准晶非线性光子晶体中二次谐波波长和温度调谐的研究

在八重准周期极化的铌酸锂非线性光子晶体中,通过调节基频光波长实现了多个波长的同时共线准相位匹配倍频,最高转换效率达36%.同时,测量了准晶非线性光子晶体中二次谐波转换效率随晶体温度以及入射波长的变化,结果表明二次谐波在长波处具有更宽的温度以及波长调谐带宽.该项研究对于准周期非线性光子晶体在实际工作中的运用具有重要的指导意义. 关键词： 准周期 非线性光子晶体 温度调谐 波长调谐     

多光子非线性Compton散射的能量转换

研究了多光子非线性Compton散射中电子与光子的能量转换及其转换效率.结果表明:散射光子频率随电子吸收光子数n的增大而增大,随碰撞非弹性成分ξ的增大而迅速减小.在超强激光场中,当极端相对论性电子与光子发生多光子非线性Compton散射且被光场俘获时,能量转换效率趋于无限大,即电子可以从超强激光场中获得巨大的加速能量.用高速电子束入射并与光子发生多光子非线性Compton散射,是提高非线性Compton散射能量转换效率的重要途径.     

高掺杂浓度掺镱光纤的光子暗化效应

采用光纤激光器和放大器结构方案，观察到了高浓度掺镱光纤（YDF）的光子暗化（Photo-darkening）现象.对激光器阈值和输出功率、放大器输出谱的测量结果表明，光子暗化效应导致了高掺杂浓度YDF的功率转换效率随泵浦作用时间的增加而下降，且下降为单调不可逆过程，但随着泵浦时间的增加，这种下降逐渐变缓、功率转换效率最终可趋于稳定.     

利用叠层一维光子晶体调控半透明有机太阳能电池的性能

利用叠层一维光子晶体提高半透明有机太阳能电池的光电转换效率和调控器件的透视颜色.采用传输矩阵法计算了基于叠层一维光子晶体的半透明有机太阳能电池中活性层的吸收光谱和器件的透过率光谱,进而计算了器件的光电转换效率和透视颜色.研究结果表明,通过合理设计叠层一维光子晶体中顶光子晶体和底光子晶体的禁带中心波长,可以将器件的光电转换效率提高24.4%.此外,通过控制顶光子晶体和底光子晶体的禁带中心波长,可以调控半透明有机太阳能电池的透视颜色,获得透视颜色分别为蓝色、绿色和红色的半透明电池器件.与单层一维光子晶体相比,叠层一维光子晶体可以使器件获得更高的光电转换效率,并能在更大光谱范围内调控器件的透视颜色.     

泵浦光的入射角对参量下转换的影响

利用参量下转换制备相关光子实现对各类探测器的量子效率的定标,是近年来兴起的新型定标技术。由于参量下转换的光子转换效率低,探测器输出信号信噪比小。采用短波激光器泵浦PPLN周期极化性晶体,可获得较大功率的参量光。分析了泵浦光在PPLN晶体端面的入射角对参量光的转换效率、空间分布、参量带宽及晶体周期的影响,并进行了数值模拟。分析发现当泵浦光正入射晶体端面时,参量光功率转换大,带宽小,发散角大;随着泵浦光入射角度逐渐增大,参量下转换的转换效率降低,相关光子的带宽变小,发散角变小且参量光的中心波长的空间位置会发生相对偏移。该研究结果可为相关光子探测、模拟探测器量子效率的高精度定标提供理论依据。     

超强激光与Ar团簇相互作用中X射线的研究

本文主要研究了超强超短激光与Ar团簇相互作用过程中X射线能谱、K壳层光子产额、能量转换效率以及激光对比度对X射线光子产额的影响.实验中得到K壳层的光子产额约为1× 10¹¹/发,能量转换效率约为2.8× 10^-5．同时观测到较强预脉冲离化团簇会导致预电离,产生膨胀等离子体,然而主脉冲与膨胀的等离子体相互作用的强度较未膨胀时降低了,从而导致K壳层光子产额降低,而使用高对比度的激光能增加X射线光子产额.     

纳米结构硅薄膜太阳电池的温度特性研究

温度是影响太阳电池性能的关键因素之一。本文采用光电耦合模型研究了温度对光子晶体型纳米结构薄膜硅太阳电池性能的影响,研究了温度对其光学吸收特性与电学特性的影响。研究发现,随着温度的升高,其光学吸收特性增强,而电学特性降低,整体转换效率降低。光学吸收的增强弥补不了电学特性的减小,因此导致整体转换效率减小。此外,我们还研究了热膨胀系数对纳米结构薄膜太阳电池性能的影响,研究发现,热膨胀系数的影响可以忽略。     

基于KTP晶体的斯塔克啁啾快速绝热通道波长转换

通过近似类比原子绝热布居理论,建立了基于KTP晶体的斯塔克啁啾快速绝热通道理论的波长转换模型,系统研究了晶体耦合调制中的耦合迟延参数和宽度参数、泵浦强度、温度、入射波长等因素对转换效率的影响.结果表明在KTP晶体中能实现入射光能量到出射光能量近乎完全的转换,同时转换过程中中间光能量保持极低.离最优晶体耦合调制参数越远,转换效率越低.转换效率先随泵浦强度的增大不断增大,当转换效率达到最大值,增大泵浦强度对转换效率几乎无影响.温度和入射波长的变化对转换效率影响较小.研究结果表明基于KTP晶体的斯塔克啁啾快速绝热通道理论的波长转换具有很好的鲁棒性.该研究可为紫外到中红外光源的获取以及光子器件的制造提供理论依据.     

基于杂质光伏效应的镍掺杂对砷化镓太阳电池性能的影响

利用杂质光伏效应能够使太阳电池充分利用那些能量小于禁带宽度的太阳光子,从而提高电池的转换效率.为了更好地利用杂质光伏效应提高砷化镓太阳电池的转换效率,本文利用数值方法研究在砷化镓太阳电池中掺入镍杂质以形成杂质光伏太阳电池,分析掺镍对电池的短路电流密度、开路电压以及转换效率的影响;同时,探讨电池的陷光结构对杂质光伏太阳电池器件性能的影响.结果表明:利用杂质光伏效应掺入镍杂质能够增加子带光子的吸收,使得电池转换效率提高3.32%;转换效率的提高在于杂质光伏效应使电池的红外光谱响应得到扩展;另外,拥有良好的陷光结构是取得好的杂质光伏效应的关键.由此得出:在砷化镓太阳电池中掺镍形成杂质光伏太阳电池是一种能够提高砷化镓太阳电池转换效率的新方法.     

共振增强的光学参变下转换

多光子纠缠态是量子通讯网络中的重要资源,光与二阶非线性介质相互作用的自发参变下转换过程是目前制备多光子态较成熟的方案之一.尽管脉冲光可以提高非线性转换效率并简化通信协议,但是进一步增强光与介质间的相互作用对提高多光子的产生效率依然必要.设计了飞秒脉冲激光谐振腔系统,在不改变脉冲重复频率和频率梳结构的情况下,提高了下转换...     

压力与温度双参量传感优化系统的研制

研究了一种基于管式弹性应变敏感元件的光纤光栅传感器结构。利用双光纤布拉格光栅(FBG)产生双反射峰．对压力和温度进行了同时区分测量。在压力为0～20MPa,温度为20～150℃的范围内,布拉格反射波长对应压力与温度的变化均呈现良好的线性响应特性,响应灵敏度分别为0．089nm／MPa和0．024nm／C^-。压力温度双参量系数矩阵的实验拟合值与理论计算值之差仅占理论计算值的1．8％。该方法与标准测量方法比较,压力的准确度为0．47％;温度的准确度为0．74％。该方法还较好地削减了压力与温度交叉敏感的影响,按压力与温度测量的最大量限计算,温度对压力交叉影响的误差仅为0．16％。     

Super-pressed and super-cooled (?) P(EO)20LiBETI

High pressure conductivity measurements have been carried out on P(EO)₂₀LiBETI from 295 K to 368 K. The decrease of electrical conductivity with pressure is larger in the partially crystalline phase (low temperature and low pressure or high temperature and high pressure) than in the fully amorphous phase (high temperature and low pressure). It is found that if the phase transition is approached from the crystalline phase (decreasing pressure), the pressure of the phase transition varies from 0 to 0.23 GPa as the temperature increases from 336 K to 358 K. The shift of the phase transition temperature with pressure is approximately the same as the shift of the glass transition temperature with pressure for pure PEO. This can be understood in terms of the defect diffusion model. If the material is above 336 K and is in the fully amorphous phase, after pressure is increased above the critical pressure, the material remains in the amorphous phase for extended periods of time before transforming to the partially crystalline phase. This is reminiscent of a super-pressed state but may be an indication of slow crystallization kinetics.     

Hydrostatic pressure and temperature effects on the electronic energy levels of a spherical quantum dot placed at the center of a nano-wire

The effect of pressure and temperature on the electronic structure of an InAs spherical quantum dot located at the center of a GaAs cylindrical nano-wire have been determined using finite element method, within the effective mass approximation. The energy levels and transition energies are numerically calculated as a function of the dot radius, pressure and temperature. It is shown that the pressure and temperature effects are significant and should be considered in the study of low-dimensional semiconducting systems. The results show that; energy levels (i) decrease as the dot radius increases (ii) decrease as the pressure increases and (iii) increase as the temperature increases. For very small dot radii, the energy levels show unusual behavior, such that the energy levels increase as the pressure increases. We also found that the transition energy (i) increases as the dot size decreases (ii) increases as the pressure increases and (iii) decreases as the temperature increases.     

微波脉冲氮气等离子体发射光谱测量

通过发射光谱测量和拟合不同的微波脉宽和气压下C波段微波放电的氮气等离子体振动温度、转动温度和电子激发温度。气压在266~400Pa时,等离子体的振动温度为(2700±100)K,电子激发温度为(0.32±0.015)eV,转动温度随脉宽增加而上升,实验中测得的最大转动温度为370K。偏离266~400Pa时,振动温度和电子激发温度同时出现了下降的趋势,而转动温度出现了上升的趋势。这意味着电子激发温度和振动温度具有很强的关联性。     

光子晶体光纤温度压力传感器

提出了一种在高温环境下同时测量温度和气压的光子晶体光纤温度压力传感器.在普通单模光纤和光子晶体光纤之间熔接一段空心光纤构成干涉结构.空心光纤段构成非本征法布里-珀罗干涉仪,利用光子晶体光纤的微孔与外界相通,通过气体折射率变化来测量环境中的气压变化;光子晶体光纤段构成本征法布里-珀罗干涉仪,利用热膨胀效应和热光效应来测量环境中的温度.传感器的解调通过自制的白光干涉解调仪实现,实验通过测量腔长得到被测环境的温度和气压.在不同温度和气压环境下,对腔长分别为306μm和1535μm的温度压力光纤传感器进行连续测量.实验结果表明,传感器能够在28~800℃的温度下和0~10 MPa的气压下稳定工作,测量范围内温度灵敏度可达17.4 nm/℃,压力灵敏度随温度增加而降低,在28℃时可达1460.5 nm/MPa.     

温度和压力对Au反射特性影响及动高压下的测温应用分析

基于金属电子气模型,进行了温度、压力对Au反射率变化影响的研究与分析。利用DAC装置开展了压力对Au反射率变化测量实验,以及激光加热的动态温升条件下温度对Au反射率变化测量实验,获得了探测光束波长为488 nm条件下,温度(室温至350 ℃)和压力(11 GPa范围内)对Au反射特性影响的实验结果。结果表明:在11 GPa压力范围内,与温度因素相比,压力对Au的反射率变化影响可忽略;Au对488 nm波长激光的反射率变化趋势为单调递增,变化幅值达约10%,且具有反射率与温度的一一对应特性。通过动高压加载下材料温度瞬态测量要求分析,认为基于Au在488 nm波长下的反射变化特性,可建立一种适用于动高压加载下低温段(低于1000 K)的瞬态测温方法,用于解决材料动高压领域的瞬态测温技术难点。     

Magnetic contribution to the Gibbs energy of elements versus temperature and pressure

A model for the pressure and temperature dependence of the magnetic contributions to the Gibbs energy of ferromagnetic and antiferromagnetic elements is presented. These contributions are described by three parameters: (1) a critical temperature which is represented by the Curie temperature for ferromagnetic elements or Néel temperature for antiferromagnetic elements, (2) the pressure dependence of that critical temperature, (3) the average magnetic moment per atom. Using thermal expansion data, all these parameters and consequently the pressure and temperature dependence of the magnetic contribution can be calculated. Nickel, a ferromagnetic element, is used as an example.     

Polymorphic transformations in nanostructured anatase (TiO2) under high-pressure shock compression

The action of dynamic pressure and temperature on polymorphic transformations in nanostructured (grain size of 8–20 nm) anatase (TiO₂) is studied. The dynamic pressure of a loading pulse (10–45 GPa) is measured with a manganin gauge. The temperature of shock-compressed specimens, which is varied by varying the initial temperature and initial porosity, is found to fall into the range 500–2500 K. It is shown that as the temperature and shock compression pressure rise, the nanostructured anatase turns into a nanoanatase-nanocolumbite or columbite-rutile mixture or into almost impurity-free (pure) nanocolumbite or impurity-free microcrystalline rutile.     

Pressure-induced colossal piezoresistance effect and the collapse of the polaronic state in the bilayer manganite (La(0.4)Pr(0.6))(1.2)Sr(1.8)Mn2O7

We have investigated the effect of hydrostatic pressure as a function of temperature on the resistivity of a single crystal of the bilayer manganite (La(0.4)Pr(0.6))(1.2)Sr(1.8)Mn(2)O(7). Whereas a strong insulating behaviour is observed at all temperatures at ambient pressure, a clear transition into a metallic-like behaviour is induced when the sample is subjected to a pressure (P) of ~1.0 GPa at T < 70 K. A huge negative piezoresistance ~10(6) in the low temperature region at moderate pressures is observed. When the pressure is increased further (5.5 GPa), the high temperature polaronic state disappears and a metallic behaviour is observed. The insulator to metal transition temperature exponentially increases with pressure and the distinct peak in the resistivity that is observed at 1.0 GPa almost vanishes for P > 7.0 GPa. A modification in the orbital occupation of the e(g) electron between 3d(x(2)-y(2)) and 3d(z(2)-r(2)) states, as proposed earlier, leading to a ferromagnetic double-exchange phenomenon, can qualitatively account for our data.     

Temperature correction of PSP measurement using dual-luminophor coating

We developed a dual-luminophor pressure/temperature sensitive paint (DPTSP) to correct the temperature dependence of pressure-sensitive paint. The DPTSP is composed of two sensor molecules, PtTFPP and Rhodamine B (RhB), and Poly-IBM-co-TFEM as a binder. Temperature was determined from the image of RhB, and the temperature dependence of PtTFPP was corrected using the calculated temperature. To validate the capability of DPTSP for temperature correction, the pressure field on a delta wing model was measured by the DPTSP measurement system. The pressure values obtained with DPTSP were in good quantitative agreement with pressure tap data. It has been validated that DPTSP is effective in correcting the temperature dependence of PSP.