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Recent progress of the optoelectronic properties of 2D Ruddlesden-Popper perovskites
Authors:Haizhen Wang  Chen Fang  Hongmei Luo  Dehui Li
Affiliation:School of Optical and Electronic Information and Wuhan National Laboratory for Optoelectronics;Department of Chemical and Materials Engineering
Abstract:Two-dimensional(2 D) hybrid organic-inorganic perovskites have recently attracted attention due to their layered nature, naturally formed quantum well structure, large exciton binding energy and especially better long-term environmental stability compared with their three-dimensional(3 D) counterparts. In this report, we present a brief overview of the recent progress of the optoelectronic applications in 2 D perovskites. The layer number dependent physical properties of 2 D perovskites will first be introduced and then the different synthetic approaches to achieve 2 D perovskites with different morphologies will be discussed. The optical, optoelectronic properties and self-trapped states in 2 D perovskites will be described, which are indispensable for designing the new device structures with novel functionalities and improving the device performance. Subsequently, a brief summary of the advantages and the current research status of the 2 D perovskite-based heterostructures will be illustrated.Finally, a perspective of 2 D perovskite materials is given toward their material synthesis and novel device applications.
Keywords:2D perovskite  optoelectronics  self-trapped exciton  heterostructures
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