Boson peak in low-frequency Raman spectra of polymethylmethacrylate |
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Authors: | M A Korshunov V F Shabanov |
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Affiliation: | 1.Kirenskii Institute of Physics, Siberian Branch,Russian Academy of Sciences,Krasnoyarsk,Russia;2.Krasnoyarsk Scientific Center,Krasnoyarsk,Russia |
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Abstract: | The role of the local field, anharmonicity, and degree of disorder in the formation of the boson peak has been studied. The low-frequency Raman spectrum of a model polymethylmethacrylate crystal with disorder elements was calculated using the method of atom-atom potentials taking into account the effect of local fields on the spectrum. The calculations were carried out for a crystal containing rigid molecules of an isotactic polymethylmethacrylate oligomer and for a structure with flexible molecules. |
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