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161.
Hartmut Koehler Tobias Frische Ingo Dobner Peter Behrend Maike Schaefer Heidi Taubner Bernd Jastorff Jürgen Warrelmann Ulrich Walter 《Environmental Sciences Europe》2001,13(5):291-300
Results of a field experiment (please refer to Warrelmann et al. 2000a) document TNT-degradation and regeneration after the establishment of a phytoremediation. Various approaches are included in a complex monitoring system, which are conducted in the field (nitroaromatics in soil, seepage water, and plants; soil fauna; soil fungi; decomposition) as well as in the lab (a battery of 6 biotests). The data document a high heterogeneity of the TNT-contamination, a rapid initial decrease and a mediocre displacement of nitroaromatics in plants and seepage water. The initial rapid transformation of TNT to aminodinitrotoluenes ceases significantly after 3 months. Results of the biotest battery allow a sophisticated assessment of soil toxicity; the results from the soil ecological field investigations make the long-term effects of TNT-contamination likely. In a third part of the series of articles, a synopsis and judgement of the project will be delivered. 相似文献
162.
Hyun‐Han Kwon Abedalrazq F. Khalil Tobias Siegfried 《Journal of the American Water Resources Association》2008,44(2):436-448
Abstract: It is now widely acknowledged that climate variability modulates the frequency of extreme hydrological events. Traditional methodologies for hydrologic frequency analysis are not devised to account for variation in the exogenous teleconnections. Flood frequency analysis is further plagued by the assumptions of stationary in the causal structure as well as ergodicity. Here, we propose a dynamical hierarchical Bayesian analysis to account for exogenous forcing that govern the summer season rainfall. The precursors for Korean summer rainfall at different frequencies are identified utilizing wavelet and independent component analyses. The sea surface temperatures, the ensemble of rainfall predictions by General Circulation Model, in addition to the typhoon attributes were found to have direct correlation with extreme rainfall events and were used as inputs to the logistic regression model. The model parameters are estimated using Markov Chain Monte Carlo and the resulting posterior distributions associated with individual inputs are analyzed to advance our understanding of the spatiotemporal impact of the teleconnections. Eight rainfall stations throughout Korea are considered in this analysis. We demonstrate that the probability of occurrence of extreme events could be successfully projected at a 90% rate of correct classification of extreme events. 相似文献
163.
Carl Linderholm Alberto Abad Tobias Mattisson Anders Lyngfelt 《International Journal of Greenhouse Gas Control》2008,2(4):520
Chemical-looping combustion, CLC, is a technology with inherent separation of the greenhouse gas CO2. The technique uses an oxygen carrier made up of particulate metal oxide to transfer oxygen from combustion air to fuel. In this work, an oxygen carrier consisting of 60% NiO and 40% NiAl2O4 was used in a 10 kW CLC reactor system for 160 h of operation with fuel. The first 3 h of fuel operation excepted, the test series was accomplished with the same batch of oxygen carrier particles. The fuel used in the experiments was natural gas, and a fuel conversion to CO2 of approximately 99% was accomplished. Combustion conditions were very stable during the test period, except for the operation at sub-stoichiometric conditions. It was shown that the methane fraction in the fuel reactor exit gas was dependent upon the rate of solids circulation, with higher circulation leading to more unconverted methane. The carbon monoxide fraction was found to follow the thermodynamical equilibrium for all investigated fuel reactor temperatures, 660–950 °C. Thermal analysis of the fuel reactor at stable conditions enabled calculation of the particle circulation which was found to be approximately 4 kg/s, MW. The loss of fines, i.e. the amount of elutriated oxygen carrier particles with diameter <45 μm, decreased during the entire test period. After 160 h of operation the fractional loss of fines was 0.00022 h−1, corresponding to a particle life time of 4500 h. 相似文献
164.
Sabine Grundmann Ulrike Dörfler Bernhard Ruth Christine Loos Tobias Wagner Heidrun Karl Jean Charles Munch Reiner Schroll 《Water, Air, & Soil Pollution: Focus》2008,8(2):177-185
A recently designed two-chamber-lysimeter-test-system allows the detailed investigation of degradation, transport and transfer
processes of 14C-labeled substances in soil–plant–atmosphere-systems under outdoor conditions. With this test system it is feasible to distinguish
between 14C-emissions from soil surfaces and 14C-emissions from plant surfaces in soil monoliths under real environmental conditions. Special soil humidity sensors allow
the measurement of soil water content near to the soil surface, in 1 and 5 cm depth. The behavior of organic chemicals can
be followed for a whole vegetation period and a mass balance for the applied chemical can be established. Some selected results
of the herbicides isoproturon and glyphosate – using the two-chamber-lysimeter-test-system – are presented to demonstrate
its applicability for the identification and quantification of the processes that govern pesticide behavior in soil–plant-systems.
Mineralization of 14C-isoproturon was very different in four different soils; the mineralization capacity of the soils ranged from 2 to 60%. Leaching
of isoproturon in general was very low, but depending on the soil type and environmental conditions isoproturon and its metabolites
could be leached via preferential flow, especially shortly after application. For the herbicide 14C-glyphosate no accumulation of residues in the soil and no leaching of the residues to deeper soil layers could be observed
after three applications. Glyphosate was rapidly degraded to AMPA in the soil. Glyphosate and AMPA were accumulated in soy
bean nodules. 相似文献
165.
Mol Marcos Paulo Gomes Zolnikov Tara Rava Neves Arthur Couto dos Santos Giulia Roriz Tolentino Júlia Luiza Lopes de Vasconcelos Barros Raphael Tobias Heller Leo 《Environmental science and pollution research international》2022,29(28):42466-42475
Environmental Science and Pollution Research - There are increasing worldwide concerns about the negative impacts of healthcare waste generated in hospitals, especially in low- and middle-income... 相似文献