically for a nanometer-scale single-domain antiferromagnet with biaxial crystal symmetry in the presence of an external magnetic field applied along the easy anisotropy axis, based on the two-sublattice model. Both the Wentzel-Kramers-Brillouin exponent and the preexponential factors are evaluated in the instanton contribution to the tunneling rate for finite and zero magnetic fields by applying the instanton technique in the spin-coherent-state path-integral representation, respectively. The quantum interference or spin-parity effects induced by the topological phase term in the Euclidean action are discussed in the rate of quantum tunneling of the Néel vector. In the absence of an external applied magnetic field, the effect of destructive phase interference or topological quenching on resonant quantum tunneling of the Néel vector is evident for the half-integer excess spin antiferromagnetic nanoparticle. In the weak field limit, the tunneling rates are found to oscillate with the external applied magnetic field for both integer and half-integer excess spins. We discuss the experimental condition on the applied magnetic field which may allow one to observe the topological quenching effect for nanometer-scale single-domain antiferromagnets with half-integer excess spins. Tunneling behavior in resonant quantum tunneling of the magnetization vector between nonequivalent magnetic wells is also studied for a nanometer-scale single-domain ferromagnet by applying the similar technique, but in the large noncompensation limit. Received 4 June 1999     

Giant mesoscopic spin Hall effect on the surface of topological insulator

We study mesoscopic spin Hall effect on the surface of a topological insulator with a step-function potential by using the McMillan method commonly used in the study of superconductor junctions. In the ballistic transport regime, we predict a giant spin polarization induced by a transverse electric current with parameter suitable to the topological insulator thin film Bi(2)Se(3). The spin polarization oscillates across the potential boundary with no confinement due to the Klein paradox, and should be observable in a spin resolved scanning tunneling microscope.     

Momentum and spin filtering of electrons on the surface of a topological insulator

We study theoretically electron tunneling through planar magnetic barrier arrays on the surface of a three-dimensional topological insulator. Interestingly, the transmission displays a collimation behavior at some specific incident angles. This feature provides us a new way to construct a momentum and spin filter in topological insulators.     

Cooper-pair injection into quantum spin Hall insulators

We theoretically study tunneling of Cooper pairs from a superconductor spanning a two-dimensional topological insulator strip into its helical edge states. The coherent low-energy electron-pair tunneling sets off positive current cross correlations along the edges, which reflect an interplay of two quantum-entanglement processes. Most importantly, superconducting spin pairing dictates a Cooper pair partitioning into the helical edge liquids, which transport electrons in opposite directions for opposite spin orientations. At the same time, Luttinger-liquid correlations fractionalize electrons injected at a given edge into counterpropagating charge pulses carrying definite fractions of the elementary electron charge.     

Inelastic tunneling of electrons through a quantum dot with an embedded single molecular magnet

We report a theoretical analysis of electron transport through a quantum dot with an embedded biaxial single-molecule magnet (SMM) based on mapping of the many-body interaction-system onto a one-body problem by means of the non-equilibrium Green function technique. It is found that the conducting current exhibits a stepwise behavior and the nonlinear differential conductance displays additional peaks with variation of the sweeping speed and the magnitude of magnetic field. This observation can be interpreted by the interaction of electron-spin with the SMM and the quantum tunneling of magnetization. The inelastic conductance and the corresponding tunneling processes are investigated with normal as well as ferromagnetic electrodes. In the case of ferromagnetic configuration, the coupling to the SMM leads to an asymmetric tunneling magnetoresistance (TMR), which can be enhanced or suppressed greatly in certain regions. Moreover, a sudden TMR-switch with the variation of magnetic field is observed, which is seen to be caused by the inelastic tunneling.     

Current correlations in quantum spin Hall insulators

We consider a four-terminal setup of a two-dimensional topological insulator (quantum spin Hall insulator) with local tunneling between the upper and lower edges. The edge modes are modeled as helical Luttinger liquids and the electron-electron interactions are taken into account exactly. Using perturbation theory in the tunneling, we derive the cumulant generating function for the interedge current. We show that different possible transport channels give rise to different signatures in the current noise and current cross correlations, which could be exploited in experiments to elucidate the interplay between electron-electron interactions and the helical nature of the edge states.     

Spin injection from topological insulator tunnel-coupled to metallic leads

We study theoretically helical edge states of 2D and 3D topological insulators (TI) tunnel-coupled to metal leads and show that their transport properties are strongly affected by contacts as the latter play a role of a heat bath and induce damping and relaxation of electrons in the helical states of TI. A simple structure that produces a pure spin current in the external circuit is proposed. The current and spin current delivered to the external circuit depend on relation between characteristic lengths: damping length due to tunneling, contact length and, in case of 3D TI, mean free path and spin relaxation length caused by momentum scattering. If the damping length due to tunneling is the smallest one, then the electric and spin currents are proportional to the conductance quantum in 2D TI, and to the conductance quantum multiplied by the ratio of the contact width to the Fermi wavelength in 3D TI.     

Surface scattering via bulk continuum states in the 3D topological insulator Bi2Se3

We have performed scanning tunneling microscopy and differential tunneling conductance (dI/dV) mapping for the surface of the three-dimensional topological insulator Bi(2)Se(3). The fast Fourier transformation applied to the dI/dV image shows an electron interference pattern near Dirac node despite the general belief that the backscattering is well suppressed in the bulk energy gap region. The comparison of the present experimental result with theoretical surface and bulk band structures shows that the electron interference occurs through the scattering between the surface states near the Dirac node and the bulk continuum states.     

Scattering of Wave Packets on the Surface of Topological Insulators in the Presence of Potential Barriers with Magnetization

The nonstationary Schrödinger equation is solved numerically by the Cayley method for wave packets that are formed from surface states on the surface of topological insulators and are scattered by a potential barrier, including a barrier with magnetization. The transmission coefficient and spin density distributions are calculated. Expressions are found for the static transmission coefficient through a barrier with the use of the plane-wave approximation and its generalization for wave packets. It is shown that the two-dimensional nature of wave packets leads to noticeable differences in the behavior of the transmission coefficient compared to that in the plane-wave scattering problem. For instance, two-dimensional packets exhibit a significant suppression of Klein tunneling in some energy regions. The results obtained show that the tunneling and spin density of localized wave-packet-type electronic states in structures based on topological insulators can be affected through potential barriers.     

Photon-assisted tunneling in a biased strongly correlated Bose gas

We study the impact of coherently generated lattice photons on an atomic Mott insulator subjected to a uniform force. Analogous to an array of tunnel-coupled and biased quantum dots, we observe sharp, interaction-shifted photon-assisted tunneling resonances corresponding to tunneling one and two lattice sites either with or against the force and resolve multiorbital shifts of these resonances. By driving a Landau-Zener sweep across such a resonance, we realize a quantum phase transition between a paramagnet and an antiferromagnet and observe quench dynamics when the system is tuned to the critical point. Direct extensions will produce gauge fields and site-resolved spin flips, for topological physics and quantum computing.     

Two-dimensional topological insulator state and topological phase transition in bilayer graphene

We show that gated bilayer graphene hosts a strong topological insulator (TI) phase in the presence of Rashba spin-orbit (SO) coupling. We find that gated bilayer graphene under preserved time-reversal symmetry is a quantum valley Hall insulator for small Rashba SO coupling λ(R), and transitions to a strong TI when λ(R)>√[U(2)+t(⊥)(2)], where U and t(⊥) are, respectively, the interlayer potential and tunneling energy. Different from a conventional quantum spin Hall state, the edge modes of our strong TI phase exhibit both spin and valley filtering, and thus share the properties of both quantum spin Hall and quantum valley Hall insulators. The strong TI phase remains robust in the presence of weak graphene intrinsic SO coupling.     

Spin-asymmetric Josephson effect

We propose that with ultracold Fermi gases one can realize a spin-asymmetric Josephson effect in which the two spin components of a Cooper pair are driven asymmetrically--corresponding to driving a Josephson junction of two superconductors with different voltages V(↑) and V(↓) for spin up and down electrons, respectively. We predict that the spin up and down components oscillate at the same frequency but with different amplitudes. Furthermore our results reveal that the standard interpretation of the Josephson supercurrent in terms of coherent bosonic pair tunneling is insufficient. We provide an intuitive interpretation of the Josephson supercurrent as interference in Rabi oscillations of pairs and single particles, the latter causing the asymmetry.     

Quantum coherence and W∞ × SU(2) algebra in bilayer quantum Hall systems

We analyze the bilayer quantum Hall (QH) system by mapping it to the monolayer QH system with spin degrees of freedom. By this mapping the tunneling interaction term is identified with the Zeeman term. We clarify the mechanism of a spontaneous development of quantum coherence based on the Chern-Simons gauge theory with the lowest-Landau-level projection taken into account. The symmetry group is found to be W_∞ × SU(2), which says that the spin rotation affects the total electron density nearby. Using it extensively we construct the Landau-Ginzburg theory of the coherent mode. Skyrmion excitations are topological solitions in this coherent mode. We point out that they are detectable by measuring the Hall current distribution.     

Quasiparticle states and quantum interference induced by magnetic impurities on a two-dimensional topological superconductor

We theoretically study the effect of localized magnetic impurities on two-dimensional topological superconductor (TSC). We show that the local density of states (LDOS) can be tuned by the effective exchange field m, the chemical potential μ of TSC, and the distance Δr as well as the relative spin angle α between two impurities. The changes in Δr between two impurities alter the interference and result in significant modifications to the bonding and antibonding states. Furthermore, the bound-state spin LDOS induced by single and double magnetic impurity scattering, the quantum corrals and the quantum mirages are also discussed. Finally, we briefly compare the impurities in TSC with those in topological insulators.     

Superexchange interaction enhancement of the quantum transport in a DNA-type molecule

We use the transfer matrix method and the Green function technique to theoretically study the quantum tunnelling through a DNA-type molecule. Ferromagnetic electrodes are used to produce the spin-polarized transmission probability and therefore the spin current. The distance-dependent crossover comes from the topological variation from the one-dimensional to the two-dimensional model transform as we switch on the interstrand coupling; a new base pair will present N-1 extrachannels for the charge and spin as N being the total base pairs. This will restrain the decay of the transmission and improve the stability of the quantum transport. The spin and charge transfer through the DNA-type molecule is consistent with the quantum tunneling barrier.