首页 | 官方网站   微博 | 高级检索  
相似文献
 共查询到20条相似文献,搜索用时 31 毫秒
1.
The aim of this study was to estimate the current concentrations of 90Sr and 137Cs in the urine of Finnish people and to estimate the doses. Two to three daily urine samples were collected from 18 adult Finnish volunteers in connection with studies of 137Cs body burdens in 1999-2001. The 90Sr activities in urine varied between 1.4 and 11 mBq l(-1). The 137Cs activity in urine varied between 0.36 and 56 Bq l(-1). The daily urinary excretion was found to be 4.8-17 mBq for 90Sr and 0.81-68 Bq for 137Cs. Assuming that the daily 90Sr intake was constant and that 18% of the ingested activity was excreted in urine, the mean intake in the investigated group would vary between 27 and 96 mBq d(-1). Based on these estimated intake values, the respective annual effective internal doses from 90Sr and 90Y varied from 0.3 to 1.0 microSv and from 137Cs from 4 to 350 microSv during the sampling period.  相似文献   

2.
An estimate of the tritium dose to the public in the vicinity of the heavy water research reactor facility at AECL-Chalk River Laboratories, Ontario, Canada, has largely been accomplished from analyses on regularly-collected samples of air, precipitation, drinking water and foodstuffs (pasture, fruit, vegetables and milk) and environmental dose models. To increase the confidence with which public doses are calculated, tritium doses were estimated directly from the ratio of tritiated species in urine samples from members of the general public. Single cumulative 24 h urine samples from a few adults living in the vicinity of the heavy-water research reactor facility at Chalk River Laboratories, Canada were collected and analysed for tritiated water and organically bound tritium. The participants were from Ottawa (200 km east), Deep River (10 km west) and Chalk River Laboratories. Tritiated water concentrations in urine ranged from 6.5 Bq.l-1 for the Ottawa resident to 15.9 Bq.l-1 for the Deep River resident, and were comparable to the ambient levels of tritium-in-precipitation at their locations. The ultra-low levels of organically bound tritium in urine from these same individuals were measured by 3He-ingrowth mass spectrometry and were 0.06 Bq.l-1 (Ottawa) and 0.29 Bq.l-1 (Deep River). For Chalk River Laboratories workers, tritiated water concentrations in urine ranged from 32 Bq.l-1 to 9.2 x 10(4) Bq.l-1, depending on the ambient levels of tritium in their workplace. The organically bound tritium concentrations in urine from the same workers were between 0.08 Bq.l-1 and 350 Bq.l-1. With a model based on the ratio of tritiated water to organically bound tritium in urine, the estimated dose arising from organically bound tritium in the body for the Ottawa and Deep River residents was about 26% and 50%, respectively, of the body water tritium dose. The workers in a reactor building at Chalk River Laboratories had less than 10% dose contribution from organically bound tritium, but had higher overall tritium dose due to frequent intakes of tritiated water vapour in the workplace. The results of this study suggest that most of the tritium dose to workers at Chalk River and general population near Chalk River is the result of tritiated water intakes and not due to dietary intake of organically bound tritium.  相似文献   

3.
The activity concentrations of (226)Ra and (228)Ra in drinking water were determined in water samples from 176 drilled wells. (226)Ra activity concentrations were in the range of <0.01-1.0 Bq l(-1) and (228)Ra activity concentrations in the range of <0.03-0.3 Bq l(-1). The mean activity concentration of (226)Ra and (228)Ra were 0.041 and 0.034 Bq l(-1), respectively. High radium activity concentrations in drinking water were rare. Only 2-4% of the drilled wells exceeded a (226)Ra concentration of 0.5 Bq l(-1) and 1-2% of the wells exceeded a (228)Ra concentration of 0.2 Bq l(-1). These are the activity concentrations that cause a 0.1 mSv annual effective dose for users of drinking water. The maximum annual effective doses from (226)Ra and (228)Ra for users of drilled wells were 0.21 mSv, and 0.16 mSv respectively. The elevated activity concentrations of (226)Ra and (228)Ra did not occur simultaneously in the same groundwaters and the correlation between (226)Ra and (228)Ra was small.  相似文献   

4.
Tritium content in air moisture, soil water, rain water and plant water samples collected around the Kaiga site, India was estimated and the scavenging ratio, wet deposition velocity and ratio of specific activities of tritium between soil water and air moisture were calculated and the results are interpreted. Scavenging ratio was found to vary from 0.06 to 1.04 with a mean of 0.46. The wet deposition velocity of tritium observed in the present study was in the range of 3.3E-03 to 1.1E-02 m s(-1) with a mean of 6.6E-03 m s(-1). The ratio of specific activity of tritium in soil moisture to that in air moisture ranged from 0.17 to 0.95 with a mean of 0.49. The specific activity of tritium in plant water in this study varied from 73 to 310 Bq l(-1). The present study is very useful for understanding the process and modelling of transfer of tritium through air/soil/plant system at the Kaiga site.  相似文献   

5.
The activity concentrations of naturally occurring radionuclides ((238)U, (226)Ra, (228)Ra, (210)Pb and (40)K) in Jordanian phosphate ore, fertilizer material and phosphogypsum piles were investigated. The results show the partitioning of radionuclides in fertilizer products and phosphogypsum piles. The outcome of this study will enrich the Jordanian radiological map database, and will be useful for an estimation of the radiological impact of this industrial complex on the immediate environment. The activity concentration of (210)Pb was found to vary from 95 +/- 8 to 129 +/- 8 Bq kg(-1) with a mean value of 111 +/- 14 Bq kg(-1) in fertilizer samples, and from 364 +/- 8 to 428 +/- 10 Bq kg(-1) with a mean value of 391 +/- 30 Bq kg(-1) in phosphogypsum samples; while in phosphate wet rock samples, it was found to vary between 621 +/- 9 and 637 +/- 10 Bq kg(-1), with a mean value of 628 +/- 7 Bq kg(-1). The activity concentration of (226)Ra in fertilizer samples (between 31 +/- 4 and 42 +/- 5 Bq kg(-1) with a mean value of 37 +/- 6 Bq kg(-1)) was found to be much smaller than the activity concentration of (226)Ra in phosphogypsum samples (between 302 +/- 8 and 442 +/- 8 Bq kg(-1) with a mean value of 376 +/- 62 Bq kg(-1)). In contrast, the activity concentration of (238)U in fertilizer samples (between 1011 +/- 13 and 1061 +/- 14 Bq kg(-1) with a mean value of 1033 +/- 22 Bq kg(-1)) was found to be much higher than the activity concentration of (238)U in phosphogypsum samples (between 14 +/- 5 and 37 +/- 7 Bq kg(-1) with a mean value of 22 +/- 11 Bq kg(-1)). This indicates that (210)Pb and (226)Ra show similar behaviour, and are concentrated in phosphogypsum piles. In addition, both isotopes enhanced the activity concentration in phosphogypsum piles, while (238)U enhanced the activity concentration in the fertilizer. Due to the radioactivity released from the phosphate rock processing plants into the environment, the highest collective dose commitment for the lungs was found to be 1.02 person nGy t(-1). Lung tissue also shows the highest effect due the presence of (226)Ra in the radioactive cloud (0.087 person nGy t(-1)).  相似文献   

6.
Natural radioactivity in drinking water was determined in population-based random study of 472 private wells. The mean concentrations of (222)Rn, (226)Ra, (234)U, (238)U, (210)Pb and (210)Po in drilled wells were 460, 0.05, 0.35, 0.26, 0.04 and 0.05 Bq l(-1), and in wells dug in the soil were 50, 0.016, 0.02, 0.015, 0.013 and 0.007 Bq l(-1), respectively. Approximately 10% of the drilled wells exceeded a radon concentration of 1000 Bq l(-1) and 18% a uranium concentration of 15 microg l(-1). The mean annual effective dose from natural radionuclides for a drilled well user was 0.4 mSv and 0.05 mSv for a user of a well dug in the soil. The effective dose arising from (222)Rn was 75% of the total of all natural radionuclides for drilled well users. As regards long-lived radionuclides, (210)Po and (210)Pb caused the largest portion of the effective dose. The dose arising from (238)U, (234)U and (226)Ra was only 8% of the total of all natural radionuclides.  相似文献   

7.
Measurements of (222)Rn activity concentration were carried out in 39 samples collected from the domestic and drinking water sources used in the island and mainland of Penang, northern peninsular, Malaysia. The measured activity concentrations ranged from 7.49 to 26.25 Bq l(-1), 0.49 to 9.72 Bq l(-1) and 0.58 to 2.54 Bq l(-1) in the raw, treated and bottled water samples collected, respectively. This indicated relatively high radon concentrations compared with that from other parts of the world, which still falls below the WHO recommended treatment level of 100 Bq l(-1). From this data, the age-dependent associated committed effective doses due to the ingestion of (222)Rn as a consequence of direct consumption of drinking water were calculated. The committed effective doses from (222)Rn resulting from 1 y's consumption of these water were estimated to range from 0.003 to 0.048, 0.001 to 0.018 and 0.002 to 0.023 mSv y(-1), for age groups 0-1, 2-16 and >16 y, respectively.  相似文献   

8.
The effect of ionising radiation on biological systems depends among other factors on time and place of exposure and population involved. Socio-economic factors in human daily activities have subjected humans to certain environmental health risks. In most cases the risk appears to be higher outdoors than indoors. In order to quantify the radiation exposure levels to individuals in the outdoors in areas with high human and vehicular densities, roadside soil samples were collected from major bus stops and round-about in the metropolis of Ibadan and were analysed for their activity concentration levels using gamma-ray spectrometry. The 40K activity concentration ranged between 96.1 and 336.5 Bq kg(-1) with a mean of 219.8 +/- 71.4 Bq kg(-1); 238U was in the range of 10.2-40.7 Bq kg(-1) with a mean of 20.3 +/- 6.9 Bq kg(-1) while that of 232Th ranged between 13.3 and 29.7 Bq kg(-1) with a mean of 21.2 +/- 5.3 Bq kg(-1). The total gamma absorbed dose rates in air ranged between 17.2 and 41.8 nGy h(-1) with an average of 32.0 +/- 5.8 nGy h(-1). The gamma absorbed dose rates at the roadsides in traffic density areas were found to be lower when compared with previously reported values in natural and undisturbed locations in non-traffic density areas in the city.  相似文献   

9.
In the first part of this work, the potential alpha energy concentration (PAEC) of radon progeny, the equilibrium factor (F), the activity concentration of 222Rn gas (Co) and the unattached fraction (fp), were determined in 15 living rooms at El-Minia City, Egypt. The activity size distribution of (214)Pb was measured by using a low pressure Berner impactor. Based on the parameters of that distribution the total effective dose through the human lung was evaluated by using a dosimetric model calculation of ICRP. An electrostatic precipitation method was used for the determination of 222Rn gas concentration. The mean activity concentration of 222Rn gas (Co) was found to be 123 +/- 22 Bq m(-3). A mean unattached fraction (fp) of 0.11 +/- 0.02 was obtained at a mean aerosol particle concentration (Z) of (3.0 +/- 0.21) x 10(3) cm(-3). The mean equilibrium factor (F) was determined to be 0.35 +/- 0.03. The mean PAEC was found to be 37 +/- 8.1 Bq m(-3). The activity size distribution of (214)Pb shows mean activity median diameter of 290 nm with mean geometric standard deviation (sigma) of 2.45. At a total deposition fraction of approximately 23% the total effective dose to the lung was determined to be approximately 1.2 mSv. The second part of this paper deals with a study of natural radionuclide contents of samples collected from the building materials of those rooms under investigation given in part one of this paper. Analyses were performed in Marinelli beakers with a gamma multichannel analyser provided with a NaI(Tl) detector. The samples have revealed the presence of the uranium-radium and thorium radioisotopes as well as (40)K. Nine gamma-lines of the natural radioisotopes that correspond to 212Pb, 214Pb, 214Bi, 228Ac, 40K and 208Tl were detected and measured. The activity concentrations of 226Ra, 232Th and 40K were determined with mean specific activities of 65 +/- 22, 35 +/- 12 and 150 +/- 60 Bq kg(-1), respectively. These activities amount to a radium equivalent (Ra(eq)) of 126 Bq kg(-1) and to a mean value of external hazard index of 0.34.  相似文献   

10.
A new radioanalytical method was developed for rapid determination of (226)Ra in human urine samples. The method is based on organic removal and decolourisation of a urine sample by a polymeric (acrylic ester) solid phase sorbent material followed by extraction and preconcentration of (226)Ra in an organic solvent using a dispersive liquid-liquid microextraction technique. Radiometric measurement of (226)Ra was carried out using a liquid scintillation counting instrument. The minimum detectable activity for the method (0.15 Bq l(-1)) is lower than the required sensitivity of 0.2 Bq l(-1) for (226)Ra in human urine samples as defined in the requirements for radiation emergency bioassay techniques for the public and first responders based on the dose threshold for possible medical attention recommended by the International Commission on Radiological Protection (ICRP). The accuracy (expressed as relative bias, B(r)) and repeatability of the method (expressed as relative precision, S(B)) evaluated at the reference level (2 Bq l(-1)) were found to be -4.5 and 2.6 %, respectively. The sample turnaround time was <5 h for a single urine sample and <20 h for a batch of six urine samples. With the fast sample turnaround time combined with the potential to carry out the analysis in a field deployable mobile laboratory, the newly developed method can be used for emergency radiobioassay of (226)Ra in human urine samples following a radiological or nuclear accident.  相似文献   

11.
Five hot springs called 'Abegarm-e-Mahallat', located in the central part of Iran, have a mean water temperature of 46 +/- 1 degrees C and are used by visitors as spas. This is an area of high natural radiation background due to the presence of (226)Ra and its decay products in the deposited travertine (CaCO(3)). The mean concentration of (226)Ra in these hot springs, measured by the emanation method, ranged from 0.48 +/- 0.05 to 1.35 +/- 0.13 Bq l(-1). (222)Rn concentrations measured in the hot springs using a liquid scintillation counter ranged from 145 +/- 37 to 2731 +/- 98 Bq l(-1). Mean radon concentrations in air were 487 +/- 160 and 15.4 +/- 2.7 Bq m(-3) for indoor and outdoor, respectively. Radiation levels above that of normal background ( approximately 100 nGy h(-1)) were mainly limited to the Quaternary travertine formations in the vicinity of the hot springs. The results of environmental radiological studies in this region are presented and discussed.  相似文献   

12.
The vertical distribution of natural radionuclides ((232)Th decay, (238)U decay, (40)K and (210)Pb) was assessed in sediment cores collected from the Amvrakikos Gulf, (Ionian Sea, Western Greece). Two collection stations were selected, the first at the western part of the Gulf near Preveza Strait (13A station) and the other near the centre of the Gulf (13B station). Activity concentrations were measured by means of gamma-ray spectrometry using high-purity germanium (HPGe) detectors installed at two national laboratories. The activity concentration of (226)Ra was found in a range from 10 to 20 Bq kg(-1), while the activity concentration of (222)Rn daughters ((214)Pb, (214)Bi) ranged from 6 to 20 Bq kg(-1). The activity concentration of (228)Ac varied from 20 to 28 Bq kg(-1), while (220)Rn daughters ((212)Pb, (208)Tl) from 7 to 35 Bq kg(-1). As concerns (40)K and (210)Pb, their activities varied from 400 to 830 Bq kg(-1) and from 11 to 360 Bq kg(-1), respectively. Also, the data of (210)Pb were utilised in the calculations of the sedimentation rate along the sediment cores. Both locations were characterised by a consistent pattern with the average rates of 0.55 ± 0.02 and 0.32 ± 0.02 cm y(-1), corresponding to 13A and 13B stations, respectively. Finally, the measurements constituted the basis of the first reported database concerning the radiological condition of the Gulf and which can be reclaimed as reference values in future monitoring studies.  相似文献   

13.
A survey was carried out to determine activity concentration levels and associated dose rates from the naturally occurring radionuclides 232Th, 238U and 40K, in the various geological formations of Cyprus, by means of high-resolution gamma ray spectrometry. A total of 115 representative soil samples were collected from all over the bedrock surface of the island, based on the different lithological units of the study area, sieved through a fine mesh, sealed in 1000 ml plastic Marinelli beakers and measured in the laboratory with respect to gamma radioactivity for a counting time of 18-h each. From the measured spectra, activity concentrations were determined for 232Th (range from 1.0 x 10(-2) to 39.8 Bq kg(-1)), 238U (from 1.0 x 10(-2) to 39.3 Bq kg(-1)) and (40)K (from 4.0 x 10(-2) to 565.8 Bq kg(-1)). Gamma absorbed dose rates in air outdoors were calculated to be in the range from 1.1 x 10(-2) to 51.3 nGy h(-1), depending on the geological features, with an overall mean value of 8.7 nGy h(-1) and a standard deviation of 8.4 nGy h(-1). This value is by a factor of about seven below the corresponding population-weighted world-averaged value of 60 nGy h(-1) and one of the lowest that has been reported from similar investigations worldwide. Assuming a 20% occupancy factor, the corresponding effective dose rates outdoors equivalent to the population were calculated to be between 1.3 x 10(-2) and 62.9 microSv y(-1), with an arithmetic mean value of 10.7 microSv y(-1) and a standard deviation of 10.3 microSv y(-1).  相似文献   

14.
A group of subjects of Bangladeshi adults from both sexes were studied for internal radioactivity and effective dose by measuring the whole-body activity of naturally occurring (40)K using a whole-body counter. The mean activity concentration in the whole body and effective dose due to naturally occurring (40)K for the average male were found to be 2.0 +/- 0.4 Bq.g(-1) and 100 +/- 26 microSv.y(-1), respectively and those for the average female were 1.7 +/- 0.3 Bq.g(-1) and 100 +/- 20 microSv.y(-1), respectively. The mean activity concentration in the whole body and effective dose for both sexes were 1.9 +/- 0.4 Bq.g(-1) and 100 +/- 25 microSv.y(-1), respectively. The effective dose from (40)K for subjects is below the value reported by the UNSCEAR.  相似文献   

15.
The present work was aimed at the establishment of baseline radioactive data in the proposed Lambapur and Peddagattu uranium mining areas in the Andhra Pradesh state, India. The background concentrations of naturally occurring radioactivity in the near-surface soils of the study areas were estimated and the results were analysed. The (238)U concentration in the near-surface soil of the study area was found to vary from 100 to 176 Bq kg(-1), with a mean of 138±24 Bq kg(-1). (232)Th in the study area soils was found to vary between 64 and 116 Bq kg(-1), with a mean of 83±15 Bq kg(-1). The (40)K concentration was found to vary between 309 and 373 Bq kg(-1), with a mean of 343±20 Bq kg(-1). The mean natural background radiation levels were also measured with thermoluminescence (TL) dosimetry technique and with a μR-survey meter, in the villages of the study area. Dose rates measured by TL are found to vary from 1287 to 3363 μGy y(-1), with a mean of 2509 ± 424 μGy y(-1). The dose rates measured in the same villages with a μR-survey meter were found to be in the range of 1211-3255 μGy y(-1), with a mean of 2524 ± 395 μGy y(-1). The mean radiation levels in the study area are found to be relatively high when compared with (Indian) national and international averages. Correlations among radon, thoron and gamma dose rates were found to be poor. The pre-operational data produced in this work will be useful for comparison with future radiation levels during the proposed uranium mining operations.  相似文献   

16.
Long-term (circa 3 months) simultaneous measurements of indoor concentrations of thoron gas, airborne thoron progeny and radon were made using passive alpha track detectors in 205 dwellings in Ireland during the period 2007-09. Thoron progeny concentrations were measured using passive deposition monitors designed at the National Institute of Radiological Sciences (NIRS), Japan, whereas thoron gas concentrations were measured using Raduet detectors (Radosys, Budapest). Radon concentrations were measured in these dwellings by means of NRPB/SSI type alpha track radon detectors as normally used by the Radiological Protection Institute of Ireland (RPII). The concentration of thoron gas ranged from <1 to 174 Bq m(-3) with an arithmetic mean (AM) of 22 Bq m(-3). The concentration of radon gas ranged from 4 to 767 Bq m(-3) with an AM of 75 Bq m(-3). For radon, the estimated annual doses were 0.1 (min), 19.2 (max) and 1.9 (AM) mSv y(-1). The concentration of thoron progeny ranged from <0.1 to 3.8 Bq m(-3) [equilibrium equivalent thoron concentration (EETC)] with an AM of 0.47 Bq m(-3) (EETC). The corresponding estimated annual doses were 2.9 (max) and 0.35 (mean) mSv y(-1). In 14 or 7% of the dwellings, the estimated doses from thoron progeny exceeded those from radon.  相似文献   

17.
Radon activity concentrations have been measured in 53 from a total of 66 public primary schools throughout of Patras, Greece, during December 1999 to May 2000 using solid-state nuclear track detectors (LR-115 II). The indoor radon levels in the classrooms were generally low, ranging from 10 to 89 Bqm(-3). The mean (arithmetic mean) indoor concentration was 35 +/- 17 Bq m(-3) and an estimated annual effective dose of 0.1 +/- 0.1 mSv y(-1) was calculated for students and 0.2 +/- 0.1 mSv y(-1) for teachers, assuming an equilibrium factor of 0.4 and occupancy factor of 12 and 14%, respectively. The research was also focused on parameters affecting radon concentration levels such as floor number of the classrooms and the age of the buildings in relation to building materials.  相似文献   

18.
The natural background dose and the radium equivalent due to the natural radioactivity levels in rocks and sediments collected around Ikogosi warm spring, Nigeria, has been determined in this study using a highly sensitive HpGe detector. The mean activity concentration of (40)K, (226)Ra and (228)Ac were measured to be 585.50 +/- 17.40 Bq kg(-1), 66.91 +/- 5.23 Bq kg(-1) and 48.91 +/- 2.10 Bq kg(-1), respectively, in rock samples while in sediment samples the activity concentrations were found to be 113.89 +/- 5.64 Bq kg(-1) for (40)K, 21.47 +/- 5.14 Bq kg(-1) for (226)Ra and 14.20 +/- 1.07 Bq kg(-1) for (228)Ac. This mean values give rise to average absorbed dose rate of 85.87 nGy h(-1) at a distance of 1.0 m above the ground level and a mean human effective dose equivalent of 0.53 man Sv y(-1) for rock samples. A radium equivalent of 50.55 Bq kg(-1) was measured for the sediment samples. The radium equivalent value is far less than the 370 Bq kg(-1) limit for materials that can be used as building materials while the human effective dose equivalent falls below the world average background dose of 2.4 man Sv y(-1).  相似文献   

19.
This paper presents the results of radon ((222)Rn) concentration measurements in municipal supply drinking water in metropolitan Lahore city of Pakistan and evaluation of consequent radiological effects. In this respect, water samples were collected in all nine municipal towns of Lahore city and analysed employing a high-resolution gamma spectrometric system. Radon concentration varied from 2.0 +/- 0.3 to 7.9 +/- 2.1 Bq l(-1). Mean value of annual effective dose for an individual consumer was assessed to be 16.5 +/- 12.8 microSv y(-1). (222)Rn mean concentration measured in this study is comparable with the reported values for drinking water determined worldwide and found to be less than the limit of 100 Bq l(-1) recommended by the World Health Organisation for public water supplies. The results of this study may be helpful in establishing background levels of radon in drinking water that could be used not only to distinguish additional contributions when a contamination event occurs but also to implement water quality standards by the concerned authorities to maintain radioactive contamination free drinking water supplies for the population.  相似文献   

20.
Radon and gamma dose rate measurements have been performed in 561 workplaces in 19 prefectures of Greece. The distribution of radon concentration can be well described by a log-normal distribution. Most of the radon concentrations are between 50 and 200 Bq m(-3) with an arithmetic mean of 123 Bq m(-3). The maximum measured value of radon gas concentration is 695 Bq m(-3). About 10% of the workplaces exceed 200 Bq m(-3). Only a small fraction ( approximately 1%) of workplaces exceed the European Commission action level (400 Bq m(-3)). Despite the relative small fraction of workplaces which exceed the value of 400 Bq m(-3), it is clear from the results of the present work that for certain prefectures, further and more extensive research is needed.  相似文献   

设为首页 | 免责声明 | 关于勤云 | 加入收藏

Copyright©北京勤云科技发展有限公司    京ICP备09084417号-23

京公网安备 11010802026262号