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Facile fabrication of g‐C3N4/MIL‐53(Al) composite with enhanced photocatalytic activities under visible‐light irradiation
Authors:Di Guo  Rongying Wen  Minmin Liu  Hongxu Guo  Jianhua Chen  Wen Weng
Affiliation:College of Chemistry and Environment, Minnan Normal University, Zhangzhou, PR China
Abstract:A novel visible‐light‐driven g‐C3N4/MIL‐53(Al) composite photocatalyst was successfully prepared using a facile stirring method at room temperature. The g‐C3N4/MIL‐53(Al) composites were characterized and their effects on the photocatalytic activities for rhodamine B degradation were investigated. The g‐C3N4(20 wt%)/MIL‐53(Al) photocatalyst displayed optimal photocatalytic degradation efficiency, which was about five times higher than the photocatalytic activity of pure g‐C3N4. The improved photocatalytic performance of the g‐C3N4/MIL‐53(Al) photocatalyst was predominantly attributed to the efficient separation of electron–hole pairs and the low charge‐transfer resistance. g‐C3N4/MIL‐53(Al) also exhibited excellent stability and reusability. A proposed mechanism for the enhanced photocatalytic activity is also discussed based on the experimental results. Copyright © 2015 John Wiley & Sons, Ltd.
Keywords:g‐C3N4/MIL‐53(Al)  composite  photocatalytic degradation  rhodamine B  mechanism
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