Estimate of the effect of the 11-year solar activity cycle on the ozone content in the stratosphere

Using spectral, cross-spectral, and regression methods, we analyzed the effect of the 11-year cycle of solar activity on the ozone content in the stratosphere and lower mesosphere via satellite measurement data obtained with the help of SBUV/SBUV2 instruments in 1978–2003. We revealed a high coherence between the ozone content and solar activity level on the solar cycle scale. In much of this area, the ozone content varies approximately in phase with the solar cycle; however, in areas of significant gradients of ozone mixing ratio in the middle stratosphere, the phase shift between ozone and solar oscillations can be considerable, up to π/2. This can be caused by dynamical processes. The altitude maxima of ozone sensitivity to the 11-year solar cycle were found in the upper vicinity of the stratopause (50–55 km), in the middle stratosphere (35–40 km), and the lower stratosphere (below 25 km). Maximal changes in ozone content in the solar cycle (up to 10% and more) were found in winter and spring in polar regions.     

冬季太阳11年周期活动对大气环流的影响

利用气象场的再分析资料和太阳辐射活动资料,对太阳11年周期活动影响北半球冬季(11月~3月)大气环流的过程进行了统计分析和动力学诊断.根据赤道平流层纬向风准两年振荡(QBO)的东、西风状态对太阳活动效应进行了分类讨论,结果表明：东风态QBO时,太阳活动效应主要集中在赤道平流层中、高层和南半球平流层,强太阳活动时增强的紫外辐射加热了赤道地区的臭氧层,造成平流层低纬明显增温,同时加强了南半球的Brewer-Dobson(B-D)环流,引起南极高纬平流层温度增加;而北半球中高纬的环流主要受行星波的影响,太阳活动影响很小.西风态QBO时,太阳活动效应在北半球更为重要,初冬时强太阳活动除了加热赤道地区臭氧层外,还抑制了北半球的B-D环流,造成赤道平流层温度增加和纬向风梯度在垂直方向的变化,从而改变了对流层两支行星波波导的强度;冬末时在太阳活动调制下,行星波向极波导增强,B-D环流逐渐恢复,造成北半球极地平流层明显增温,同时伴随着赤道区域温度的下降.     

Ozone variation in the lower stratosphere and its mechanism

Seasonal variations of ozone are studied by taking into consideration both photochemical and dynamical processes. Assuming that the seasonal variations of total ozone amounts are linear combinations of photochemical equilibrium variations and those due to atmospheric motions, the observed variations of the total ozone amount seem reasonably to be explained.The concept mentioned above implies that the time scale of ozone might be rather short in the lower stratosphere. The order of the half restoration time was estimated to be 10 to 10² days in the lower stratosphere. Thus the estimated time scale of ozone must be somewhat longer than that of the temperature in the lower stratosphere, of which variation usually shows its maximum in the midwinter in middle latitudes, while that of ozone shows its maximum in the late winter or early spring. As the maximum values of both quantities would appear in the early summer without air motions, the similarity in the phase differences of temperature and ozone suggests the validity of the concept of this paper.     

Simulation of the stratospheric ozone and temperature response to the solar irradiance variability during sun rotation cycle

Despite substantial progress in atmospheric modeling, the agreement of the simulated atmospheric response to decadal scale solar variability with the solar signal in different atmospheric quantities obtained from the statistical analysis of the observations cannot be qualified as successful. An alternative way to validate the simulated solar signal is to compare the sensitivity of the model to the solar irradiance variability on shorter time scales. To study atmospheric response to the 28-day solar rotation cycle, we used the chemistry–climate model SOCOL that represents the main physical–chemical processes in the atmosphere from the ground up to the mesopause. An ensemble simulation has been carried out, which is comprised of nine 1-year long runs, driven by the spectral solar irradiance prescribed on a daily basis using UARS SUSIM measurements for the year 1992. The correlation of zonal mean hydroxyl, ozone and temperature averaged over the tropics with solar irradiance time series have been analyzed. The hydroxyl has robust correlations with solar irradiance in the upper stratosphere and mesosphere, because the hydroxyl concentration is defined mostly by the photolysis. The simulated sensitivity of the hydroxyl to the solar irradiance changes is in good agreement with previous estimations. The ozone and temperature correlations are more complicated because their behavior depends on non-linear dynamics and transport in the atmosphere. The model simulates marginally significant ozone response to the solar irradiance variability during the Sun rotation cycle, but the simulated temperature response is not robust. The physical nature of this is not clear yet. It seems likely that the temperature (and partly the ozone) daily fields possess their own internal variability, which is not stable and can differ from year to year reflecting different dynamical states of the system.     

Sensitivity of the Earth’s middle atmosphere to short-term solar variability and its dependence on the choice of solar irradiance data set

We simulate the time evolution of the neutral and charged species in the terrestrial middle atmosphere using a 1-D radiative-convective model with interactive neutral and ion chemistry driven by four different sets of daily spectral solar irradiance (SSI) available in the literature for the year 2000. Obtained daily time series of ozone, hydroxyl and electron densities are used to calculate their sensitivity to the short-term SSI variability at 205 nm. All applied SSI data sets possess 27-day solar rotation cycle; however, its amplitude and phase as well as the correlation between considered SSI time series differ among data sets leading to the different behavior of the atmospheric response. Contrary, the ozone and hydroxyl sensitivities to the SSI changes during solar rotation cycle are almost identical for all applied SSI data sets in the stratosphere. In the mesosphere, the difference in correlation between SSI in Herzberg continuum and Lyman-α line in considered SSI data sets leads to substantial scatter of the sensitivity estimates based on 205 nm. Our results show that for the sensitivity analysis in the stratosphere based on the SSI at 205 nm any considered SSI data sets can be applied. For the mesosphere, where the sensitivity strongly varies among applied SSI data sets more robust results can be obtained using the sensitivity calculations based on the SSI in Lyman-α line.     

中国南部对流层中上层臭氧增加的气象场判识及臭氧变化的多尺度特征

副热带急流对中国南部地区对流层中上层臭氧浓度的影响程度及地理范围目前还研究较少,且缺乏综合使用常规气象资料及卫星资料来判识对流层中上层臭氧浓度增高的方法.本文利用NCEP再分析与最终分析资料、日本GMS-5地球静止卫星水汽云图资料,以2001年3月27~29日中国南部的临安、昆明、香港臭氧探测个例为基础,结合1996年3月29日香港与2001年4月13日临安对流层中上层高浓度臭氧分布个例对副热带急流对中国南部对流层中上层臭氧浓度的影响进行了详细分析,提出根据气象要素场判识春季中国南部对流层中上层臭氧浓度增高的充分条件为根据卫星水汽图像上的暗区、高空急流入口区的左侧辐合区、高空锋区、对流层中上层≥1 PVU的向下伸展的舌状高位涡区来综合判断.本文的分析结果表明,本文个例中对流层中上层高浓度臭氧来自平流层;香港对流层中上层低浓度臭氧来自热带海洋地区.不仅臭氧垂直廓线的多个极小与极大值表明臭氧垂直分布的多尺度变化特征,而且对流层中上层PV分布以及卫星水汽图像分析也表明大气中的多尺度运动对臭氧垂直分布特征有显著影响.本文的结果表明与副热带高空急流相联系的平流层空气侵入不仅发生在中国大陆的较高纬度地区,较低纬度的昆明与香港地区也有平流层空气侵入导致对流层中上层臭氧浓度升高.     

Mid-latitude summer response of the middle atmosphere to short-term solar UV changes

Temperature and wind data obtained with Rayleigh lidar since 1979 and Russian rockets since 1964 are analyzed to deduce the summer response of the middle atmosphere to short-term solar UV changes. The equivalent width of the 1083 nm He I line is used as a proxy to monitor the short-term UV flux changes. Spectral analyses are performed on 108-day windows to extract the 27-day component from temperature, wind and solar data sets. Linear regressions between these spectral harmonics show some significant correlations around 45 km at mid-latitudes. For large 27-day solar cycles, amplitudes of 2 K and 6 m s⁻¹ are calculated for temperature data series over the south of France (44°N), and on wind data series over Volgograd (49°N), respectively. Cross-spectrum analyses have indicated correlations between these atmospheric parameters and the solar proxy with a phase lag of less than 2 days. These statistically correlative results, which provide good qualitative agreement with numerical simulations, are both obtained at mid-latitude. However, the observed amplitudes are larger than expected, with numerical models suggesting that dynamical processes such as equatorial or gravity waves may be responsible.     

Long-term changes of the upper stratosphere as seen by Japanese rocketsondes at Ryori (39°N, 141°E)

Wind and temperature profiles measured routinely by rockets at Ryori (Japan) since 1970 are analysed to quantify interannual changes that occur in the upper stratosphere. The analysis involved using a least square fitting of the data with a multiparametric adaptative model composed of a linear combination of some functions that represent the main expected climate forcing responses of the stratosphere. These functions are seasonal cycles, solar activity changes, stratospheric optical depth induced by volcanic aerosols, equatorial wind oscillations and a possible linear trend. Step functions are also included in the analyses to take into account instrumental changes. Results reveal a small change for wind data series above 45 km when new corrections were introduced to take into account instrumental changes. However, no significant change of the mean is noted for temperature even after sondes were improved. While wind series reveal no significant trends, a significant cooling of 2.0 to 2.5 K/decade is observed in the mid upper stratosphere using this analysis method. This cooling is more than double the cooling predicted by models by a factor of more than two. In winter, it may be noted that the amplitude of the atmospheric response is enhanced. This is probably caused by the larger ozone depletion and/or by some dynamical feedback effects. In winter, cooling tends to be smaller around 40–45 km (in fact a warming trend is observed in December) as already observed in other data sets and simulated by models. Although the winter response to volcanic aerosols is in good agreement with numerical simulations, the solar signature is of the opposite sign to that expected. This is not understood, but it has already been observed with other data sets.     

Trends in total ozone and the effect of the equatorial zonal wind QBO

Trends in total column ozone have been analyzed in terms of the equatorial zonal wind. We used zonal monthly mean total ozone from Total Ozone Mapping Spectrometer (TOMS) and monthly mean zonal wind in the equatorial stratosphere at 30 hPa to define the phases of the quasi-biennial oscillation (QBO). Total column ozone trends have been assessed during the period 1979–2004, for both Hemispheres, and for each month, under three conditions considering, all the ozone dataset, ozone values during easterly phase and ozone values during westerly phase of the QBO. When the whole dataset is considered, negative trends are observed. From low to midlatitudes a zonal pattern is noticed with increasing negative values toward higher latitudes. When the data is filtered according to the QBO phase, statistically significant positive trends appear in the westerly case during January to May at low latitudes .The trend pattern in the case of the easterly phase presents more negative values.     

Annual and semiannual oscillations of stratospheric ozone

The global structures of annual oscillation (AO) and semiannual oscillation (SAO) of stratospheric ozone are examined by applying spherical harmonic analysis to the ozone data obtained from the Nimbus-7 solar backscattered UV-radiation (SBUV) measurements for the period November 1978 to October 1980. Significant features of the results are: (1) while the stratospheric ozone AO is prevalent only in the polar regions, the ozone SAO prevails both in the equatorial and polar stratospheres; (2) the vertical distribution of the equatorial ozone SAO has a broad maximum of the order of 0.5 (mixing ratio in g/g) and the maximum appears earlier at high altitude (shifting from May [and November] at 0.3 mb [60 km] to November [and May] at 40 mb); (3) above the 40 km level, the maximum of the polar ozone SAO shifts upward towards later phase with altitude with a rate of approximately 10 km/month in both hemispheres; (4) vertical distributions of the polar ozone AOs and SAOs show two peaks in amplitude with a minimum (nodal layer) in between and a rapid phase change with altitude takes place in the respective nodal layers; and (5) the heights of the ozone AO- and SAO-peaks decrease with latitude. The main part of AOs and SAOs of stratospheric ozone including hemispheric asymmetries is ascribable to: (i) temperature dependent ozone photochemistry in the upper stratosphere and mesosphere, (ii) variations of radiation field in the lower stratosphere affected by the annual cycle of solar illumination and temperature in the upper stratosphere and (iii) meridional ozone transport by dynamical processes in the lower stratosphere.     

Stratospheric ozone response to a solar proton event: Hemispheric asymmetries

Ozone depression in the polar stratosphere during the energetic solar proton event on 4 August 1972 was observed by the backscattered ultraviolet (BUV) experiment on the Nimbus 4 satellite. Distinct asymmetries in the columnar ozone content, the amount of ozone depressions and their temporal variations above 4 mb level (38 km) were observed between the two hemispheres. The ozone destroying solar particles precipitate rather symmetrically into the two polar atmospheres due to the geomagnetic dipole field These asymmetries can be therefore ascribed to the differences mainly in dynamics and partly in the solar illumination and the vertical temperature structure between the summer and the winter polar atmospheres. The polar stratosphere is less disturbed and warmer in the summer hemisphere than the winter hemisphere since the propagation of planetary wave from the troposphere is inhibited by the wind system in the upper troposphere, and the air is heated by the prolonged solar insolation. Correspondingly, the temporal variations of stratospheric ozone depletion and its recovery appear to be smooth functions of time in the (northern) summer hemisphere and the undisturbed ozone amount is slighily, less than that of its counterpart. On the other hand, the tempotal variation of the upper stratospheric ozone in the winter polar atmosphere (southern hemisphere) indicates large amplitudes and irregularities due to the disturbances produced by upward propagating waves which prevail in the polar winter atmosphere. These characteristic differences between the two polar atmospheres are also evident in the vertical distributions of temperature and wind observed by balloons and rocker soundings.     

The effect of the 11-year solar cycle on the temperature in the lower stratosphere

Two temperature datasets are analyzed for quantifying the 11-year solar cycle effect in the lower stratosphere. The analysis is based on a regression linear model that takes into account volcanic, Arctic Oscillation (AO), Quasi-Biennial Oscillation (QBO) and El Nino Southern Oscillation (ENSO) effects. Under solar maximum conditions, temperatures are generally warmer for low- and mid-latitudes than under solar minimum, with the effect being the strongest in northern summer. At high latitudes, the vortex is generally stronger under solar maximum conditions, with the exception of February and to a lesser extent March in the Northern Hemisphere; associated with this positive signal at high latitudes, there is a significant negative signal at the equator. Observations also suggest that contrary to the beginning of the winter, in February–March, the residual circulation in the Northern Hemisphere is enhanced. A better understanding of the mechanisms at work comes from further investigations using the ERA-40 reanalysis dataset. First, a consistent response in terms of temperature and wind is obtained. Moreover, considering Eliassen-Palm (EP) flux divergence and residual circulation stream functions, we found an increased circulation in the Northern Hemisphere in February during solar maxima, which results in more adiabatic warming at high latitudes and more adiabatic cooling at low latitudes, thus demonstrating the dynamical origin of the response of the low stratosphere to the solar cycle.     

Ozone distribution in winter at high latitudes in the northern hemisphere

The ozone winter maximum at high latitudes in the northern hemisphere is not evenly distributed along the longitudes. This is mainly due to the upper air circulation, both horizontally and vertically. In addition it is also strongly influenced by the largest mountain ranges. During the last two decades the air circulation in the North Atlantic has intensified. This has led to ascending motion in the upper troposphere and the lower stratosphere, which in turn has resulted in a reduced total ozone column in Northwest Europe.The large mounter ranges in Asia are initiating standing waves, with descending motions in the atmosphere behind the mountains. The descending motion leads to adiabatic warming of the lower stratosphere and the upper troposphere. Ozone-rich air is transported downwards to lower levels and stored there, where the ozone is less affected by heterogeneous chemical destruction.     

Low ozone event at Madrid in November 1996

A sudden transient increase of the solar ultraviolet (UV) radiation was detected with a ground-based photometer in Madrid (Spain, 41°N, 3°W) on 25 November 1996 (Cordoba et al., 2000. UV-B irradiance at Madrid during 1996, 1997 and 1998. J. Geophys. Res. 105 (D4) (2000) 4903–4906). The data obtained by the TOMS satellite instrument revealed that this event was related to a reduction of the total ozone column values. This low ozone episode has been analysed. The ozone decrease was accompanied by a reduction of air temperature in the lower stratosphere. The anti-correlation between total ozone and air parcel height along the three-dimensional isentropic back-trajectories suggests that the adiabatic uplift of air contributed significantly to both the ozone and the temperature decreases observed. The uplift could be caused by the propagation into the lower stratosphere of the high-pressure cell located over the mid-Atlantic region.     

The signal of the 11-year solar cycle in the global stratosphere

The search for a signal of the 11-year sunspot cycle in the heights and temperatures of the lower stratosphere was previously successfully conducted for the northern hemisphere with a data set from the Freie Universität Berlin, covering four solar cycles. This work has been extended to the whole globe by means of the NCEP/NCAR reanalyses for the period 1968–1996. The re-analyses show that the signal exists in the southern hemisphere too, and that it is of nearly the same size and shape as on the northern hemisphere. The NCEP/NCAR reanalyses yield higher correlations with the solar cycle than do the Berlin analyses for the same period, because the interannual variability is lower in the NCEP/NCAR data.The correlations between the solar cycle and the zonally averaged temperatures at the standard levels between 200 and 10 hPa are largest between the tropopause and the 25 km level, that is, in the ozone layer. This may be partly a direct effect in this layer, because of more absorber (ozone) and more ultraviolet radiation from the sun in the peaks of the 11-year solar cycle. However, it is more likely to be mainly an indirect dynamical consequence of UV absorption by ozone in the middle and upper stratosphere.The largest temperature correlations move with the sun from one summer hemisphere to the other, and the largest height correlations move poleward from winter to summer.     

火山活动对北半球平流层气候异常变化的影响

文中利用逐次滤波法滤除北半球平流层70 hPa约15~22 km高空大气温度异常变化中太阳活动的影响之后,进一步分析了火山活动的气候效应,分析结果表明,火山活动能引起平流层较大幅度增温,对于北半球70hPa高空气候异常变化的影响超过了总方差的30%;火山活动影响最显著的高度是平流层70 hPa约15~22 km高空,由此高度向上或向下,火山活动的影响都逐渐减小;火山活动引起平流层大气升温的同时还将引起对流层大气降温,其分界线大致位于对流层顶300 hPa附近;强火山爆发如皮纳图博火山爆发、阿贡火山爆发和堪察加北楮缅奴等火山爆发是引起未来两年左右平流层中下层温度异常变化最重要的因素,其方差贡献率超过百分之五十三！;火山喷发高度越高,引起平流层增温效应的层次也越高;北半球大气温度异常变化对南半球火山活动响应的滞后时间比北半球火山活动长. 平流层高空气候异常变化还具有显著的22年变化周期,分析认为是大气温度场对太阳磁场磁性周期22年异常变化的响应,其方差贡献率超过9%.     

Solar cycle changes to planetary wave propagation and their influence on the middle atmosphere circulation

Recent observations suggest that there may be a causal relationship between solar activity and the strength of the winter Northern Hemisphere circulation in the stratosphere. A three-dimensional model of the atmosphere between 10–140 km was developed to assess the influence of solar minimum and solar maximum conditions on the propagation of planetary waves and the subsequent changes to the circulation of the stratosphere. Ultraviolet heating in the middle atmosphere was kept constant in order to emphasise the importance of non-linear dynamical coupling. A realistic thermo-sphere was achieved by relaxing the upper layers to the MSIS-90 empirical temperature model. In the summer hemisphere, strong radiative damping prevents significant dynamical coupling from taking place. Within the dynamically controlled winter hemisphere, small perturbations are reinforced over long periods of time, resulting in systematic changes to the stratospheric circulation. The winter vortex was significantly weakened during solar maximum and western phase of the quasi-biennial oscillation, in accordance with reported 30 mb geopotential height and total ozone measurements.     

Studies of variations in the vertical ozone profiles over India

The latitudinal and temporal variations in the vertical profiles of ozone over the Indian subcontinent are discussed. In the equatorial atmosphere represented by Trivandrum (8°N) and Poona (18°N), while tropospheric ozone shows marked seasonal variations, the basic pattern of the vertical distribution of ozone in the stratosphere remains practically unchanged throughout the year, with a maximum at about 28 to 26 km and a minimum just below the tropopause. The maximum total ozone occurs over Trivandrum in the summer monsoon season and the latitudinal anomaly observed over the Indian monsoon area at this time is explained as arising from the horizontal transport of ozone-rich stratospheric air from over the thermal equator to the southern regions.In the higher latitudes represented by New Delhi (28°N), the maximum occurs at 23 km. Delhi, which lies in the temperate regime in winter, shows marked day-to-day variations in association with western disturbances and the strong westerly jet stream that lies over north and central India at this time.Although the basic pattern of the vertical distribution of ozone in the equatorial atmosphere is generally the same in all seasons, significant though small changes occur in the lower stratosphere and in the troposphere. There are small perturbations in the ozone and temperature structures, distinct ozone maxima being always associated with temperature inversions. There are also large perturbances not related to temperature, ozone-depleted regions normally reflecting a stratification of either destructive processes or materials such as dust layers or clouds at these levels. Particularly interesting are the upper tropospheric levels just below the tropopause where the ozone concentration is consistently the smallest, in all seasons and at all places where soundings have been made in India.     

The 11-year solar-cycle effects on the temperature in the upper-stratosphere and mesosphere: Part I—Assessment of observations

Three independent temperature datasets have been analyzed for quantifying the influence of the 11-year solar cycle modulation of the UV radiation. The datasets used include: US rocketsondes, the OHP lidar, and the global temperature database made by the successive SSU on the NOAA satellites, adjusted and provided by the UK Meteorological Office. These measurements cover the upper stratosphere and the mesosphere, where the direct photochemical effect is expected. The improvement of the analysis compared to previous ones was possible because the overall quality and the continuity of many data series have been checked more carefully during the last decade in order to look for anthropogenic fingerprints and the one used here have been recognized as the best series according to their temporal continuity. The analysis of the different data set is based on the same regression linear model. The 11-year solar temperature response observed presents a variable behavior, depending on the location. However, an overall adequate agreement among the results has been obtained, and thus the global picture of the solar impact in the upper stratosphere and lower mesosphere has been obtained and is presented here. In the tropics, a 1–2 K positive response in the mid and upper stratophere has been found, in agreement with photochemical theory and previous analyses. On the opposite, at mid-latitudes, negative responses of several Kelvin have been observed, during winters, in the analyses of the datasets analyzed here. In the mesosphere, at sub-tropic and mid-latitude regions, we observe a positive response all the year round increasing by a factor of two during winter.     

Relationship between phases of quasi-decadal oscillations of total ozone and the 11-year solar cycle

Temporal variability of the relationship between the phases of quasi-decadal oscillations (QDOs) of total ozone (TO), measured at the Arosa station, and the Ri international sunspot number have been analyzed for the period of 1932–2009. Before the 1970s, the maximum phase of ozone QDOs lagged behind solar activity variations by about 2.5–2.8 years and later outstripped by about 1.5 years. We assumed that the TO QDOs in midlatitudes of the Northern Hemisphere were close to being in resonance with solar activity oscillations in the period from the mid-1960s to the mid-1970s and assessed the characteristic delay period of TO QDOs. The global distribution of phases and amplitudes of TO QDOs have been studied for the period from 1979 to 2008 based on satellite data. The maximum phase of TO QDOs first onsets in northern middle and high latitudes and coincides with the end of the growth phase of the 11-year solar cycle. In the tropics, the maximum oscillation phase lags behind by 0.5–1 year. The maximum phase lag near 40–50° S is about two years. The latitudinal variations of the phase of TO QDOs have been approximated.