Modelling the effect of air exchange on 222Rn and its progeny concentration in a tunnel atmosphere

The effect of air exchange on the concentration of 222Rn and its progeny in the atmosphere of the Roselend tunnel, in the French Alps, is estimated using a box modelling scheme. In this scheme, the atmosphere is divided into a small number of well mixed zones, separated by flow restricted interfaces, characterized by their exchange rate. A four-box model, representing the three sections of the tunnel present until 2001 and an adjacent inner room, accounts for the spatial variations of the background 222Rn concentration, and for the time structure of transient bursts observed regularly in this tunnel since 1995. A delay of the order of one day, observed during some transient bursts in the inner room with respect to the end of the tunnel, is accounted for if the bursts are assumed to be mainly generated in the end section of the tunnel, and stored temporarily in the inner room via air exchange. The measured radon concentration is reproduced by this model for an air exchange rate of 1.6x10(-6) s-1 between the room and the tunnel, in a context of a global ventilation rate of 10(-5) s-1 in the tunnel. Gradual onset and decay phases, varying from burst to burst, are also suggested. The equilibrium factor of 222Rn with its progeny, measured in 2002 with values varying from 0.60+/-0.05 to 0.78+/-0.06, is interpreted with a five-box model representing the five sections of the tunnel present after 2001. This model indicates that the equilibrium factor does not provide additional constraints on the air exchange rates, but the value of the deposition rate of the unattached short-lived radon progeny can be inferred, with results varying from 0.2 to 6 h-1 in the various sections. This study illustrates the benefits of a simple modelling tool to evaluate the effect of natural ventilation on 222Rn and its progeny concentration in underground cavities, which is important for radioprotection and for a reliable characterization of signatures of hydrogeological or geodynamical processes. Conversely, this study shows that 222Rn and progeny measurements provide a non-invasive method for characterizing natural ventilation conditions in delicate underground cavities, such as painted caves.     

A prediction method for radon in groundwater using GIS and multivariate statistics

Radon (222Rn) in groundwater constitutes a source of natural radioactivity to indoor air. It is difficult to make predictions of radon levels in groundwater due to the heterogeneous distribution of uranium and radium, flow patterns and varying geochemical conditions. High radon concentrations in groundwater are not always associated with high uranium content in the bedrock, since groundwater with a high radon content has been found in regions with low to moderate uranium concentrations in the bedrock. This paper describes a methodology for predicting areas with high concentrations of 222Rn in groundwater on a general scale, within an area of approximately 185x145km2. The methodology is based on multivariate statistical analyses, including principal component analysis and regression analysis, and investigates the factors of geology, land use, topography and uranium (U) content in the bedrock. A statistical variable based method (the RV method) was used to estimate risk values related to different radon concentrations. The method was calibrated and tested on more than 4400 drilled wells in Stockholm County. The results showed that radon concentration was clearly correlated to bedrock type, well altitude and distance from fracture zones. The weighted index (risk value) estimated by the RV method provided a fair prediction of radon potential in groundwater on a general scale. Risk values obtained using the RV method were compared to radon measurements in 12 test areas (on a local scale, each of area 25x25km2) in Stockholm County and a high correlation (r=-0.87) was observed. The study showed that the occurrence and spread of radon in groundwater are guided by multiple factors, which can be used in a radon prediction method on a general scale. However, it does not provide any direct information on the geochemical and flow processes involved.     

Radon and Natural Ventilation in Newer Danish Single-Family Houses

Abstract To investigate the effect of ventilation on indoor radon (²²²Rn), simultaneous measurements of radon concentrations and air change rates were made in 117 Danish naturally ventilated slab-on-grade houses built during the period 1984–1989. Radon measurements (based on CR-39 alpha-track detectors) and air change rate measurements (based on the perfluorocarbon tracer technique; PFT) were in the ranges 12–620 Bq m^?3 and 0.16?0.96 h^?1, respectively. Estimates of radon entry rates on the basis of such time-averaged results are presented and the associated uncertainty is discussed. It was found that differences in radon concentrations from one house to another are primarily caused by differences in radon entry rates whereas differences in air change rates are much less important (accounting for only 80,0% of the house-to-house variation). In spite of the large house-to-house variability of radon entry rates it was demonstrated, however, that natural ventilation does have a significant effect on the indoor radon concentration. Most importantly, it was found that the group of houses with an air change rate above the required level of 0.5 h^?1 on average had an indoor radon concentration that was only 50% (0.5±0.1) of that of the group of houses with air change rates below 0.5 h^?1. The reducing effect of increased natural ventilation on the indoor radon concentration was found to be due mainly to dilution of indoor air. No effect could be seen regarding reduced radon entry rates.     

Radon hazard in shallow groundwaters: Amplification and long term variability induced by rainfall

²²²Rn concentrations have been determined with a RAD7 radon detector in shallow groundwaters of the Pietramelara Plain, north-western Campania, southern Italy, where pyroclastic deposits, along with recent stream alluvial sediments, come in contact with Mesozoic carbonate reservoirs. The aim of this study has been to study the annual variation of ²²²Rn concentration in the shallow groundwaters, scarcely considered in the literature and of obvious relevance for radon hazard evaluation. Our results definitely show that ²²²Rn levels are characterized by a clear annual periodicity, strictly related to rainfall and water table levels, with a pronounced difference between the dry and the wet season. In this last case with concentrations increasing up to two orders of magnitude (up to two times the lower threshold given in the Recommendation 2001/928/EURATOM for public waters). In relation to this, experimental field data will be presented to demonstrate that this variability is due to purely hydrological mechanisms, mainly rinse out and discharge that control leaching efficiency. The detected cycle (Radon Hydrological Amplification Cycle, RHAC) has been generalized for the Mediterranean Tyrrhenian climate. The marked and seasonally persistent amplification in ²²²Rn levels poses the problem of evaluating the epidemiological risk brought up by this previously not yet reported mechanism. This mechanism, occurring in shallow groundwaters, very likely should strongly influence indoor radon levels via groundwater-soil-building exchange.     

222Rn concentrations in greenhouses in Aomori Prefecture, Japan

Greenhouses are possible places with high 222Rn concentrations, since soil, the source of 222Rn, is directly exposed inside them. To examine this point, 222Rn concentrations in 28 greenhouses at five locations in Aomori Prefecture were measured for approximately 1 year with passive Rn detectors. For 1 week, measurements of 222Rn concentration and working level were also carried out with active detectors to get equilibrium factors and the ratio of 222Rn concentration in working time to non-working time in selected greenhouses. The geometric mean of annual 222Rn concentrations in greenhouses was 13 Bq m-3, and the same as that in dwellings and lower than that in indoor workplaces in the prefecture. However, variation of the 222Rn concentrations was far larger than in other environments, and ranged from the lowest level in outdoor workplaces to the highest level in indoor workplaces. Significant seasonal variation was also observed in 222Rn concentrations. The mean effective dose from 222Rn and its progenies was estimated to be 0.047 mSv year-1 for a farmer working in a greenhouse.     

Meteorological parameters contributing to variability in 222Rn activity concentrations in soil gas at a site in Sapporo, Japan

Continuous ²²²Rn monitoring in soil gas since November 22, 2004 has revealed variability in activity concentration with time in the semi-natural woods on the campus of Hokkaido University in Sapporo, Japan. Among various factors affecting soil radon levels and variability, temperature was found to be dominant during three seasons when activity concentrations of ²²²Rn showed a diurnal high and nocturnal low with a boundary around 10 o'clock in the morning. This pattern was disturbed by low pressure fronts with occasional rain. The activity gradually decreased as soil temperatures decreased from late November to mid-December. After the ground surface was completely covered with snow, soil radon levels became low with a small fluctuation. There were several peaks of ²²²Rn on the time-series chart in winter. Those peaks appearing in early winter and early spring may be interpreted by considering meteorological parameters. In a few cases, the radon activity suddenly increased with increasing pressure in the soil at a depth of 10 cm, which may be associated with subsurface events such as seismic activity in the area.     

Impact of constructional energy‐saving measures on radon levels indoors

Energy‐efficient building refurbishment has the aim of saving energy and thus reducing CO₂ emissions. Increased energy efficiency of a building often implies reduced air exchange. Together with other indoor air quality problems, this may lead to an increase in indoor radon concentration (Rn‐222). In order to investigate the extent of this problem, measurements of radon concentration in energy‐efficient refurbished and low‐energy houses (passive houses) were carried out. Track etch detectors were exposed in each type of building over a period of 1 year. A reference sample of non‐refurbished non‐passive buildings was drawn from the National Radon Database for comparison. Buildings were selected that have the same radon relevant properties and were built on comparable geological subsoil like those investigated. The reference sample was compiled in such a way that the measured values from the rooms on the ground floor of the refurbished and passive houses were each assigned a measured value from the database. The statistical analysis shows that the houses refurbished for energy efficiency have a wider distribution of radon concentrations indoors than the non‐refurbished ones. Both the mean value and the median of the radon concentration have nearly doubled in buildings refurbished for energy efficiency. The difference is statistically significant. On the other hand, there is no significant difference between the distributions of passive houses and houses not refurbished for energy efficiency.     

Increased radon concentrations in classrooms used for pottery workshops.

In a pilot study of nine schools the radon (Rn) concentrations were measured systematically. The mean radon concentrations in the classrooms on the ground-floor and on higher floors was 52 Bq/m3, which is equivalent to the mean values in Central Europe. Several of the basement rooms used for handicraft lessons had significantly increased Rn levels with a mean concentration of 617 Bq/m3. In all other parts of the basement Rn levels were clearly lower with a mean concentration of 136 Bq/m3. In the rooms used for handicraft lessons numerous articles of pottery were on display. After removing these the Rn in air concentration was reduced to a mean value of 83 Bq/m3.     

Radon hazard in shallow groundwaters II: dry season fracture drainage and alluvial fan upwelling

²²²Rn concentrations have been measured in a well located on the edge of a large Pleistocene-Holocene fan and belonging to the shallow pyroclastic aquifer of the Pietramelara Plain, southern Italy. The aim of this study has been both to characterise the hydrological inputs that determine the influx of ²²²Rn to the shallow aquifer and to understand the correlations between ²²²Rn, major ions, physical-chemical parameters and rainfall. Results obtained from the time series indicate that the studied well shows a ²²²Rn variability that is inconsistent with a mechanism of pure hydrological amplification, such as described in Radon hazard in shallow groundwaters: Amplification and long term variability induced by rainfall (De Francesco et al., 2010a). On the contrary, in this well hydrological amplification appears to be mainly tied to the upwelling of alluvial fan waters, rich in radon, in response to pistoning from recharge in the carbonate substrate. This upwelling of alluvial fan waters occurs during almost the whole period of the annual recharge and is also responsible of the constant increase in ²²²Rn levels during the autumn-spring period, when both the water table level and weekly rainfall totals drop. Furthermore, a rapid delivery mechanism for ²²²Rn likely operates through fracture drainage in concomitance with the very first late summer-early autumn rains, when rainfall totals appear largely insufficient to saturate the soil storage capacity. Results obtained from this study appear to be particularly significant in both radon hazard zoning in relation to the shallow aquifer and possibly also for indoor radon, owing to possible shallow aquifer-soil-building exchanges. Moreover, both the spike-like events and the long wave monthly scale background fluctuations detected can also have potential significance in interpreting ²²²Rn time series data as seismic and/or volcanic precursors. Finally, ²²²Rn has proved to be an excellent tracer for hydrological inputs to the shallow aquifer when combined with major ions, physical-chemical data and geological and geomorphological controls.     

Temporal and small-scale spatial variability of Rn gas in a soil with a high gravel content

To quantify the small-scale spatial and long-term temporal variability of the ²²²Rn concentration in a typical soil with a high gravel content, we monitored this radionuclide every week for 1 year, at 0.5 m and 1.0 m depth at nine sampling positions in a 20×20-m field, and at the four corners of a 1×1-m plot within this field. The data show that the ²²²Rn soil gas concentrations exhibited a spatial variability which is characterised in the 20×20-m field by coefficients of variation from 20 to 30% at 0.5 m depth, and from 15 to 20% at 1.0 m depth. Within the 1×1-m plot, these values were at both depths only 5–10%. In the winter months, the ²²²Rn soil gas concentration was higher at 0.5 m depth compared to that at 1.0 m depth. However, in the summer months, the opposite behavior was observed. Time series analysis of the data showed that the ²²²Rn concentrations in the soil gas determined at a given position and depth is strongly correlated with the preceding observation at this point. In addition, strong cross-correlations are present between the ²²²Rn concentration time series observed at different positions and depths. The above results are used to calculate the probability for estimating, within a given deviation, the annual mean ²²²Rn soil gas concentration from a single measurement on an arbitrary day of a given month at a limited number of sampling positions only. Because the ²²²Rn concentration in the soil gas can vary considerably even within 1 month, ²²²Rn measurement obtained only once in a given month (especially in January and February) cannot be used to obtain a good estimate of the mean annual radon concentration, even if a large number of samples in the field are taken.     

Geothermal ground gas emissions and indoor air pollution in Rotorua, New Zealand

The emission of toxic gases from the soil is a hazard in geothermal regions that are also urbanized because buildings constructed on geothermal ground may be subject to the ingress of gases from the soil directly into the structure. The Rotorua geothermal field, New Zealand, is extensively urbanized but to date no studies have evaluated the extent of the ground gas hazard. The main gases emitted are hydrogen sulphide (H2S) and carbon dioxide (CO2), both of which are highly toxic and denser than air. This paper reports preliminary findings from a study of selected buildings constructed in the gas anomaly area. Properties were investigated for evidence of ingress by H2S, CO2, and 222Rn, with a view to determine the means and rates of gas entry and the nature of any consequent hazard. H2S and CO2 were investigated using infrared active gas analysers and passive detector tubes left in place for 10-48 h. 222Rn was measured over a period of 3 months by poly-allyl diglycol carbonate sensors. Eight of the nine buildings studied were found to suffer problems with soil gases entering the indoor air through the structure. The primary means of gas entry was directly from the ground through the floors, walls, and subsurface pipes. Indoor vents were located and found emitting up to approximately 200 ppm H2S and approximately 15% CO2, concentrations high enough to present an acute respiratory hazard to persons close to the vent (e.g., children playing at floor level). In some properties, gas problems occurred despite preventative measures having been made during construction or during later renovations. Typically, these measures include the under-laying of concrete floors with a gas-proof butanol seal, under-floor ventilation systems or the installation of positive-pressure air conditioning. Recently constructed buildings (<10 years) with butanol seals were nevertheless affected by ground gas emissions, and we conclude that such measures are not always effective in the long term.     

Use of 222radon as a simple tool for surface water–groundwater connectivity assessment: a case study in the arid Limarí basin,north‐central Chile

We report the results from a pilot study on the use of ²²²Rn (²²²radon) for river–aquifer interaction assessment in the Limarí watershed, north‐central Chile. Previous studies on this tool for such applications are not abundant at international level, and no records exist for Chile. The lowest ²²²Rn levels (less than 1000 Bq/m³) were found in water reservoirs, thus indicating that this isotope is easily lost (and therefore usually absent) in surface waters. Conversely, the highest levels of ²²²Rn were found in groundwater, with maxima activities around 20 000 Bq/m³. This remarkable contrast allowed clear identification of zones of surface water–groundwater connectivity in the searched watershed domain.     

Experience from retrospective radon exposure estimations for individuals in a radon epidemiological study using solid-state nuclear track detectors

The relation between increased risk of lung cancer and exposure to indoor radon is assessed in epidemiological studies. Both the quality and reliability of smoking data and the radon exposure data are of primary importance. Contemporary measurement of radon concentration in the dwellings of individuals in a case-control study is traditionally used to assess past history of radon exposure. These assessments are somewhat unreliable since presently measured radon concentration might not be representative for a given location long ago. The measurement of long-lived decay products from 222Rn remaining indoors on hard surfaces, such as glass, makes it possible to assess the exposure to indoor radon. At the Swedish Radiation Protection Institute, a combination of two different solid-state nuclear track detectors has been developed to assess the 210Pb activity implanted in glass surfaces by measuring 210Po alpha activity. This detector (a RETRO detector) is used in the Swedish radon epidemiological case-control study of non-smokers with the aim to provide an alternative estimate of individual radon exposure and to evaluate the usefulness of RETRO measurements. A total of 576 different objects were found and 568 were measured. For 225 individuals, we measured two personal objects that had been in the same person's possession for more than 20 years. The standard deviation of the average radon concentration obtained from these two objects had a median value of 13 Bq/m3 indicating a precision of exposure of approximately 20%. The correlation between 210Po surface activity measured earlier and the mean values of radon concentrations in a number of Swedish dwellings is used to estimate the historical, average radon concentration. This average correlation factor seems also to be valid for measurements in the non-smoker epidemiological study.     

浅析水产加工车间低温空调的设计

通过对氟利昂直接膨胀式系统和乙二醇／盐水系统这两种空调方式的分析，探讨了这两种系统在水产加工车间低温空调应用中的各自优缺点，强调了在水产加工车间空调设计中应注意的一些要点。     

空调室内氡及粒子污染的传播及其数值模拟

室内氡(含氡子体)污染的传播与粒子(悬浮颗粒)污染在室内的传播过程相关,通风空调气流对氡及粒子污染的传播影响很大。本文详细阐述了室内氡和粒子的来源和特点、氡及其子体在空气中的传播机理以及除去方法,分析了通风空调系统对室内氡及子体传输的影响、以及氡在空气中迁移的动力学模型,分析比较了通风室内氡及粒子污染物迁移沉降过程的数值模拟方法,提出了空调气流环境下氡及粒子污染传播及其数值模拟中的关键问题。     

Radon risk management: the future challenge for the nuclear community

The short-lived decay products (Rn-d) of radon gas (222Rn, 220Rn) have been identified as a health hazard in occupational exposure situations, as well as a public health risk in general. Decisions will have to be made concerning the initiation and scale of national Rn-mitigation programmes. In view of the potentially significant socio-economic impact of such programmes, it is recommended to proceed from the current approach based on Rn-d risk assessment to the integrated approach of radon risk management (RRM). A seven-step RRM is proposed, ranging from the selection of an action level based on an incremental risk-reduction, to the conduct of auditing procedures, monitoring the RRM-outreach factor.     

In situ gamma spectroscopy to characterize building materials as radon and thoron sources

In situ gamma spectroscopy is widely utilized to determine the outdoor gamma dose rate from the soil and to calculate the natural and artificial radionuclide concentration and their contribution to the dose rate. The application of in situ gamma spectroscopy in indoor environments can not supply quantitative information about activity concentration of radionuclides in building materials, but this technique can provide interesting information about building materials as radon source. In fact, a method based on analyses of gamma spectra data has been developed by the authors to provide, in field, quantitative estimation of disequilibrium in 226Ra and 228Ac sub-chains due to 222Rn and 220Rn exhalation. The method has been applied to data of gamma spectroscopy measurements carried out with HPGe detector (26%) in seven dwellings and one office in Rome. The first results of the data analysis show that, as regards especially the 226Ra sub-chain disequilibrium, different building materials (tuff, concrete, etc.) can show very different characteristics. If, in addition to the spectrometric data, other indoor environment parameters (indoor gamma dose rates, room dimensions, wall thickness, etc.) (Bochicchio et al., Radiat Prot Dosim 1994;56(1-4):137-140; Bochicchio et al., Environ Int 1996a;22:S633-S639) are utilized in a room model, an evaluation of 226Ra, 228Ac and 40K activity concentration and an indication of the exhalation features, by means of estimation of exhaled 222Rn activity concentration, can be achieved.     

Radon and 'King Solomon's Miners': Faynan Orefield, Jordanian Desert

Concentrations of 222Rn were measured in ancient copper mines which exploited the Faynan Orefield in the South-Western Jordanian Desert. The concentrations of radon gas detected indicate that the ancient metal workers would have been exposed to a significant health risk and indicate that any future attempt to exploit the copper ores must deal with the hazard identified. Seasonal variations in radon concentrations are noted and these are linked to the ventilation of the mines. These modern data are used to explore the differential exposure to radon and the health of ancient mining communities.     

Evaluation of distributed environmental control systems for improving IAQ and reducing energy consumption in office buildings

Conventional heating, ventilation, and air conditioning (HVAC) systems are incapable of providing control over individual environments or adjusting fresh air supply based on the dynamic occupancy of individual rooms in an office building. This paper introduces the concept of distributed environmental control systems (DECS) and shows that improvement in indoor air quality (IAQ) and energy efficiency can be achieved by providing required amounts of fresh air directly to the individual office spaces through distributed demand controlled ventilation (DDCV). In DDCV, fresh air is provided to each micro-environment (room or cubicle) based on input from distributed sensors (CO₂, VOC, occupancy, etc.) or intelligent scheduling techniques to provide acceptable IAQ for each occupant, rather than for groups or populations of occupants. In order to study DECS, a numerical model was developed that incorporates some of the best available models for studying building energy consumption, indoor air flow, contaminant transport and HVAC system performance. The developed model was applied to a DECS in a model office building equipped with a DDCV system. By implementing DECS/DDCV and intelligent scheduling techniques it is possible to achieve an improvement in IAQ along with a reduction in annual energy consumption compared to conventional ventilation systems.     

机场航站楼暖通空调设计探讨

阐述了太原武宿机场航站楼的基本情况及暖通空调设计思路,提出了采暖和空调两套系统并用的方法,以此为基础详细探讨了空调风系统、空调水系统、采暖系统、自动控制系统、通风及防排烟系统等暖通空调主要组成部分的设计,以供参考借鉴。