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41.
Yuki Akinaga Tokuhisa Kawawaki Hinano Kameko Yuki Yamazaki Kenji Yamazaki Yuhi Nakayasu Kosaku Kato Yuto Tanaka Adie Tri Hanindriyo Makito Takagi Tomomi Shimazaki Masanori Tachikawa Akira Yamakata Yuichi Negishi 《Advanced functional materials》2023,33(33):2303321
Single-atom (SA) catalysts exhibit high activity in various reactions because there are no inactive internal atoms. Accordingly, SA cocatalysts are also an active research fields regarding photocatalytic hydrogen (H2) evolution which can be generated by abundant water and sunlight. Herein, it is investigated whether 10 transition metal elements can work as an SA on graphitic carbon nitride (g-C3N4; i.e., gCN), a promising visible-light-driven photocatalyst. A method is established to prepare SA-loaded gCN at high loadings (weight of ≈3 wt.% for Cu, Ni, Pd, Pt, Rh, and Ru) by modulating the photoreduction power. Regarding Au and Ag, SAs are formed with difficulty without aggregation because of the low binding energy between gCN and the SA. An evaluation of the photocatalytic H2-evolution activity of the prepared metal SA-loaded gCN reveals that Pd, Pt, and Rh SA-loaded gCN exhibits relatively high H2-evolution efficiency per SA. Transient absorption spectroscopy and electrochemical measurements reveal the following: i) Pd SA-loaded gCN exhibits a particularly suitable electronic structure for proton adsorption and ii) therefore they exhibit the highest H2-evolution efficiency per SA than other metal SA-loaded gCN. Finally, the 8.6 times higher H2-evolution rate per active site of Pd SA is achieved than that of Pd-nanoparticles cocatalyst. 相似文献
42.
43.
Y Takashima M Yoshida A Kokaze Y Orido S Tsugane M Ishikawa Y Takeuchi Y Takagi N Tanaka S Watanabe T Akamatsu 《Canadian Metallurgical Quarterly》1998,8(4):216-226
To clarify how and why blood pressure differs between occupations, the proportions of hypertensives, and the measures of blood pressure, body mass index (BMI) and alcohol consumption among the individuals not taking antihypertensive drugs were compared between the eight occupational categories using the data from a health check-up for 589 middle-aged Japanese males, mostly randomly selected from five areas in Japan. After adjusting for age, the relationships of occupation to the proportion of hypertensives and the mean systolic and diastolic blood pressure substantially differed among the five areas. However, after further adjustment for residence, these blood pressure levels (the proportion of hypertensives, and the mean systolic and diastolic blood pressure) were found to be higher for the "Personnel in transport and communications", the "Clerical personnel", the "Managerial and civil personnel" and the "Professional and technical personnel", whereas these values were consistently lowest in the "Service personnel". Age and residence-adjusted mean BMI was also higher for the four occupational categories with the increased blood pressure levels. According to a weighted multiple regression analysis across the eight occupations, the age and residence-adjusted mean BMI was a significant predictor of the age and residence-adjusted mean systolic and diastolic blood pressure (p = 0.068 and 0.018, respectively). These results suggest that the occupation-related changes in BMI may largely contribute to the occupation-related changes in blood pressure. 相似文献
44.
Research findings and various published studies point to interleukin 4 (IL-4) and CD23 antigen as instrumental in allergic reactions of allergy patients because these two substances are part of the main triggering mechanisms in cells producing IgE antibodies. In this study it was investigated whether the control of IL-4 and CD23 levels result in a decrease of the severity of allergic reactions. It is well known that azelastine hydrochloride (AZ, CAS 79307-93-0) suppresses symptoms of nasal allergy. The antiallergic activity of this drug includes the suppression of IgE antibody production, antigen-antibody reactions, liberation of mediators and mediator antagonism. One report states that the cytokines IL-2, IL-3, and IL-4 were suppressed by AZ in cultured cells. There have been no reports regarding cytokines in clinical treatment using AZ. Therefore, the effects of AZ treatment on IL-4, soluble CD23, and RAST (radioallergosorbent test) levels in the sera of allergic rhinitis patients were studied. The results show that the levels of IL-4 and soluble CD23 were significantly reduced by the administration of AZ over a 4-week period, especially in patients with "excellent" or "good" efficacy of therapy. 相似文献
45.
Yuichiro Ezoe Ikuyuki Mitsuishi Utako Takagi Masaki Koshiishi Kazuhisa Mitsuda Noriko Y. Yamasaki Takaya Ohashi Fumiki Kato Susumu Sugiyama Raul E. Riveros Hitomi Yamaguchi Shinya Fujihira Yoshiaki Kanamori Kohei Morishita Kazuo Nakajima Ryutaro Maeda 《Microsystem Technologies》2010,16(8-9):1633-1641
We are developing novel ultra light-weight and high-resolution X-ray micro pore optics for space X-ray telescopes. In our method, curvilinear micro pore structures are firstly fabricated by silicon deep reactive ion etching (DRIE) or X-ray LIGA processes. Secondly, side walls of the micro structures are smoothed by magnetic field assisted finishing and/or hydrogen annealing techniques for high reflectivity mirrors. Thirdly, to focus parallel X-ray lights from astronomical objects, these structures are elastically or plastically bent into a spherical shape. Fourthly, the bent structures are stacked to form a multi-stage X-ray telescope. In this paper, we report on fabrication and X-ray reflection tests of silicon and nickel X-ray mirrors using the DRIE and LIGA processes, respectively. For the first time, X-ray reflections were confirmed on both of the mirrors. Estimated rms roughnesses were 5 nm and 3 nm for the silicon and nickel mirrors, respectively. 相似文献
46.
Yoshifumi Morita Norihiro Toya Ryosuke Takeichi Hitomi Hattori Hirofumi Tanabe Yoshiaki Takagi 《Advanced Robotics》2016,30(21):1406-1414
We developed a new training system, called ‘UR-System 2’, for the recovery of motor function of a plegic upper limb after stroke. UR-System 2, which was redesigned based on knowledge gained from clinical tests using UR-System 1, was newly equipped with a function for testing the motor function of patients, such as isolated movement. In order to verify the effectiveness of UR-System 2, we conducted the following procedures: we verified the safety of training in healthy persons; we gathered standard data on pronation and supination of healthy forearms during tests; and, we verified that the test function was effective in evaluating the recovery effect of isolated movement in two hemiplegic patients. 相似文献
47.
Ergonomic Chair Design by Fusing Qualitative and Quantitative Criteria Using Interactive Genetic Algorithms 总被引:3,自引:0,他引:3
Brintrup A.M. Ramsden J. Takagi H. Tiwari A. 《Evolutionary Computation, IEEE Transactions on》2008,12(3):343-354
This paper emphasizes the necessity of formally bringing qualitative and quantitative criteria of ergonomic design together, and provides a novel complementary design framework with this aim. Within this framework, different design criteria are viewed as optimization objectives, and design solutions are iteratively improved through the cooperative efforts of computer and user. The framework is rooted in multiobjective optimization, genetic algorithms, and interactive user evaluation. Three different algorithms based on the framework are developed, and tested with an ergonomic chair design problem. The parallel and multiobjective approaches show promising results in fitness convergence, design diversity, and user satisfaction metrics. 相似文献
48.
Site-specific electronic structures were investigated by electron energy loss spectroscopy (EELS) under electron channeling conditions. The Al-K and Mn-L(2,3) electron energy loss near-edge structure (ELNES) of, respectively, NiAl2O4 and Mn3O4 were measured. Deconvolution of the raw spectra with the instrumental resolution function restored the blunt and hidden fine features, which allowed us to interpret the experimental spectral features by comparing with theoretical spectra obtained by first-principles calculations. The present method successfully revealed the electronic structures specific to the differently coordinated cationic sites. 相似文献
49.
50.
M. Tanaka K. Higashida H. Nakashima H. Takagi M. Fujiwara 《International Journal of Fracture》2006,139(3-4):383-394
Fracture toughness of silicon crystals has been investigated using indentation methods, and their surface energies have been
calculated by molecular dynamics (MD). In order to determine the most preferential fracture plane at room temperature among
the crystallographic planes containing the 〈001〉, 〈110〉 and 〈111〉 directions, a conical indenter was forced into (001), (110)
and (111) silicon wafers at room temperature. Dominant {110}, {111} and {110} cracks were introduced from the indents on (001),
(011) and (111) wafers, respectively. Fracture occurs most easily along {110}, {111} and {110} planes among the crystallographic
planes containing the 〈001〉, 〈011〉 and 〈111〉 directions, respectively. A series of surface energies of those planes were calculated
by MD to confirm the orientation dependence of fracture toughness. The surface energy of the {110} plane is the minimum of
1.50 Jm−2 among planes containing the 〈001〉 and 〈111〉 directions, respectively, and that of the {111} plane is the minimum of 1.19
Jm−2 among the planes containing the 〈011〉 direction. Fracture toughness of those planes was also derived from the calculated
surface energies. It was shown that the K
IC value of the {110} crack plane was the minimum among those for the planes containing the 〈001〉 and 〈111〉 directions, respectively,
and that K
IC value of the {111} crack plane was the minimum among those for the planes containing the 〈011〉 direction. These results are
in good agreement with that obtained conical indentation. 相似文献