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1.
Kedong Xia Shuoshuo Yu Yunling Li Huijuan Han Lingyao Duan Zhenyu Hou Xiao Liu 《Journal of the European Ceramic Society》2021,41(4):2375-2385
In this study, C/SiOC and C/SiO2 composites were prepared by using carbonaceous microspheres with different surface functional groups. Carbonaceous microspheres based on hydrothermal reaction of glucose contains hydroxyl group, while the surface carboxyl group increases after NaOH etching. The hydroxyl group increases the oxygen-enriched structural units of SiOC ceramics, and the C spheres are closely enwrapped in SiOC matrix after pyrolysis at 900 °C. However, the interfacial reaction of surface carboxyl with Si–OH results in the formation of cristobalite SiO2, and C spheres are not only encased inside the SiOC matrix, but also dispersed outside of SiOC ceramics. After removal of C via calcination at 500 °C for 5 h, C/SiOC and C/SiO2 composites are transformed into amorphous SiO2 and cristobalite SiO2, respectively. The thermogravimetric analysis indicates the oxidation resistance of SiOC is superior to that of C and SiO2. 相似文献
2.
Ying Zhang Jian Chen Yixing Cai Qingfeng Zhang Yinmei Lu Haitao Huang Yunbin He 《Journal of the American Ceramic Society》2021,104(2):928-935
Traditional self-powered ultraviolet photodetectors, which are usually designed based on p-n junction interfacial effects, exhibit low responsivity and specific detectivity because the photogenerated electrons and holes cannot be separated effectively. Unlike wide band-gap semiconductor materials, ferroelectrics have large remnant polarization and thus high depolarization electric field throughout the whole bulk region, which can cause effective separation of photogenerated electrons and holes. Based on this, in this study, we prepare Pb0.93La0.07(Zr1-xTix)0.9825O3 (PLZT) ferroelectric thin films with large remnant polarization and self-powered ultraviolet photodetectors with Au/PLZT/FTO structure. The results indicate that the photoelectric response performances of the detectors improve as the remnant polarization of the PLZT thin film and positive poling voltage increase. By adjusting the Ti content, due to large remnant polarization of 47.4 μC/cm2 in the PLZT thin films with 80 mol% Ti, the corresponding photodetector exhibits the best self-powered ultraviolet photoelectric response with the high photo/dark current ratio of 2600, responsivity of 2.05 mA/W, specific detectivity of 5.45 × 1010 Jones, and fast response speed (rise time of 18 ms). These values are superior to those of recently reported self-powered ultraviolet photodetectors. 相似文献
3.
在非均匀杂波和密集目标环境下,由于没有足够的独立同分布(IID)训练样本,传统空时自适应处理(STAP)方法的杂波抑制性能严重下降。针对以上问题,该文提出一种对阵元误差稳健的机载面阵雷达非均匀杂波抑制方法。该方法首先根据雷达系统参数先验知识构造杂波表示基矩阵。然后在考虑阵元误差的情况下,基于最小二乘准则迭代地估计杂波表示系数和阵元误差,最后利用估计得到的最优杂波表示系数和阵元误差直接在阵元脉冲域进行杂波对消。该方法无须估计待检测单元统计特性;没有孔径损失;不需要训练样本;即使在距离模糊情况下也能有效地抑制密集目标环境下机载面阵雷达回波数据中的非均匀杂波。仿真结果验证了该文方法的有效性。 相似文献
4.
5.
Mengying Ma Haoran Cai Chenlu Xu Renzhi Huang Shurong Wang Huilin Pan Yong-Sheng Hu 《Advanced functional materials》2021,31(25):2100278
Engineering the structure and chemistry of solid electrolyte interface (SEI) on electrode materials is crucial for rechargeable batteries. Using hard carbon (HC) as a platform material, a correlation between Na+ storage performance, and the properties of SEI is comprehensively explored. It is found that a “good” SEI layer on HC may not be directly associated with certain kinds of SEI components, such as NaF and Na2O. Whereas, arranging nano SEI components with refined structures constructs the foundation of “good” SEI that enables fast Na+ storage and interface stability of HC in Na-ion batteries. A layer-by-layer SEI on HC with inorganic-rich inner layer and tolerant organic-rich outer flexible layer can facilitate excellent rate and cycling life. Besides, SEI layer as the gate for Na+ from electrolyte to HC electrode can modulate interfacial crystallographic structures of HC with pillar-solvent that function as “pseudo-SEI” for fast and stable Na+ storage in optimal 1 m NaPF6-TEGDME electrolytes. Such a layer-by-layer SEI combined with a “pseudo-SEI” layer for HC enables an outstanding rate of 192 mAh g−1 at 2 C and stable cycling over 1100 cycles at 0.5 C. This study provides valuable guidance to improve the electrochemical performance of electrode materials through regulation of SEI in optimal electrolytes. 相似文献
6.
针对复杂背景下因像素点噪声及高亮边缘干扰导致的对红外弱小目标检测率低、虚警率高的问题,提出一种基于局部
积加权对比的红外弱小目标检测算法。 首先,分别计算目标区域与背景区域均值,并得到目标与局部背景的差异性;提出一种
局部积加权方法,极大增强了小目标的显著性与抑制背景杂波的能力;其次,采用多尺度算法增强算法的自适应能力;最后,对
显著性图像进行自适应阈值分割,得到待检测的真实目标。 仿真实验结果表明,所提算法的信杂比增益( SCRg)和背景抑制因
子(BSF)相比现有算法均有一定提升,在复杂背景及强噪声干扰下仍具有良好的准确性和鲁棒性,实现了提高检测率,降低虚
警率的目的。 相似文献
7.
Wei Guan Dong Yuan Juntao Wu Xiaobo Zhou Hong Zhao Fei Guo Lianjie Zhang Ke Zhou Wei Ma Wanzhu Cai Junwu Chen Liming Ding Lintao Hou 《半导体学报》2021,42(3):17-20
Organic solar cell(OSC)has attracted great interests due to its potential applications[1-9].To date,18%power conversion efficiency(PCE)has been achieved in single-junction OSC[10?13],indicating the feasibility of commercialization.This photovoltaic technology currently faces the performance gap between laboratory cells and large-area modules. 相似文献
8.
针对新能源汽车电机壳体压铸件产生粘模缺陷的问题,从模具结构设计、3D打印嵌件平衡模具温度,防止高温铝液破坏模具表面致密层等方面,在生产过程中对新能源电机壳体压铸件粘模缺陷进行改善,提出了应用3D打印嵌件的解决方案。 相似文献
9.
基于某款缸内直喷柴油发动机,将2-甲基呋喃(MF)分别与生物柴油,柴油燃料混合,研究不同燃料的热效率与?效率.试验结果表明,柴油-MF混合燃料随着MF质量分数的增加,热效率与?效率先增加后减小,热效率在纯柴油90%负荷工作时取得最大值为41.2%,?效率在MF质量比例为20%的混合燃料70%负荷工作时取得最大值为38.64%.而在生物柴油-MF混合燃料中,随着MF质量分数的增加,混合燃料的热效率与?效率一直减小,其排气气体的能量效率与?效率反而增加.在掺混同等低质量分数(10%)的MF下,生物柴油混合燃料比柴油混合燃料具有更高的热效率和?效率,而在掺混同等较高质量分数的MF(30%)下,生物柴油混合燃料的热效率和?效率比柴油混合燃料低. 相似文献
10.
Zhuolong Tu Mi Chen Min Wang Zhenxuan Shao Xiaoqi Jiang Kangyan Wang Zhe Yao Shiwei Yang Xingxing Zhang Weiyang Gao Cai Lin Bo Lei Cong Mao 《Advanced functional materials》2021,31(30):2100924
Diabetic wound healing still faces great challenges due to the excessive inflammation, easy infection, and impaired angiogenesis in wound beds. The immunoregulation of macrophages polarization toward M2 phenotype that facilitates the transition from inflammation to proliferation phase has been proved to be an effective way to improve diabetic wound healing. Herein, an M2 phenotype-enabled anti-inflammatory, antioxidant, and antibacterial conductive hydrogel scaffolds (GDFE) for producing rapid angiogenesis and diabetic wound repair are reported. The GDFE scaffolds are fabricated facilely through the dynamic crosslinking between polypeptide and polydopamine and graphene oxide. The GDFE scaffolds possess thermosensitivity, self-healing behavior, injectability, broad-spectrum antibacterial activity, antioxidant and anti-inflammatory ability, and electronic conductivity. GDFE effectively activates the polarization of macrophages toward M2 phenotype and significantly promotes the proliferation of dermal fibroblasts, the migration, and in vitro angiogenesis of endothelial cells through paracrine mechanisms. The in vivo results from a full-thickness diabetic wound model demonstrate that GDFE can rapidly promote the diabetic wound repair and skin regeneration, through fast anti-inflammation and angiogenesis and M2 macrophage polarization. This study provides highly efficient strategy for treating diabetic wound repair through designing the M2 polarization-enabled anti-inflammatory, antioxidant, and antibacterial bioactive materials. 相似文献