Fission gas induced swelling in uranium at high temperatures and pressures

The effect of externally applied hydrostatic pressures from 0–1000 bar at 900 °C on the fission gas induced swelling in uranium has been studied. The swelling is a sensitive function of pressures below 110 bar and relatively insensitive to pressures above 110 bar. Metallography of the samples show that the average diameter of the bubbles is reduced from 3300 to 1800 Å and the total number increased from 0.9 to 4.2 × 10¹²/cm³ as the annealing pressure is increased from 0–110 bar respectively. Further increases in pressure from 110–1000 bar have little effect on the average bubble size and density. The mechanism of pressure reduced swelling is discussed in terms of the equilibrium number of vacancies that can be associated with fission gas atoms under stress. It is also shown, both experimentally and theoretically, that there is a loss of surface area when bubbles coalesce under pressure.