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气体裂变产物88Kr半衰期测量
引用本文:杨志红,丁有钱,张生栋,杨磊,孙宏清,马鹏.气体裂变产物88Kr半衰期测量[J].原子能科学技术,2020,54(10):1737-1744.
作者姓名:杨志红  丁有钱  张生栋  杨磊  孙宏清  马鹏
作者单位:中国原子能科学研究院,北京102413
摘    要:为准确测定气体裂变产物88Kr的半衰期,本工作从辐照铀靶中分离得到3个放化纯的88Kr气体测量源。以85Kr作内标监督源,137Cs或57Co作外标监督源,使用多个HPGe探测器分别采用单探测器位置接力法和双探测器位置接力法跟踪测量88Kr 196.3 keV能量的特征γ射线,跟踪时间均在8个半衰期以上,以获得其半衰期数据。对3次独立测量数据用多种方法进行处理,最终得到88Kr半衰期测定结果为(2.796±0.015) h。

关 键 词:88Kr" target="_blank">88Kr')">88Kr    半衰期    放化分离    位置接力法

Half-life Determination of Gaseous Fission Product 88Kr
YANG Zhihong,DING Youqian,ZHANG Shengdong,YANG Lei,SUN Hongqing,MA Peng.Half-life Determination of Gaseous Fission Product 88Kr[J].Atomic Energy Science and Technology,2020,54(10):1737-1744.
Authors:YANG Zhihong  DING Youqian  ZHANG Shengdong  YANG Lei  SUN Hongqing  MA Peng
Affiliation:China Institute of Atomic Energy, Beijing 102413, China
Abstract:To determine the half-life of gaseous fission product 88Kr accurately, three purified 88Kr sources were prepared from irradiated uranium targets by using a radiochemical separation process. With 85Kr as the internal monitor, 137Cs/57Co as the external label sources, both single detector position relay method and double detectors position relay method were applied to track the characteristic 196.3 keV gamma rays by multiple high purity germanium detectors covering more than eight times half-lives. The results from three separate determinations were discussed, and a half-life of (2.796±0.015) h for 88Kr was presented.
Keywords:88Kr" target="_blank">88Kr')">88Kr                                                                                                                        half-life                                                                                                                        radiochemical separation                                                                                                                        position relay method
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