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1.
This study investigated the deposition of coke in a fractionation tower following thermal cracking of heavy feedstocks. A simple microscopic technique was used to determine whether the coke formed in situ in the fractionator or was formed elsewhere (e.g. in the reactor vessel) and was subsequently entrained in the vapour phase. The reflectance of coke types, mode of occurrence, and distributions from the bottom to the top of the fractionator were used to interpret the range of temperatures responsible for coke formation. Both isotropic and anisotropic (mosaic) coke was observed in the samples. The anisotropic textural features indicated that asphaltenes carry-over was a minor problem and that the vast majority of the isotropic coke precursors were the maltenes present in the gas phase that entered the fractionator. The formation of perfectly spherical mesophase was attributed to the gas oil stream itself used to quench the vapours exiting the thermal cracking vessel. Microscopic evidence, along with metals concentration in the coke at various locations of the operation provided useful information as to the nature of the coke precursors. 相似文献
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This work develops a transfer learning (TL) framework for modeling and predictive control of nonlinear systems using recurrent neural networks (RNNs) with the knowledge obtained in modeling one process transferred to another. Specifically, transfer learning uses a pretrained model developed based on a source domain as the starting point, and adapts the model to a target process with similar configurations. The generalization error for TL-based RNN (TL-RNN) is first derived to demonstrate the generalization capability on the target process. The theoretical error bound that depends on model capacity and the discrepancy between source and target domains is then utilized to guide the development of pretrained models for improved model transferability. Subsequently, the TL-RNN model is utilized as the prediction model in model predictive controller (MPC) for the target process. Finally, the simulation study of chemical reactors via Aspen Plus Dynamics is used to demonstrate the benefits of transfer learning. 相似文献
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This paper proposes a switching multi-objective model predictive control (MOMPC) algorithm for constrained nonlinear continuous-time process systems. Different cost functions to be minimized inMPC are switched to satisfy different performance criteria imposed at different sampling times. In order to ensure recursive feasibility of the switching MOMPC and stability of the resulted closed-loop system, the dual-mode control method is used to design the switching MOMPC controller. In this method, a local control law with some free-parameters is constructed using the control Lyapunov function technique to enlarge the terminal state set of MOMPC. The correction termis computed if the states are out of the terminal set and the free-parameters of the local control laware computed if the states are in the terminal set. The recursive feasibility of the MOMPC and stability of the resulted closed-loop system are established in the presence of constraints and arbitrary switches between cost functions. Finally, implementation of the switching MOMPC controller is demonstrated with a chemical process example for the continuous stirred tank reactor. 相似文献
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Maciej ?awryńczuk 《Chemical engineering science》2011,(21):5253
For nonlinear processes the classical model predictive control (MPC) algorithm, in which a linear model is used, usually does not give satisfactory closed-loop performance. In such nonlinear cases a suboptimal MPC strategy is typically used in which the nonlinear model is successively linearised on-line for the current operating point and, thanks to linearisation, the control policy is calculated from a quadratic programming problem. Although the suboptimal MPC algorithm frequently gives good results, for some nonlinear processes it would be beneficial to further improve control accuracy. This paper details a computationally efficient nonlinear MPC algorithm in which a neural model is linearised on-line along the predicted trajectory in an iterative way. The algorithm needs solving on-line only a series of quadratic programming problems. Advantages of the discussed algorithm are demonstrated in the control system of a high-purity ethylene–ethane distillation column for which the classical linear MPC algorithm does not work and the classical suboptimal MPC algorithm is slow. It is shown that the discussed algorithm can give practically the same control accuracy as the algorithm with on-line nonlinear optimisation and, at the same time, the algorithm is significantly less computationally demanding. 相似文献
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Fátima Barceló-Rico José M. Gozálvez-ZafrillaAsunción Santafé-Moros 《Chemical Engineering Research and Design》2011,89(1):107-115
This paper presents a methodology for the design of a fuzzy controller applicable to continuous processes based on local fuzzy models and velocity linearizations. It has been applied to the implementation of a fuzzy controller for a continuous distillation tower. Continuous distillation towers can be subjected to variations in feed characteristics that cause loss of product quality or excessive energy consumption. Therefore, the use of a fuzzy controller is interesting to control process performance.A dynamic model for continuous distillation was implemented and used to obtain data to develop the fuzzy controller at different operating points. The fuzzy controller was built by integration of linear controllers obtained for each linearization of the system. Simulation of the model with controller was used to validate the controller effectiveness under different scenarios, including a study of the sensibility of some parameters to the control.The results showed that the fuzzy controller was able to keep the target output in the desired range for different inputs disturbances, changing smoothly from a predefined target output to another. The developed techniques are applicable to more complex distillation systems including more operating variables. 相似文献
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We study the control of a solution copolymerization reactor using a model predictive control algorithm based on multiple piecewise linear models. The control algorithm is a receding horizon scheme with a quasi-infinite horizon objective function which has finite and infinite horizon cost components and uses multiple linear models in its predictions. The finite horizon cost consists of free input variables that direct the system towards a terminal region which contains the desired operating point. The infinite horizon cost has an upper bound and takes the system to the final operating point. Simulation results on an industrial scale methyl methacrylate vinyl acetate solution copolymerization reactor model demonstrate the ability of the algorithm to rapidly transition the process between different operating points. 相似文献
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为算出一座焦炭塔堵焦阀接管处的管端推力(矩)数值及塔体接管部位的应力,特选用等值刚度法FAOP及有限元法MSC两个标准程序分别对该塔的高温进油管系及塔体接管部位进行了柔性分析及应力计算。为了验证计算方法的正确性,还在接管部位用电测法进行了高温应力测定试验。结果证明两者数值吻合 相似文献
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In this paper, a new fault-tolerant control approach is presented for a class of nonlinear systems, which preserves system stability despite a time delay in fault detection. The faults are assumed to occur in the actuators and are modeled for the general form of affine nonlinear systems. A fault detection and diagnosis (FDD) block is designed based on the multiple model method. The bank of extended Kalman filters (EKF) is used to detect predefined actuator faults and to estimate the unknown parameters of actuator position. The estimated parameters are then used to correct the model of the faulty system and to reconfigure the controller. The reconfigurable controller is designed based on the stabilizing nonlinear model predictive control (NMPC) scheme. On the other hand, in the duration between fault occurrence and fault detection, because of the mismatch between the process and the model, the system states may go off the attraction region. The proposed method is based on designing multiple local controllers for individual predefined faults. Depending on the value of a system variable at the moment of fault detection, one of these controllers will operate. This leads to a stability region of a set of auxiliary equilibrium points (AEPs), which is larger than the attraction region. Moreover, a framework for preserving system stability is presented. Finally, a practical chemical process example is presented to illustrate the effectiveness of this method. 相似文献
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Nonlinear model predictive control (NMPC) scheme is an effective method of multi-objective optimization control in complex industrial systems. In this paper, a NMPC scheme for the wet limestone flue gas desulphurization (WFGD) system is proposed which provides a more flexible framework of optimal control and decision-making compared with PID scheme. At first, a mathematical model of the FGD process is deduced which is suitable for NMPC structure. To equipoise the model's accuracy and conciseness, the wet limestone FGD system is separated into several modules. Based on the conservation laws, a model with reasonable simplification is developed to describe dynamics of different modules for the purpose of controller design. Then, by addressing economic objectives directly into the NMPC scheme, the NMPC controller can minimize economic cost and track the set-point simultaneously. The accuracy of model is validated by the field data of a 1000 MW thermal power plant in Henan Province, China. The simulation results show that the NMPC strategy improves the economic performance and ensures the emission requirement at the same time. In the meantime, the control scheme satisfies the multiobjective control requirements under complex operation conditions (e.g., boiler load fluctuation and set point variation). The mathematical model and NMPC structure provides the basic work for the future development of advanced optimized control algorithms in the wet limestone FGD systems. 相似文献
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Jinfeng Liu Xianzhong Chen David Muñoz de la Peña Panagiotis D. Christofides 《American Institute of Chemical Engineers》2010,56(8):2137-2149
In this work, we focus on distributed model predictive control of large scale nonlinear process systems in which several distinct sets of manipulated inputs are used to regulate the process. For each set of manipulated inputs, a different model predictive controller is used to compute the control actions, which is able to communicate with the rest of the controllers in making its decisions. Under the assumption that feedback of the state of the process is available to all the distributed controllers at each sampling time and a model of the plant is available, we propose two different distributed model predictive control architectures. In the first architecture, the distributed controllers use a one‐directional communication strategy, are evaluated in sequence and each controller is evaluated only once at each sampling time; in the second architecture, the distributed controllers utilize a bi‐directional communication strategy, are evaluated in parallel and iterate to improve closed‐loop performance. In the design of the distributed model predictive controllers, Lyapunov‐based model predictive control techniques are used. To ensure the stability of the closed‐loop system, each model predictive controller in both architectures incorporates a stability constraint which is based on a suitable Lyapunov‐based controller. We prove that the proposed distributed model predictive control architectures enforce practical stability in the closed‐loop system and optimal performance. The theoretical results are illustrated through a catalytic alkylation of benzene process example. © 2010 American Institute of Chemical Engineers AIChE J, 2010 相似文献
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Yash P. Gupta 《加拿大化工杂志》1993,71(4):617-624
In predictive control, control calculations are done such that the difference between the desired and the predicted response of the process is minimized. The number of points on the prediction horizon at which the error is minimized and the number of future control moves considered affect the on-line computational effort involved in the solution of the constrained optimization problem. Earlier papers have shown that the control performance obtained using the DMC algorithm can also be obtained by using a simplified algorithm where the error is minimized at one point and one future control move is calculated. Because of its computational advantages, the simplified algorithm is analyzed further in this paper. Its transfer function is compared with the transfer function of the DMC algorithm. Characteristic equations to select tuning parameters are presented. The paper also compares the robust stability of the simplified and the DMC algorithms on SISO and MIMO process models. The results provide additional support to the viability of the simplified algorithm and thus indicate that it is possible for some processes to benefit from predictive control with only modest computational resources. 相似文献
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Nádson M. N. Lima Lamia Zuñiga Liñan Rubens Maciel Filho Maria R. Wolf Maciel Marcelo Embiruçu Filipe Grácio 《American Institute of Chemical Engineers》2010,56(4):965-978
In this study, a predictive control system based on type Takagi‐Sugeno fuzzy models was developed for a polymerization process. Such processes typically have a highly nonlinear dynamic behavior causing the performance of controllers based on conventional internal models to be poor or to require considerable effort in controller tuning. The copolymerization of methyl methacrylate with vinyl acetate was considered for analysis of the performance of the proposed control system. A nonlinear mathematical model which describes the reaction plant was used for data generation and implementation of the controller. The modeling using the fuzzy approach showed an excellent capacity for output prediction as a function of dynamic data input. The performance of the projected control system and dynamic matrix control for regulatory and servo problems were compared and the obtained results showed that the control system design is robust, of simple implementation and provides a better response than conventional predictive control. © 2009 American Institute of Chemical Engineers AIChE J, 2010 相似文献
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Martin Wijaya Hermanto Richard D. Braatz Min‐Sen Chiu 《American Institute of Chemical Engineers》2011,57(4):1008-1019
Polymorphism, a phenomenon in which a substance can have more than one crystal form, is a frequently encountered phenomenon in pharmaceutical compounds. Different polymorphs can have very different physical properties such as crystal shape, solubility, hardness, color, melting point, and chemical reactivity, so that it is important to ensure consistent production of the desired polymorph. In this study, an integrated batch‐to‐batch and nonlinear model predictive control (B2B‐NMPC) strategy based on a hybrid model is developed for the polymorphic transformation of L ‐glutamic acid from the metastable α‐form to the stable β‐form crystals. The hybrid model comprising of a nominal first‐principles model and a correction factor based on an updated PLS model is used to predict the process variables and final product quality. At each sampling instance during a batch, extended predictive self‐adaptive control (EPSAC) is employed as a NMPC technique to calculate the control action by using the current hybrid model as a predictor. At the end of the batch, the PLS model is updated by utilizing the measurements from the batch and the above procedure is repeated to obtain new control actions for the next batch. In a simulation study using a previously reported model for a polymorphic crystallization with experimentally determined parameters, the proposed B2B‐NMPC control strategy produces better performance, where it satisfies all the state constraints and produces faster and smoother convergence, than the standard batch‐to‐batch strategy. © 2010 American Institute of Chemical Engineers AIChE J, 2011 相似文献
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A number of decentralized and distributed control schemes based on model predictive control (MPC) have been introduced in the last years. They have been proposed as viable solutions to the computational, transmission and robustness issues arising in the centralized context in case of large-scale and/or distributed plants. Such MPC-based control schemes are very heterogeneous, based on different model structures and realizations, with different features and infrastructural/memory/computational requirements.In this paper, we test and compare, with a realistic case study, a robust non-cooperative scheme and a cooperative iterative one. The main scope is to analyze and unravel, in a fair comparison scenario, these methods from different viewpoints, spanning from the model realization issues to the communication and computational requirements, to the control performances. The benchmark case study consists of an existing natural gas refrigeration plant. Realistic simulations and validation tests are obtained through in the DynSim industrial process simulation environment. 相似文献
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Gorazd Karer Gaper Mui
Igor krjanc Borut Zupan
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《Computers & Chemical Engineering》2007,31(12):1552-1564
Processes in industry, such as batch reactors, often demonstrate a hybrid and non-linear nature. Model predictive control (MPC) is one of the approaches that can be successfully employed in such cases. However, due to the complexity of these processes, obtaining a suitable model is often a difficult task. In this paper a hybrid fuzzy modelling approach with a compact formulation is introduced. The hybrid system hierarchy is explained and the Takagi–Sugeno fuzzy formulation for the hybrid fuzzy modelling purposes is presented. An efficient method for identifying the hybrid fuzzy model is also proposed.
A MPC algorithm suitable for systems with discrete inputs is treated. The benefits of the MPC algorithm employing the proposed hybrid fuzzy model are verified on a batch-reactor simulation example: a comparison between MPC employing a hybrid linear model and a hybrid fuzzy model was made. We established that the latter approach clearly outperforms the approach where a linear model is used. 相似文献
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Th. Lorenz J. Diekmann K. Frueh R. Hiddessen J. Moeller J. Niehoff K. Schügerl 《Journal of chemical technology and biotechnology (Oxford, Oxfordshire : 1986)》1987,38(1):41-53
Penicillin V was produced in a 98-dm3 tower loop reactor using a production strain of Penicillium chrysogenum in pellet form. By using control devices, the aeration, the only energy input in a tower loop reactor, decreased by an average of 75%. The amounts of precursor substance (phenoxyacetic acid), acid, base, ammonium sulfate and urea, added during the penicillin fermentation process, were reduced by applying an automatic analysing system to the process. 相似文献