Interplay between the mesoscopic Stoner and Kondo effects in quantum dots

We consider electrons confined to a quantum dot interacting antiferromagnetically with a spin-1 / 2 Kondo impurity. The electrons also interact among themselves ferromagnetically with a dimensionless coupling J , where J =1 denotes the bulk Stoner transition. We show that as J approaches 1 there is a regime with enhanced Kondo correlations, followed by one where the Kondo effect is destroyed and impurity is spin polarized opposite to the dot electrons. The most striking signature of the first, Stoner-enhanced Kondo regime is that a Zeeman field increases the Kondo scale, in contrast to the case for noninteracting dot electrons. Implications for experiments are discussed.     

Singlet-triplet transition in a quantum dot: effect on mesoscopic transport

The T=0 transport properties of a wire interacting with a lateral two-level quantum dot are studied by using an exact numerical calculation. The wire conductance, the spin–spin correlation and the Kondo temperature are obtained as a function of the dot level energy spacing. When the dot has two electrons and spin S_D1, the wire current is totally quenched by the S=1 Kondo effect. The Kondo temperature is maximum at the singlet–triplet transition and its dependence upon the dot energy spacing follows a non-universal scaling law.     

Effect of localized spins in coherent transport through quantum dots

The effect of localized spins on the quantum coherence in solids is discussed. A quantum dot with an odd number of electrons can be a model system for a localized spin. It is experimentally shown that a spin flip scattering by a quantum dot pulls the trigger of quantum decoherence. On the other hand, spin flip scattering is the basic process to construct the Kondo singlet state around a magnetic impurity. Through an interference effect of the Kondo state (the Fano–Kondo effect) in a side-coupled dot system, we show experimentally that the Kondo singlet state is quantum mechanically coherent. The analysis of the Fano–Kondo lineshape indicates the locking of the phase shift to π/2, which is in agreement with theoretical predictions. The Fano–Kondo effect is also observed in an Aharonov–Bohm ring, in which a quantum dot is embedded, and also indicates the phase shift locking to π/2.     

Dynamically induced Kondo effect in double quantum dots

A new mechanism of resonance Kondo tunneling via a composite quantum dot (QD) is proposed. It is shown that, owing to the hidden dynamic spin symmetry, the Kondo effect can be induced by a finite voltage eV applied to the contacts at an even number N of electrons in a QD with zero spin in the ground state. As an example, a double QD is considered in a parallel geometry with N=2, which possesses the SO(4) type symmetry characteristic of a singlet-triplet pair. In this system, the Kondo peak of conductance appears at an eV value compensating for the exchange splitting.     

Quantum dots with even number of electrons: kondo effect in a finite magnetic field

We show that the Kondo effect can be induced by an external magnetic field in quantum dots with an even number of electrons. If the Zeeman energy B is close to the single-particle level spacing Delta in the dot, the scattering of the conduction electrons from the dot is dominated by an anisotropic exchange interaction. A Kondo resonance then occurs despite the fact that B exceeds by far the Kondo temperature T(K). As a result, at low temperatures T相似文献   

Nonequilibrium Keldysh formalism for interacting leads—Application to quantum dot transport driven by spin bias

The conductance through a mesoscopic system of interacting electrons coupled to two adjacent leads is conventionally derived via the Keldysh nonequilibrium Green’s function technique, in the limit of noninteracting leads [Y. Meir, N.S. Wingreen, Phys. Rev. Lett. 68 (1992) 2512]. We extend the standard formalism to cater for a quantum dot system with Coulombic interactions between the quantum dot and the leads. The general current expression is obtained by considering the equation of motion of the time-ordered Green’s function of the system. The nonequilibrium effects of the interacting leads are then incorporated by determining the contour-ordered Green’s function over the Keldysh loop and applying Langreth’s theorem. The dot–lead interactions significantly increase the height of the Kondo peaks in density of states of the quantum dot. This translates into two Kondo peaks in the spin differential conductance when the magnitude of the spin bias equals that of the Zeeman splitting. There also exists a plateau in the charge differential conductance due to the combined effect of spin bias and the Zeeman splitting. The low-bias conductance plateau with sharp edges is also a characteristic of the Kondo effect. The conductance plateau disappears for the case of asymmetric dot–lead interaction.     

Spin filters with Fano dots

We compute the zero bias conductance of electrons through a single ballistic channel weakly coupled to a side quantum dot with Coulomb interaction. In contrast to the standard setup which is designed to measure the transport through the dot, the channel conductance reveals Coulomb blockade dips rather then peaks due to the Fano-like backscattering. At zero temperature the Kondo effect leads to the formation of broad valleys of small conductance corresponding to an odd number of electrons on the dot. By applying a magnetic field in the dot region we find two dips corresponding to a total suppression in the conductance of spins up and down separated by an energy of the order of the Coulomb interaction. This provides a possibility of a perfect spin filter.Received: 6 November 2003, Published online: 2 April 2004PACS: 72.15.Qm Scattering mechanisms and Kondo effect - 73.23.Ad Ballistic transport - 72.25.-b Spin polarized transport     

Controlled dephasing of a quantum dot in the Kondo regime

Kondo correlation in a spin polarized quantum dot (QD) results from the dynamical formation of a spin singlet between the dot's net spin and a Kondo cloud of electrons in the leads, leading to enhanced coherent transport through the QD. We demonstrate here significant dephasing of such transport by coupling the QD and its leads to potential fluctuations in a nearby "potential detector." The qualitative dephasing is similar to that of a QD in the Coulomb blockade regime in spite of the fact that the mechanism of transport is quite different. A much stronger than expected suppression of coherent transport is measured, suggesting that dephasing is induced mostly in the "Kondo cloud" of electrons within the leads and not in the QD.     

Mesoscopic Kondo screening effect in a single-electron transistor embedded in a metallic ring.

We study the Kondo screening effect generated by a single-electron transistor or quantum dot embedded in a small metallic ring. When the ring circumference L becomes comparable to the fundamental length scale xi(0)(K) = Planck's constant over upsilon(F)/T(0)(K) associated with the bulk Kondo temperature, the Kondo resonance is strongly affected, depending on the total number of electrons (mod4) and magnetic flux threading the ring. The resulting Kondo-assisted persistent currents are also calculated in both Kondo and mixed-valence regimes, and the maximum values are found in the crossover region.     

Tunable Kondo effect in a double quantum dot coupled to ferromagnetic contacts

We investigate the effects induced by ferromagnetic contacts attached to a serial double quantum dot. Spin polarization generates effective magnetic fields and suppresses the Kondo effect in each dot. The superexchange interaction J(AFM), tuned by the interdot tunneling rate t, can be used to compensate the effective fields and restore the Kondo resonance when the contact polarizations are aligned. As a consequence, the direction of the spin conductance can be controlled and even reversed using electrostatic gates alone. Our results demonstrate a new approach for controlling spin-dependent transport in carbon nanotube double dot devices.     

Transition between quantum states in a parallel-coupled double quantum dot

Strong electron and spin correlations in a double quantum dot (DQD) can give rise to different quantum states. We observe a continuous transition from a Kondo state exhibiting a single-peak Kondo resonance to another exhibiting a double peak by increasing the interdot coupling (t) in a parallel-coupled DQD. The transition into the double-peak state provides evidence for spin entanglement between the excess electrons on each dot. Toward the transition, the peak splitting merges and becomes substantially smaller than t because of strong Coulomb effects. Our device tunability bodes well for future quantum computation applications.     

Quantum transport across multilevel quantum dot

The conductance across a quantum dot can be influenced by levels localized in the dot and having little hybridization with the conduction channel. Fano lineshapes arising in resonant transmission measurements, imply interference between the localized and extended states. By applying a magnetic orthogonal field, the total spin of a quantum dot can be tuned. Electron correlations drive the dot through level crossings to higher spin states. Such crossings can give rise to Kondo conductance when the dot is at Coulomb blockade close to a magnetic field induced level degeneracy. In a previous work [P. Stefański, A. Tagliacozzo, B.R. Bulka, Phys. Rev. Lett. 93 (2004) 186805] we have shown that a Fano-like pattern also appears when the continuum of the conduction states originates from a broad Kondo resonance. A bunch of localized core levels, weakly coupled to the Kondo resonance, imprints the broad Kondo peak with Fano lineshapes. A signature of the presence of correlations in the quantum dot is discussed.     

Enhancement of kondo effect in quantum dots with an even number of electrons

We investigate the Kondo effect in a quantum dot with almost degenerate spin-singlet and triplet states for an even number of electrons. We show that the Kondo temperature as a function of the energy difference between the states Delta reaches its maximum around Delta = 0 and decreases with increasing Delta. The Kondo effect is thus enhanced by competition between singlet and triplet states. Our results explain recent experimental findings. We evaluate the linear conductance in the perturbative regime.     

Probing a Kondo-correlated quantum dot with spin spectroscopy

We investigate the Kondo effect and spin blockade observed in a many-electron quantum dot and study the magnetic field dependence. At lower fields, a pronounced Kondo effect is found, which is replaced by the spin blockade at higher fields. In an intermediate regime, both effects are visible. We make use of this combined effect to gain information about the internal spin configuration of our quantum dot. We find that the data cannot be explained assuming regular filling of electronic orbitals. Instead, spin polarized filling seems to be probable.     

Selective spin injection controlled by electrical way in ferromagnet/quantum dot/semiconductor system

Selective and large polarization of current injected into semiconductor (SC) is predicted in ferromagnet (FM)/quantum dot (QD)/SC system by varying the gate voltage above the Kondo temperature. In addition, spin-dependent Kondo effect is also revealed below Kondo temperature. It is found that Kondo resonances for up spin state are suppressed with increasing of the polarization P of the FM lead. While the down one is enhanced. The Kondo peak for up spin is disappear at P=1.     

Multipeak Kondo effect in one- and two-electron quantum dots

We have fabricated a few-electron quantum dot that can be tuned down to zero electrons while maintaining strong coupling to the leads. Using a nearby quantum point contact as a charge sensor, we can determine the absolute number of electrons in the quantum dot. We find several sharp peaks in the differential conductance, occurring at both zero and finite source-drain bias, for the one- and two-electron quantum dot. We attribute the peaks at finite bias to a Kondo effect through excited states of the quantum dot and investigate the magnetic field dependence of these Kondo resonances.     

Spin-resolved splitting of Kondo resonances in the presence of RKKY-type coupling

We have performed spin-resolved measurements on a Kondo impurity in the presence of RKKY-type exchange coupling. By placing manganese phthalocyanine (MnPc) molecules on Fe-supported Pb islands, a Kondo system is devised which is exchange coupled to a magnetic substrate via conduction electrons in Pb, inducing spin splitting of the Kondo resonance. The spin-polarized nature of the split Kondo resonance and a spin filter effect induced by spin-flip inelastic electron tunneling are revealed by spin-polarized scanning tunneling microscopy and spectroscopy.     

Out-of-equilibrium Kondo effect in a mesoscopic device

We study the nonequilibrium regime of the Kondo effect in a quantum dot laterally coupled to a narrow wire. We observe a split Kondo resonance when a finite bias voltage is imposed across the wire. The splitting is attributed to the creation of a double-step Fermi distribution function in the wire. Kondo correlations are strongly suppressed when the voltage across the wire exceeds the Kondo temperature. A perpendicular magnetic field enables us to selectively control the coupling between the dot and the two Fermi seas in the wire. Already at fields of order 0.1 T only the Kondo resonance associated with the strongly coupled reservoir survives.     

Kondo Resonance Splitting in a Quantum Dot with Perpendicular Magnetic Fields

Using the nonequilibrium Green＇s function technique, we investigate the Kondo effect in the quantum dot with perpendicular magnetic fields, in which one is the Zeeman splitting lies in the z-direction and the other is the spin flip points at the x-direction. It is found whatever one or two magnetic fields are applied, the local density of states （LDOS） will split into two peaks. The positions of two Kondo resonance peaks are determined by Zeeman energy △ when J = 0, and by √△^2＋J^2 when J≠0.     

Screening and interaction of magnetic impurities in Luttinger liquids

The spin and charge correlations induced in the conduction electron sea by the presence of a spin-1=2 magnetic impurity are investigated for one-dimensional electrons. For correlated conduction electrons, the RKKY interaction between magnetic impurities exhibits only a slow algebraic decay with distance. Increasing the exchange coupling between conduction electrons and magnetic impurity leads to a competition between the RKKY interaction and the Kondo effect. For a two-impurity model, we study the influence of the electronic correlations on this competition. Furthermore, the Kondo screening cloud and the local spin susceptibility far away from a magnetic impurity are discussed.