Design of plasmonic nanoantennae for enhancing spontaneous emission

We apply two- and three-dimensional numerical calculations to study optical nanoantennae made of two coupled gold nanostructures, enclosing a single emitter in their gap. We show that, using structures manufacturable with today's nanotechnology, it is possible to increase the radiative decay rate by three orders of magnitude while keeping a quantum efficiency larger than 80% in the near-infrared regime. We examine the competition between the radiative and nonradiative processes in the presence of the antennae as a function of wavelength and antenna geometry. Our results hold great promise for improving the quantum efficiency of poor emitters such as silicon nanocrystals or carbon nanotubes.     

Radiative and non-radiative decay of a single molecule close to a metallic nanoparticle

We study the spontaneous emission of a single emitter close to a metallic nanoparticle, with the aim to clarify the distance dependence of the radiative and non-radiative decay rates. We derive analytical formulas based on a dipole-dipole model, and show that the non-radiative decay rate follows a R⁻⁶ dependence at short distance, where R is the distance between the emitter and the center of the nanoparticle, as in Förster’s energy transfer. The distance dependence of the radiative decay rate is more subtle. It is chiefly dominated by a R⁻³ dependence, a R⁻⁶ dependence being visible at plasmon resonance. The latter is a consequence of radiative damping in the effective dipole polarizability of the nanoparticle. The different distance behavior of the radiative and non-radiative decay rates implies that the apparent quantum yield always vanishes at short distance. Moreover, non-radiative decay is strongly enhanced when the emitter radiates at the plasmon-resonance frequency of the nanoparticle.     

Fabry–Perot effect on dimer nanoantennas

In this work, we investigate the interaction between a single quantum emitter and dimer nanoantennas through a Fabry–Perot structure composed of an appropriate combination of two dielectric layers. This type of dielectric configuration is well known in the microwave region to increase the antenna performance, such as directivity, radiation efficiency, and radiation resistance. Here, the Fabry–Perot concept is transposed to the optical domain. The single emitter couples to the antenna through the dielectric structure, giving rise to a wide aperture field on top of the dielectrics with the same polarization of the emitter. This purely polarized aperture field can be used to excite one or more conveniently spaced nanoantennas. We demonstrate by 3D numerical calculations that the directivity and excitation rate of a single dimer is highly increased. Also, we show that multiple dimers arranged in an array configuration can be enhanced due to the wide aperture field generated by a single emitter.     

Crucial role of the emitter-particle distance on the directivity of optical antennas

We demonstrate that the reflecting properties of a single particle nanoantenna can be extremely sensitive to its distance from a quantum emitter at frequencies lower than the plasmon resonance. The phenomenon is shown to arise from rapid phase variations of the emitter field at short distances associated with a phase of the antenna particle polarizability lower than π/4.     

Non-radiative decay of a dipole emitter close to a metallic nanoparticle: Importance of higher-order multipole contributions

The contribution of higher-order multipoles to radiative and non-radiative decay of a single dipole emitter close to a spherical metallic nanoparticle is re-examined. Taking a Ag spherical nanoparticle (AgNP) with the radius of 5 nm as an example, a significant contribution (between 50% and 101% of the total value) of higher-order multipoles to non-radiative rates is found even at the emitter distance of 5 nm from the AgNP surface. On the other hand, the higher-order multipole contribution to radiative rates is negligible. Consequently, a dipole-dipole approximation can yield only an upper bound on the apparent quantum yield. In contrast, the non-radiative rates calculated with the quasistatic Gersten and Nitzan method are found to be in much better agreement with exact electrodynamic results. Finally, the size corrected metal dielectric function is shown to decrease the non-radiative rates near the dipolar surface plasmon resonance.     

Single quantum dot coupled to a scanning optical antenna: a tunable superemitter

The interaction of a single quantum dot with a bowtie antenna is demonstrated for visible light. The antenna is generated at the apex of a Si3N4 atomic force microscopy tip by focused ion beam milling. When scanned over the quantum dot, its photoluminescence is enhanced while its excited-state lifetime is decreased. Our observations demonstrate that the relaxation channels of a single quantum emitter can be controlled by coupling to an efficiently radiating metallic nanoantenna.     

Triggered single photons and entangled photons from a quantum dot microcavity

Current quantum cryptography systems are limited by the attenuated coherent pulses they use as light sources: a security loophole is opened up by the possibility of multiple-photon pulses. By replacing the source with a single-photon emitter, transmission rates of secure information can be improved. We have investigated the use of single self-assembled InAs/GaAs quantum dots as such single-photon sources, and have seen a tenfold reduction in the multi-photon probability as compared to Poissonian pulses. An extension of our experiment should also allow for the generation of triggered, polarization-entangled photon pairs. The utility of these light sources is currently limited by the low efficiency with which photons are collected. However, by fabricating an optical microcavity containing a single quantum dot, the spontaneous emission rate into a single mode can be enhanced. Using this method, we have seen 78% coupling of single-dot radiation into a single cavity resonance. The enhanced spontaneous decay should also allow for higher photon pulse rates, up to about 3 GHz. Received 8 July 2001 and Received in final form 25 August 2001     

Scanning emitter lifetime imaging microscopy for spontaneous emission control

We report an experimental technique to map and exploit the local density of optical states of arbitrary planar nanophotonic structures. The method relies on positioning a spontaneous emitter attached to a scanning probe deterministically and reversibly with respect to its photonic environment while measuring its lifetime. We demonstrate the method by imaging the enhancement of the local density of optical states around metal nanowires. By nanopositioning, the decay rate of a pointlike source of fluorescence can be reversibly and repeatedly changed by a factor of 2 by coupling it to the guided plasmonic mode of the wire.     

Semileptonic decays of heavy quarks in quantum chromodynamics

We investigate the semileptonic decays of heavy quarks in the leading non-trivial order in quantum chromodynamics. Effects of gluon corrections and the initial quark Fermi motion on the semileptonic rates and decay distributions are calculated. The resulting lepton energy spectrum for the charm semileptonic decay is compared with data to extract the mass of the charm quark. This is combined with the semileptonic branching ratio to predict the charm-quark lifetime. We find the lepton energy spectrum very stable with respect to gluon corrections. Expected spectra from the semileptonic decays of bottom and top quarks are presented. We also study the semileptonic decay process Q → q?v_? + G, involving the emission of a single hard non-collinear gluon. This process should be observable with a branching ratio of a few percent in the decays of top (and heavier) quarks.     

Circularly polarized unidirectional emission via a coupled plasmonic spiral antenna

In this Letter, we study the emission properties of an electric dipole emitter coupled to a plasmonic spiral structure. The plasmonic spiral structure functions as an optical antenna, coupling the electric dipole emission into circularly polarized unidirectional emission in the far field. Increasing number of turns of the spiral leads to narrower angular width of the emission pattern in the far field. For a spiral antenna with six turns, antenna directivity of 23.5 dB with a directional emission into a narrow angular cone of 4.3° can be achieved. The emitted photons carry spin that is essentially determined by the handedness of the spiral antenna. By reversing the spiral, one can switch the polarization of the emission field between left-hand and right-hand circular polarizations. The spiral antenna may be used as a nanoscale circular polarization source in single molecule sensing, single-photo sources, and integrated photonic circuits.     

Hidden Vacuum Rabi Oscillations:Dynamical Quantum Superpositions of On/Off Interaction between a Single Quantum Dot and a Microcavity

We show that it is possible to realize quantum superpositions of switched-on and-off strong light-matter interaction in a single quantum dot-semiconductor microcavity system.Such superpositions enable the observation of counterintuitive quantum conditional dynamics effects.Situations are possible where cavity photons as well as the emitter luminescence display exponential decay but their joint detection probability exhibits vacuum Rabi oscillations.Remarkably,these quantum correlations are also present in the nonequilibrium steady state spectra of such coherently driven dissipative quantum systems.     

Single photon absorption by a single quantum emitter

We show that a three-level lambda quantum emitter with equal spontaneous emission rates on both optically active transitions can absorb an incident single-photon pulse with a probability approaching unity, provided that the focused light profile matches that of the emitter dipole emission. Even with realistic focusing geometries, our results could find applications in long-distance entanglement of spin qubits.     

Enhancement or quenching effect of metallic nanodimer on spontaneous emission

The plasmonic effects of a metallic (Au or Ag) nanodimer on the excitation and emission of a single emitter placed within the gap of the nanodimer are studied to identify its overall performance (enhancement or quenching) for the spontaneous emission. The process of a spontaneous emission is divided into two stages for analysis: the excitation and the subsequent emission stages. For the excitation stage, the amplification of the local electric field around the gap region is studied to show the converging-lens effect of the nanodimer for focusing an incident light. For the emission stage, the apparent quantum yield of an electric dipole (the excited emitter) in the presence of the nanodimer is studied in terms of its radiative and nonradiative decay rates. Both models are simulated by the multiple multi-pole methods for solving Maxwell's equations. The results indicate that the overall enhancement factor of a metallic nanodimer on the spontaneous emission depends not only on its dimension (radius and gap) but also on the absorption and emission spectra of the emitter. Moreover, there is an optimal dimension (radius and gap) of a nanodimer for obtaining the maximum enhancement to a specific spontaneous emission. In addition, the observed emission spectrum of the emitter can be modified by the nearby nanodimer (a low-pass filter), and its lifetime can be reduced by two or three orders of magnitude due to the energy transfer between them.     

First direct observation of two protons in the decay of 45Fe with a time-projection chamber

The decay of the ground-state two-proton emitter 45Fe was studied with a time-projection chamber and the emission of two protons was unambiguously identified. The total decay energy and the half-life measured in this work agree with the results from previous experiments. The present result constitutes the first direct observation of the individual protons in the two-proton decay of a long-lived ground-state emitter. In parallel, we identified for the first time directly two-proton emission from 43Cr, a known beta-delayed two-proton emitter. The technique developed in the present work opens the way to a detailed study of the mechanism of ground state as well as beta-delayed two-proton radioactivity.     

Entanglement and teleportation via a chaotic system

The dynamics of an entangled state interacting with a single cavity mode is investigated in the presence of a random parameter. We show that the degree of entanglement decays with time and that the rate of decay is defined by features of a random parameter. Quantum teleportation through a dissipative channel and teleportation fidelity as a function of damping rates have been studied. The sensitivity of the fidelity with respect to the random parameter is discussed. We have evaluated the time interval during which one can perform quantum teleportation and send the information with reasonable fidelity for given values of the correlation length of the random parameter.     

Impacts of pH and molecular structure on ultrasonic degradation of azo dyes

Sonochemical bleaching of monoazo dyes was investigated by irradiating 30 microM solutions of two "aryl-azo-naphthol" type model dyes in acidic, neutral and basic conditions using a 300 kHz emitter. It was found that the rate of bleaching in all cases was first order with respect to the maximum absorption of the dye in the visible band, and accelerated with increased acidity. The inhibition observed at alkaline conditions was attributed to the formation of anionic dye structures and their competition with the dye and its intermediate oxidation products for hydroxyl radicals, which are the major precursors of azo dye oxidation in sonicated water. Decolorization of the dyes was also related to the size of the molecule and the type or position of substituents about azo bonds. Comparison of color decay rates at similar conditions showed that the dye with a simple structure, low molecular mass and one ortho-substituent (hydroxyl) about the azo bond bleached considerably faster than the one having a more complicated structure (higher mass) and an additional o-substituent to the azo bond other than the OH group.     

Controlled plasmon-enhanced fluorescence by spherical microcavity

A surrounding electromagnetic environment can engineer spontaneous emissions from quantum emitters through the Purcell effect. For instance, a plasmonic antenna can efficiently confine an electromagnetic field and enhance the fluorescent process. In this study, we demonstrate that a photonic microcavity can modulate plasmon-enhanced fluorescence by engineering the local electromagnetic environment. Consequently, we constructed a plasmon-enhanced emitter (PE-emitter), which comprised a nanorod and a nanodiamond, using the nanomanipulation technique. Furthermore, we controlled a polystyrene sphere approaching the PE-emitter and investigated in situ the associated fluorescent spectrum and lifetime. The emission of PE-emitter can be enhanced resonantly at the photonic modes as compared to that within the free spectral range. The spectral shape modulated by photonic modes is independent of the separation between the PS sphere and PE-emitter. The band integral of the fluorescence decay rate can be enhanced or suppressed after the PS sphere couples to the PE-emitters, depending on the coupling strength between the plasmonic antenna and the photonic cavity. These findings can be utilized in sensing and imaging applications.     

Coupling interaction between a single emitter and the propagating surface plasmon polaritons in a graphene microribbon waveguide

The coupling interaction between an individual optical emitter and the propagating surface plasmon polaritons in a graphene microribbon （GMR） waveguide is investigated by numerical calculations, where the emitter is situated above the GMR or in the same plane of the GMR, The results reveal a multimode coupling mechanism for the strong interaction between the emitter and the propagating plasmonic waves in graphene. When the emitter is situated in the same plane of the GMR, the decay rate from the emitter to the surface plasmon polaritons increases more than 10 times compared with that in the case with the emitter above the GMR.     

Subwavelength localization of near fields in coupled metallic spheres for single-emitter polarization analysis

We numerically demonstrate selective near-field localization determined by the polarization state of a single emitter coupled to a plasmonic nanocluster. Seven gold nanospheres are carefully arranged such that up to 10 polarization states of the single emitter, including linear, circular, and elliptical polarizations, can be distinguished via the distinct field localization in four gaps. The ability to transform polarization states into field spatial localizations may find application in single emitter polarization analysis.     

功率晶体管的发射极设计

本文讨论功率晶体管设计中设计发射极时所需考虑的两个问题。一个是在给定的注入条件下如何保证足够大的电流放大;另一个是如何提高发射极发射电流的有效面积。文中着重分析在各种注入条件下发射结面上发射极电流密度的分布,亦即所谓基区电阻自偏压截止效应,最后给出主要结论。