On the background level of Tc, Sr and Cs in the North Atlantic

Mean concentrations of the anthropogenic radioactive oceanographic tracers ⁹⁹Tc, ⁹⁰Sr and ¹³⁷Cs have been measured as 0.005, 1.6 and 2.5 Bq m⁻³ in oceanic Northeast Atlantic surface water, east and northeast of the Azores, in 1992. This is, apparently, the first published value for fallout “background” ⁹⁹Tc in oceanic Atlantic water.Comparison with older data indicates an observed half life for ⁹⁰Sr and ¹³⁷Cs in the northeast Atlantic surface water of 20 yr corresponding to a mean residence time of 80–100 yr for the stable elements.The observed ⁹⁹Tc/⁹⁰Sr ratio (3 × 10⁻³) in the Azores samples is 10 times higher than the theoretical fission yield decay corrected to 1992. This is in agreement with published data on rain water samples and may be characteristic for 1960's global fallout. Furthermore, the measured ¹³⁷Cs/⁹⁰Sr ratio is not significantly different from that observed for global fallout. There do not appear to be any additional significant sources of artificial radionuclides in this region.     

The distribution of artificial radionuclides in the English Channel, southern North Sea, Skagerrak and Kattegat, 1990–1993

This paper presents the initial results concerning the distribution of artificial radionuclides from research cruises conducted in collaboration by three European institutes as part of an EEC MAST research project. Ten cruises were undertaken covering the English Channel, southern and eastern North Sea, Skagerrak and Kattegat over a period of 2.5 yr. A large number of analyses of four artificial radionuclides (¹³⁷Cs, ⁹⁹Tc, ¹²⁵Sb, ⁹⁰Sr), which behave conservatively in seawater, provided information about the general distribution of water masses and circulation patterns as well as about single transport events in the study area. Controlled liquid releases from the La Hague nuclear fuel reprocessing plant are transported eastwards, forming a characteristic distribution pattern in the Channel and the southern North Sea. This includes a near-coastal “plume” and a distinct boundary between waters contaminated predominantly by La Hague and by Sellafield. Spatial and temporal distributions of radionuclide ratios were used, for the first time, to calculate transit times from the English Channel to the coast of Jutland. The data published herein provide an essential input to the calibration of numerical models simulating water transport processes. The results demonstrate the continuing usefulness of artificial radionuclides as oceanographic tracers, even at the very low concentrations observed at present in north-west European Shelf waters.