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Cluster-assisted generation of multicharged ions in nanosecond laser ionization of carbon bisulfide clusters at 1064nm
作者姓名:肖 雪  李海洋  牛冬梅  罗晓琳
作者单位:Key Laboratory of Environmental Optics and Technology, Anhui Institute of Optics and Fine Mechanics,Chinese Academy of Sciences, Hefei 230031, China;Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, China;Key Laboratory of Environmental Optics and Technology, Anhui Institute of Optics and Fine Mechanics,Chinese Academy of Sciences, Hefei 230031, China;Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, China;Key Laboratory of Environmental Optics and Technology, Anhui Institute of Optics and Fine Mechanics,Chinese Academy of Sciences, Hefei 230031, China;Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, China
基金项目:Project supported by the National Natural Science Foundation of China (Grant No 20573111) and the Centre for Computational Science, Hefei Institutes of Physics, China (Grant No 0331405002).
摘    要:

关 键 词:  二硫化物  库仑  炸药
文章编号:1009-1963/2007/16(12)/3655-07
收稿时间:2006-11-23
修稿时间:2007-05-15

Cluster-assisted generation of multicharged ions in nanosecond laser ionization of carbon bisulfide clusters at 1064nm
Xiao Xue,Li Hai-Yang,Niu Dong-Mei and Luo Xiao-Lin.Cluster-assisted generation of multicharged ions in nanosecond laser ionization of carbon bisulfide clusters at 1064nm[J].Chinese Physics B,2007,16(12):3655-3661.
Authors:Xiao Xue  Li Hai-Yang  Niu Dong-Mei and Luo Xiao-Lin
Affiliation:Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, China; Key Laboratory of Environmental Optics and Technology, Anhui Institute of Optics and Fine Mechanics,Chinese Academy of Sciences, Hefei 230031, China; Key Laboratory of Environmental Optics and Technology, Anhui Institute of Optics and Fine Mechanics,Chinese Academy of Sciences, Hefei 230031, China;Dalian Institute of Chemical Physics, Chinese Academy of Sciences, Dalian 116023, China
Abstract:The photoionization of seeded carbon bisulfide molecular beam by a 1064\,nm nanosecond Nd-YAG laser with intensities varying from $0.8\times10^{11}$ to $5.6\times10^{11}$\,W/cm$^{2}$ have been studied by time-of-flight mass spectrometry. Multiply charged ions of S$^{q + }$ ($q$ = 2--6) and C$^{q +}$ ($q$ = 2--4) with kinetic energy of hundreds of electron volts have been observed, and there are strong experimental evidences indicating that those multicharged ions originate from the ionization of CS$_{2}$ neat clusters in the beam. An electron recolliding ionization model is proposed to explain the appearance of those multiply charged atomic ions under such low laser intensities.
Keywords:carbon bisulfide  multicharged ions  cluster  coulomb explosion
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