南海西北部一次海上海雾的微物理及化学特性分析

利用2017年3月MICAPS资料、欧洲气象中心再分析ERA-Interim数据及在南海西北部海上的海雾观测数据,分析了南海西北部一次海上海雾的微物理特征和雾水化学特性,并将海上海雾与南海岸边海雾进行对比分析。结果表明:此次海雾为南海偏南暖气流移至冷海面发生冷却并达到饱和而形成。海雾过程中气压与气温变化趋势相反,相对湿度不断增加,雾滴数浓度、液态含水量和平均直径的平均值分别为198 cm-3、0.116 g/cm3和5.6 μm。相比广东湛江东海岛和广东茂名博贺地区岸边海雾个例,本次海上海雾水汽充足,雾滴偏大。本次海雾属于酸性海雾,pH值变化范围为2.51~3.50,海雾后的雨水样本pH值则为4.05。海雾发生初期电导率比其它阶段高很多,说明海雾发生的初始阶段雾水溶解了大量的气溶胶。海上雾水中Na+和Cl-浓度最高,浓度分别为32 535 μmol/L和53 466 μmol/L,K+浓度远高于Mg2+和Ca2+,而东海岛岸边海雾相反。      

基于FY-3B卫星资料的中国南海海区1—3月海雾时空分布特征研究

为全面了解中国南海海区海雾的分布特征,为南海海雾气象服务提供基础背景资料,利用2011—2016年1—3月FY-3B气象卫星资料的雾监测产品,分析了中国南海海区海雾的时空分布特征。结果表明：中国南海海雾具有特定的区域特征,中国南海海雾多出现在华南沿海、北部湾沿海、琼州海峡和海南岛东北部沿海海区,南海南部海域出现海雾概率低;南海出现高频次海雾的时间多发生在2月,1月次之,3月最少。该研究结果可为中国南海海雾研究提供背景资料。     

基于多灰度共生矩阵特征值的黄渤海白天海雾识别算法

本文基于多灰度共生矩阵特征值,即相关性、对比度、同质性和能量,进行联合海雾遥感判识,提出一种高准确率黄渤海白天海雾识别算法。采用第二代静止气象卫星FY-4A可见光、近红外和红外数据,将该算法应用于黄渤海区域白天海雾判识,并利用2019—2020年沿黄渤海气象站点能见度实测数据及CALIPSO卫星数据产品对本算法识别结果进行精度验证。结果表明：海雾识别平均检测率(POD)为92%,误报率(FAR)为27%,临近成功指数(CSI)为69%,可以实现对海雾的动态监测,为海上交通等领域提供较好的数据支持。     

Characteristics of Quasi-Periodic Oscillations During Sea Fog Events

Based on the high-resolution datasets collected in a sea fog field experiment at the northern coast of South China Sea, the variations of liquid water content (LWC) and net longwave radiation flux (NLRF) during two sea fog events on 16th-17th and 18th-19th March, 2008 are exaimeed by wavelet analysis, and the cooling mechanisms for fog formation and persistence are also investigated. The main results are shown as follows. (1) Sea fog may develop and persist whether it is cloudy or not aloft. However, when there is cloud aloft the LWC is less and wind speed in sea fog is higher than that in the clear sky. (2) The quasi-periodic oscillations (QPOs) of NLRF are observed in the formation stage of the two fogs. QPOs of LWC are only found in the developing stage no matter with cloudless or cloudy condition. (3) It is likely that sea fog forms by the cooling effects of longwave radiation and develops through the vertical mixing induced by the radiative cooling at the upper level. (4) During sea fog development and persistence, other mechanisms could also play important roles in fog-layer cooling, such as turbulent heat transport and radiation transport between air-sea interfaces.     

闽南沿海一次春季海雾过程微物理特征分析

利用地面自动站观测、风廓线雷达、ERA5再分析资料、葵花8号高分辨率卫星资料以及FM-120型雾滴谱资料,分析了2019年4月7日闽南沿海一次强浓雾过程的环流形势以及微物理特征。环流形势分析表明,此次海雾过程500 hPa为槽底偏西西北气流,700 hPa至地面为一致的偏南气流,探空形势稳定。海雾发生前,整层风速明显减小,弱风速层厚度迅速增大,为海雾的形成提供了稳定的环流背景。卫星监测分析表明,海雾首先快速形成于台湾海峡上,在偏南气流作用下,平流至沿海地区。水文条件分析表明,福建近海存在一条冷水带,从海峡中部至沿海海温梯度大,海温在18~24℃,近海气海温差介于0~2℃,有利于海峡内平流冷却雾的形成。雾滴谱分析表明,翔安站能见度显著下降伴随着粒子数浓度、液态水含量显著增加,雾滴谱爆发性拓宽。海雾过程中,5 min平均粒子数浓度最大超过200个·cm^-3,瞬时数浓度最大达到468个·cm^-3,雾过程平均数浓度为100个·cm^-3。5 min平均液态水含量最高达到0.41 g·m^-3,瞬时液态水含量最大达到1.35 g·m^-3,雾过程平均液态水含量为0.17 g·m^-3。粒子浓度呈现双峰结构特征,峰值分别位于4~6和22~26μm,表明小粒子和大粒子对海雾的形成均有明显的贡献。     

华南沿海暖海雾过程中的湍流热量交换特征

湍流交换是海雾中的关键物理过程, 在海雾的热量和水汽平衡过程中起重要作用。本文根据2007年3月24～25日一次海雾的外场观测数据, 分析了海雾过程中近海面湍流热量交换特征; 并在区分风切变机械湍流与雾顶长波辐射冷却热力湍流的基础上, 着重分析了两种不同性质的湍流对海雾发展和维持的作用。结果表明: (1) 本次海雾是在西南低压和变性冷高压的控制下, 来自南海东部暖水区的空气平流在近岸冷海面上形成的暖海雾; 暖海雾中的湍流热量交换过程比冷海雾更为复杂; (2) 在暖海雾的形成和消散阶段, 风切变机械湍流的热量输送起主要作用; 而在发展和维持阶段, 既有风切变机械湍流的热量输送作用, 也有雾顶长波辐射冷却热力湍流的热量输送作用; (3) 风切变机械湍流向冷海面输送热量, 对近海面空气起到降温和增湿作用; 热力湍流同样向冷海面输送热量, 但对雾层起到增温和降湿作用; (4) 暖海雾中的湍流热量交换机制与雾层的非充分混合结构有密切关系。     

The influences of macro- and microphysical characteristics of sea-fog on fog-water chemical composition

ABSTRACT During a sea-fog field observation campaign on Donghai Island in the spring of 2011, fog-water, visibility, meteorological elements, and fog droplet spectra were measured. The main cations and anions in 191 fog-water samples were Na＋, NH2, H＋, NO3, C1- and SO] , and the average concentrations of cations and anions were 2630 and 2970 p-eq L 1, respectively. The concentrations of Na＋ and C1- originated from the ocean were high. The enhancement of anthropogenic pollution might have contributed to the high concentration of NH＋, H＋, and NO^-3. The average values ofpH and electrical conductivity （EC） were 3.34 and 505 uS cm-1, respectively, with a negative correlation between them. Cold fronts associated with cyclonic circulations promoted the decline of ion loadings. Air masses from coastal areas had the highest ion loadings, contrary to those from the sea. The ranges of wind speed, wind direction and temperature corresponding to the maximum total ion concentration （TIC） were 3.5-4 m s-1, 79°-90° and 21°C-22°C, respectively. In view of the low correlation coefficients, a new parameter Lr was proposed as a predictive parameter for TIC and the correlation coefficient increased to 0.74. Based on aerosol concentrations during the sea-fog cases in 2010, we confirmed that fog-water chemical composition also depended on the species and sizes of aerosol particles. When a dust storm passed through Donghai Island, the number concentration of large aerosol particles （with diameter 〉 1 p-m） increased. This caused the ratio of CaZ＋/Na＋ in fog-water to increase significantly.     

2009年春季一次黄海海雾的观测分析及数值模拟

利用5种观测资料和RAMS（regional atmospheric modeling system）模式对2009年5月2_5日发生在黄海海域的一次海雾过程进行了观测分析和数值模拟研究。结果表明：1）所取个例的整个生命过程受同一高压系统影响,该高压在海雾过程后期的形变促使海雾消散,这在以往的黄海海雾中较为罕见。2）黄海北部形似“7”的雾区形态的出现和演化与1～3℃气海温差的变化吻合,气海温差对海雾形成和演变的重要作用得到再次验证。3）RAMS模式具有一定的海雾数值模拟能力,得到的雾顶高度分布与卫星云图所显示的雾区形态吻合良好。     

Impacts of Secondary Aerosols on a Persistent Fog Event in Northern China

The chemistry version of the Weather Research and Forecasting model (WRF/Chem) was coupled with the anthropogenic emission inventory of David Streets to investigate the impacts of secondary aerosols on a persistent fog event from 25 to 26 October 2007, in Northern China. The spatial distribution of the simulated fog is consistent with satellite observations, and the time-height distributions of the simulated boundary layer where the fog formed are also in good agreement with these observations. The sensitivity studies show that the secondary aerosols of SO 4 , NO 3 , and NH 4 formed from gaseous precursors of SO 2 , NO x , and NH 3 had substantial impacts on the formation processes and microphysical structure of the fog event. The decrease of the secondary aerosols obviously reduced the liquid water path and column droplet number concentration of the fog below the 1-km layer, and the corresponding area-averaged liquid water path and droplet number concentration of the fog decreased by 43% and 79%, respectively. The concentrations of NO x and NO 3 were found to be extremely high in this case. The concentration of interstitial aerosol NO 3 was much higher than the SO 4 and NH 4 , but the concentration of SO 4 was highest in the cloud-borne aerosols. The average activation ratios for SO 4 , NO 3 , and NH 4 were 34%, 31%, and 30%, respectively, and the maximum ratios reached 62%, 86%, and 55% during the fog episode.     

一次黄海海雾成因分析及数值模拟试验

根据GOES-9(Geostationary Operational Environmental Satellite）可见光卫星云图和韩国济州岛探空资料等,利用RAMS(Regional Atmospheric Modeling System)模式（6.1版）对2009年3月17-18日发生在黄海海域的一次大风条件下出现的海雾天气进行模拟。结果表明：与卫星云图所显示的雾区范围相比,模拟结果对海雾的生成、发展、移动都有较好吻合;云水混合比是影响大气水平能见度分布的主要因子,云水混合比大值区主要集中在距地面300 m以下的低空;雾区存在几个云水混合比大值区,并分布在不同的高度,说明海雾的团状不均匀结构;海上平流雾常发生在风速较大的情况下,RAMS模式对此具有一定的模拟能力。     

海雾的准周期振荡特征

根据南海北部海雾外场观测获取的高分辨率液态含水量、长波辐射通量数据,采用小波分析方法分析了2008年3月16—17日和18—19日两次海雾中的液态水含量、净长波辐射通量的变化特征,讨论南海北部海雾发展和维持的冷却机制。结果显示:(1)无论在有云或无云条件下,海雾都可发展和维持;但前者的液态含水量明显小于后者,而风速大于后者;(2)在地面海雾的生成之前和生成初期,净辐射通量都存在准周期振荡现象,无论无云/有云,地面海雾液态水的大幅度发展的阶段都存在含水量的准周期振荡现象;(3)含水量的准周期振荡现象与振荡发生时段的长波辐射通量关系不大,而主要通过湍流对液态水的混合作用与高空海雾液态水大量生成阶段的雾顶长波辐射间接相关。(4)海雾的生成都与雾顶长波辐射冷却密切相关,但发展和维持可通过不同的冷却机制,既可通过海气间湍流热量输送和辐射传输,也可通过雾顶长波辐射冷却。     

合肥市不同天气条件下大气气溶胶粒子理化特征分析

为探讨合肥市霾天气大气气溶胶粒子的组成及来源,在2012-2013年代表性月份用安德森分级采样器在合肥市区进行大气气溶胶粒子采样,并分析各样本中水溶性无机离子成分(NH4+、Mg2+、Ca2+、Na+、 K+、NO2-、NO3-、Cl-、SO42-)。根据同期气象资料把采样背景天气分为晴空、雾、霾、轻雾等4类,详细分析了这4种天气下大气细粒子(指PM2.1)和粗粒子(粒径大于2.1 μm部分)的浓度、组成以及主要离子组分的异同。结果表明:(1)观测期间晴空天多对应空气质量优良,雾、霾天对应轻度到重度污染,从晴空天到雾、霾天,PM2.1浓度大幅度上升,且其占总悬浮颗粒物(TSP)的比例显著上升。(2)从晴空天到雾、霾天,水溶性无机离子质量占PM2.1质量浓度的比例上升,分别为46%(晴空)、67%(霾)、61%(雾)、80%(轻雾)。PM2.1中水溶性无机离子浓度居前3位的雾、霾天是SO42-、NO3-和NH4+,晴空天为SO42-、Ca2+、NO3-。(3)与晴空天相比,霾天PM2.1中水溶性无机离子浓度变化倍数最大的是NO3-(为晴空的6.1倍,下同)、其次是NH4+(3.6倍)和SO42-(3.0倍);雾和轻雾天PM2.1中水溶性无机离子浓度变化最大的是NO3-(>10倍)、其次是NH4+(>5倍)和Cl-(>4.0倍)。(4)4种天气下,与人为污染有关的离子(SO42-、NO3-、Cl-、NH4+)尺度谱存在显著差异,呈双峰型、单峰型、三峰型等;而Ca2+的尺度谱无明显变化,基本上都呈双峰型。(5)在粒径3.3 μm以下,阳、阴离子平衡较好,随着尺度增大变差,且晴空天比雾、霾天差。主要阴离子浓度间、Cl-和Na+间的比值和相关性,在晴空天和雾、霾天差异较大。      

夏季低压控制下黄海西北部海域海雾发生气象条件合成分析

利用瞬变扰动分析的原理,提供了一个可以客观判定海雾发生时天气类型的方法。在分类结果的基础上,对环流形势、散度和垂直速度以及温度湿度的垂直廓线等进行合成分析,得到低空（1 000 hPa）为低压扰动下发生海雾（L型海雾）的环流和物理量场基本特征,并与高压控制下海雾（H型海雾）进行对比,结果表明：1）L型海雾位势高度负异常扰动主要表现在低层,其平均值为-65.66 gpm,向上逐渐减弱;2）L型海雾在发生时其逆温强度小于H型海雾,雾层较厚,雾层上空湿度仍然比较大,而H型海雾雾层上空有比较明显的干层;3）L型海雾在垂直方向上的分布具有三层结构,第一层1 000～950 hPa为辐合伴有弱上升和下沉运动,第二层950～850 hPa为辐散伴有弱下沉运动,第三层850～500 hPa为逐渐加强的上升运动;H型海雾为两层结构,1 000 hPa为辐散伴有弱的上升和下沉运动,950～500 hPa为一致的下沉运动;4）概率密度统计分析进一步定量表明了L型和H型海雾发生时垂直运动以及相对湿度在各层中的分布情况。这些结论对黄海西北部夏季低压环流形势下海雾的预报提供了重要参考。     

Microphysical characteristics of sea fog over the east coast of Leizhou Peninsula, China

Microphysical properties of sea fog and correlations of these properties were analyzed based on the measurements from a comprehensive field campaign carried out from 15 March to 18 April 2010 on Donghai Island (21°35’’N, 110°32’5’’E) in Zhanjiang, Guangdong Province, China. There were four types of circula- tion pattern in favor of sea fog events in this area identified, and the synoptic weather pattern was found to influence the microphysical properties of the sea fogs. Those influenced by a warm sector in front of a cold front or the anterior part of low pressure were found to usually have a much longer duration, lower visibility, greater liquid water content, and bigger fog droplet sizes. A fog droplet number concentration of N≥1 cm-3 and liquid water content of L≥0.001 g m-3 can be used to define sea fogs in this area. The type of fog droplet size distribution of the sea fog events was mostly monotonically-decreasing, with the spectrum width always being >20 μm. The significant temporal variation of N was due in large part to the number concentration variation of fog droplets with radius <3 μm. A strong collection process appeared when droplet spectrum width was >10 μm, which subsequently led to the sudden increase of droplet spectrum width. The dominant physical process during the sea fog events was activation with subsequent condensational growth or reversible evaporation processes, but turbulent mixing also played an important role. The collection process occurred, but was not vital.     

南海近海面风场变化特征及其与ENSO的相关性研究

利用1979—2017年共39 a欧洲中期天气预报中心（ECMWF）海表面10 m风场资料,采用经验正交函数方法（EOF）、小波时频特征分析等方法分析了南海近海面风场变化特征及其对ENSO的响应。结果表明：南海近海面风场第一模态海表面平均风速呈减小趋势, 呈现年代际变化,且与ENSO相关,但相关性在1990年后趋于减小;第二模态中南海北部和南部平均风速呈减小趋势,中部增大;第三模态中南海中部海表面平均风速趋于减小,北部和南部增大,第二和第三模态均表现为年际变化,且均与ENSO显著相关,近年来ENSO与第三模态的相关性逐渐增强。春季南海表面平均风速从南到北逐渐增加;夏季在越南沿岸部分海域仍有一个风速极大值中心,从该海域向四周逐渐减小,整片海域风向均是西南风;秋季由南向北依次增加;冬季南海整片海域风速都较大,越南沿岸和我国东沙群岛海域存在两个极大值中心。     

一次南海海雾微物理结构个例分析

本文利用2010年3月22～23日广东省湛江市一次海雾过程的雾滴谱和能见度资料,分析了海雾的微物理特征及微物理参量(数浓度、液态含水量和平均直径)之间的相关性,并讨论了影响海雾的主要物理过程。结果表明:湛江地区海雾的平均雾滴谱符合Junge分布;在海雾发展和成熟阶段,雾滴谱拓宽过程以及数浓度与平均直径的正相关关系表明本次海雾过程主要以雾滴活化和凝结增长过程为主;湍流过程的参与使得雾滴混合均匀,雾滴平均直径向3.5 μm附近集中,趋向平均化。同时湍流使雾体内部和外部空气交流,外部空气的凝结核核化,数浓度升高,凝结增长造成小雾滴变大。     

黄渤海一次持续性大雾过程特征和成因分析

利用日本MTSAT1R卫星数据、常规地面和高空观测数据、NCEP FNL客观再分析资料和NEARGOOS（NorthEast Asian Regional Global Ocean Observing System）的海表温度（SST）数据,分析了2010年5月31日至6月5日发生在黄渤海及周边地区的一次持续性海雾天气的形成、维持、消散特征及其物理机制。结果表明：大雾形成前低层水汽非常充沛,入海变性冷高压的稳定维持为这次持续性海雾过程提供了有利的背景条件,海雾在夜间辐射冷却作用下形成;大雾期间黄渤海     

春季黄海海雾WRF参数化方案敏感性研究

利用2005—2011年10次春季黄海海雾个例开展WRF模式参数化方案敏感性研究。结果表明:边界层方案对WRF模式雾区模拟结果起决定作用,而微物理方案影响较小,它主要影响海雾浓度和高度。边界层与微物理方案的最佳组合为YSU与Lin方案,最差为Mellor-Yamada与WSM5方案;Mellor-Yamada和QNSE方案模拟的近海面湍流过强,导致边界层过高,不利于海雾的发展与维持;而MYNN与YSU方案刻画的湍流强度与边界层高度合适,有利于海雾发展与维持。MYNN方案虽与YSU方案相当,但在大多数海雾个例中,后者明显优于前者,而在有些个例中却刚好相反。因此对于某一具体海雾个例而言,所用边界层方案仍需在它们之中选择最优者。这些信息可为黄海海雾WRF模式边界层与微物理方案的选择与改进提供参考。     

南岭大瑶山浓雾雾水的化学成分研究

文中利用 1998年 12月～ 1999年 1月和 2 0 0 1年 2～ 3月在南岭山地采集的雾水样品资料 ,分析了南岭山地浓雾雾水的化学成分 ;对 3次典型浓雾过程雾水的离子浓度及其可能的来源进行了分析 ;发现酸雾的频率达 5 1% ,酸雾的危害不容忽视。南岭山地的浓雾雾水中的诸离子浓度远高于雨水。不同过程雾水的化学特征变化差异明显 ,在雾水中浓度最高的阴离子是SO2 -4,其次是NO-3 ;阳离子Ca2 ,NH 4 的浓度最高。雨水比雾水酸性更强 ,说明虽然雾水中的离子浓度较雨水高得多 ,但大量的离子成分中存在更多的缓冲物质 ,比如说NH 4 和Ca2 。雾水中的Ca2 ,SO2 -4,Mg2 有明显的富集现象 ,南岭大瑶山的雾水主要受大陆环境和人类活动的影响。     

Diurnal variations of precipitation over the South China Sea

In this study, the diurnal variations of precipitation and related mechanisms over the South China Sea (SCS) are studied using the TRMM and other auxiliary atmospheric data. We have found that: (1) the amplitude and peak time of the diurnal precipitation over SCS exhibit remarkable regional features and seasonal variations. Diurnal variations are robust all the year around over the southern SCS especially over the Kalimantan Island and its offshore area. Over the middle to northern SCS, however, diurnal variations are noticeable only in the summer and autumn; (2) over the northern SCS precipitation peaks in early morning, while over the southern SCS it has two diurnal peaks: one in the early morning and another in the late afternoon; (3) the diurnal variations of precipitation over the SCS are related to the activity of the SCS summer monsoon and the ENSO events. The late afternoon precipitation increases remarkably after the onset of the SCS summer monsoon over the northern SCS. The early-morning rainfall peak is much more significant during La Nina years than during El Nino years; (4) the land–sea breeze is responsible for the diurnal cycle over the Kalimantan Island and its offshore area while the “static radiation–convection” mechanisms may result in the early-morning rainfall peak over the SCS.