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To explore the ideal architecture of Pt-Co bimetallic catalyst for aromatics saturation, various Pt-Co bimetallic catalysts were synthesized via the galvanic replacement, the co-impregnation, and the sequential impregnation methods, and were characterized by CO chemisorption, transmission electron microscopy(TEM), H_2-temperature-programmed reduction(H_2-TPR), H_2-temperature-programmed desorption(H_2-TPD), X-ray fluorescence(XRF) spectrometry, and inductively coupled plasma atomic emission spectroscopy(ICP-AES), while the catalysts were evaluated by the flow reactor study of toluene hydrogenation. These characterization results suggest that the surface decoration of Pt has little influence on the number of active sites located on the surfaces of the reduced Co-based catalysts, but can greatly suppress the oxidation of Co at room temperature and provide the activated hydrogen at a relatively low temperature. It is demonstrated that their chemical properties and catalytic performance are largely dependent on the location of Pt atoms in the bimetallic catalysts. The architecture of Pt-Co bimetallic catalyst consisting of Co/SiO_2 decorated with 0.3% of Pt, with the most of Pt atoms being situated on the surfaces of Co nanoparticles, is the active structure for aromatic saturation and has the maximum utilization of Pt. 相似文献
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为求解射表编拟中弹道计算所需的弹丸空气动力系数,采用有限容积法求解N-S方程、S-A湍流模型并考虑具体边界条件,借助FLUENT模拟弹丸外流场.对某型榴弹实现了流场模拟,得到了攻角为0°、4°、8°和马赫数为0.6~2.1时的弹丸阻力系数、升力系数、俯仰力矩系数.通过该弹气动力系数数值模拟计算值与雷达数据提取值、工程计算值、纸靶试验值进行比较,表明数值模拟得到的曲线规律较好.在此基础上,采用阻力、升力符合系数修正方法,实现了数值结果在射表编拟中的应用,且精度满足射表编拟等弹道计算应用的需要. 相似文献
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将蒜黄根中提取的总膳食纤维(total dietary ifber,TDF)添加于低脂乳化肠,探究蒜黄根TDF对低脂乳化肠品质的影响.以正常脂肪添加量为对照组,实验组减少15%(以降低脂肪含量前瘦肉与猪背膘的总质量为基准)脂肪后分别添加不同质量的蒜黄根TDF(1.25%、2.50%、3.75%、5.00%、6.25%,... 相似文献
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